G. Cantarella, Sudhir Kumar, J. Jagielski, C. Shih, G. Tröster
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引用次数: 4
摘要
柔性钙钛矿发光二极管(led)在实现超薄、轻量、高适应性和不易损坏的生动显示方面受到越来越多的关注。溶液处理卤化铅钙钛矿提供了许多独特的特点,如纯净的发射色,可调的带隙,和低制造成本。在这封信中,绿色钙钛矿led (PeLEDs)是在50 μm薄的聚酰亚胺衬底上制造的。采用胶体二维甲脒基溴化铅钙钛矿发射体制备的等离子体具有较高的电流效率(ηCE)为5.3 cd a−1,峰值发射波长为529±1 nm,窄宽度为22.8 nm。由此产生的绿色辐射在Rec. 2020标准色域区域显示出创纪录的高色彩饱和度,> 95%。为了证明其机械灵活性,通过动态弯曲实验证明了该器件的功能,该器件在手套箱中使用寿命超过36小时,ηCE和外部量子效率(ηxt)分别下降了15%和18%。
Flexible perovskite light-emitting diodes (LEDs) have attracted increasing interest to realize ultrathin, light weight, highly conformable and nonfragile vivid displays. Solution-processed lead halide perovskite offers numerous distinctive characteristics such as pure emission color, tunable bandgaps, and low fabrication cost. In this letter, green perovskite LEDs (PeLEDs) are fabricated on 50 μm thin polyimide substrates. Using colloidal 2D formamidinium lead bromide perovskite emitter, the PeLEDs show a high current efficiency (ηCE) of 5.3 cd A−1 with a peak emission at 529 ± 1 nm and a narrow width of 22.8 nm. The resultant green emission shows a record high color saturation, > 95%, in the Rec. 2020 standard gamut area. To demonstrate their mechanical flexibility, the device functionality is proved by dynamic bending experiments down to 10 mm up to 5000 cycles, resulting in device lifetime over 36 h in glove box and a drop of ηCE and external quantum efficiency (ηxt) as low as 15 % and 18 %, respectively.