Jianguo Qin , Yaping Zhang , Chuanxin Zhu , Caifeng Lai , Kai Li , Tonghua Zhu , Li An , Xinxin Lu , Yunfeng Mu
{"title":"反应堆中子环境中93mNb活度测量中182Ta和94Nb贡献的快速减去方法","authors":"Jianguo Qin , Yaping Zhang , Chuanxin Zhu , Caifeng Lai , Kai Li , Tonghua Zhu , Li An , Xinxin Lu , Yunfeng Mu","doi":"10.1016/j.nucana.2022.100009","DOIUrl":null,"url":null,"abstract":"<div><p>Niobium is one of the most important neutron dosimeters used outside of the reactor. Owing to the fluorescence effects of <sup>182</sup>Ta and <sup>94</sup>Nb radionuclides, it is a problem to quickly obtain the activity of <sup>93m</sup>Nb which produced by the neutron inelastic scattering of Nb. To solve this problem, a fast estimating method based on the Monte Carlo simulation is proposed. All the contributions from fluorescence effects that induced by gamma-rays, beta-rays and internal conversion electrons of the radionuclides in the niobium sample were considered. The comparison results demonstrated that the deviation is less than 8.0% between the calculated and the experimental activities. It shows that the contribution of radionuclide by fluorescence effects in activity measurement of the niobium sample can be subtracted quickly using this method, based just once experimental measurement.</p></div>","PeriodicalId":100965,"journal":{"name":"Nuclear Analysis","volume":null,"pages":null},"PeriodicalIF":0.0000,"publicationDate":"2022-06-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.sciencedirect.com/science/article/pii/S277318392200009X/pdfft?md5=bd099c31c32008530bbaab49b7767d3d&pid=1-s2.0-S277318392200009X-main.pdf","citationCount":"0","resultStr":"{\"title\":\"A method for quickly subtracting the contributions from 182Ta and 94Nb in activity measurement of 93mNb in reactor neutron environment\",\"authors\":\"Jianguo Qin , Yaping Zhang , Chuanxin Zhu , Caifeng Lai , Kai Li , Tonghua Zhu , Li An , Xinxin Lu , Yunfeng Mu\",\"doi\":\"10.1016/j.nucana.2022.100009\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<div><p>Niobium is one of the most important neutron dosimeters used outside of the reactor. Owing to the fluorescence effects of <sup>182</sup>Ta and <sup>94</sup>Nb radionuclides, it is a problem to quickly obtain the activity of <sup>93m</sup>Nb which produced by the neutron inelastic scattering of Nb. To solve this problem, a fast estimating method based on the Monte Carlo simulation is proposed. All the contributions from fluorescence effects that induced by gamma-rays, beta-rays and internal conversion electrons of the radionuclides in the niobium sample were considered. The comparison results demonstrated that the deviation is less than 8.0% between the calculated and the experimental activities. It shows that the contribution of radionuclide by fluorescence effects in activity measurement of the niobium sample can be subtracted quickly using this method, based just once experimental measurement.</p></div>\",\"PeriodicalId\":100965,\"journal\":{\"name\":\"Nuclear Analysis\",\"volume\":null,\"pages\":null},\"PeriodicalIF\":0.0000,\"publicationDate\":\"2022-06-01\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"https://www.sciencedirect.com/science/article/pii/S277318392200009X/pdfft?md5=bd099c31c32008530bbaab49b7767d3d&pid=1-s2.0-S277318392200009X-main.pdf\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Nuclear Analysis\",\"FirstCategoryId\":\"1085\",\"ListUrlMain\":\"https://www.sciencedirect.com/science/article/pii/S277318392200009X\",\"RegionNum\":0,\"RegionCategory\":null,\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"\",\"JCRName\":\"\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Nuclear Analysis","FirstCategoryId":"1085","ListUrlMain":"https://www.sciencedirect.com/science/article/pii/S277318392200009X","RegionNum":0,"RegionCategory":null,"ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"","JCRName":"","Score":null,"Total":0}
A method for quickly subtracting the contributions from 182Ta and 94Nb in activity measurement of 93mNb in reactor neutron environment
Niobium is one of the most important neutron dosimeters used outside of the reactor. Owing to the fluorescence effects of 182Ta and 94Nb radionuclides, it is a problem to quickly obtain the activity of 93mNb which produced by the neutron inelastic scattering of Nb. To solve this problem, a fast estimating method based on the Monte Carlo simulation is proposed. All the contributions from fluorescence effects that induced by gamma-rays, beta-rays and internal conversion electrons of the radionuclides in the niobium sample were considered. The comparison results demonstrated that the deviation is less than 8.0% between the calculated and the experimental activities. It shows that the contribution of radionuclide by fluorescence effects in activity measurement of the niobium sample can be subtracted quickly using this method, based just once experimental measurement.
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