Pub Date : 2025-12-17DOI: 10.1016/j.nucana.2025.100213
Najeba Farhad Salih , Hiwa Mohammad Qadr
This investigation assessed indoor radon concentrations across 11 laboratories using CR-39 solid-state nuclear track detectors to measure alpha particle emissions. Following exposure, detectors were chemically etched in 6.25 N sodium hydroxide solution at 70.0 ± 0.5 °C for 8 h to visualize alpha tracks, which were subsequently examined via optical microscopy. Measurements demonstrated considerable variability in radon levels between laboratories, even among those situated on identical floors. Radon concentrations ranged from 38.99 Bq m−3 (Laboratory 11, third floor) to 61.66 Bq m−3 (Laboratory 3, ground floor), yielding a mean value of 47.48 Bq m−3. Correspondingly, annual effective doses varied from 0.99 mSv y−1 to 1.56 mSv y−1, with an average of 1.20 mSv y−1. These dose estimates remained substantially below ICRP recommended reference range of 3–10 mSv y−1. Excess lifetime cancer risk calculations showed values between 3.786 × 10−3 (Laboratory 11) and 5.989 × 10−3 (Laboratory 3). A statistically significant variation in radon concentration was also observed across different age groups (P-value <0.001). Critically, all measured concentrations fell below the UNSCEAR safety threshold of 200 Bq m−3, confirming that laboratory occupants face negligible health risks from radon exposure. The findings indicate no actionable radon hazards in the studied facilities.
{"title":"Evaluating the health impact of indoor radon concentration in laboratory environments: a focus on lung cancer risk","authors":"Najeba Farhad Salih , Hiwa Mohammad Qadr","doi":"10.1016/j.nucana.2025.100213","DOIUrl":"10.1016/j.nucana.2025.100213","url":null,"abstract":"<div><div>This investigation assessed indoor radon concentrations across 11 laboratories using CR-39 solid-state nuclear track detectors to measure alpha particle emissions. Following exposure, detectors were chemically etched in 6.25 N sodium hydroxide solution at 70.0 ± 0.5 °C for 8 h to visualize alpha tracks, which were subsequently examined via optical microscopy. Measurements demonstrated considerable variability in radon levels between laboratories, even among those situated on identical floors. Radon concentrations ranged from 38.99 Bq m<sup>−3</sup> (Laboratory 11, third floor) to 61.66 Bq m<sup>−3</sup> (Laboratory 3, ground floor), yielding a mean value of 47.48 Bq m<sup>−3</sup>. Correspondingly, annual effective doses varied from 0.99 mSv y<sup>−1</sup> to 1.56 mSv y<sup>−1</sup>, with an average of 1.20 mSv y<sup>−1</sup>. These dose estimates remained substantially below ICRP recommended reference range of 3–10 mSv y<sup>−1</sup>. Excess lifetime cancer risk calculations showed values between 3.786 × 10<sup>−3</sup> (Laboratory 11) and 5.989 × 10<sup>−3</sup> (Laboratory 3). A statistically significant variation in radon concentration was also observed across different age groups (<em>P</em>-value <0.001). Critically, all measured concentrations fell below the UNSCEAR safety threshold of 200 Bq m<sup>−3</sup>, confirming that laboratory occupants face negligible health risks from radon exposure. The findings indicate no actionable radon hazards in the studied facilities.</div></div>","PeriodicalId":100965,"journal":{"name":"Nuclear Analysis","volume":"5 1","pages":"Article 100213"},"PeriodicalIF":0.0,"publicationDate":"2025-12-17","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145924684","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2025-12-12DOI: 10.1016/j.nucana.2025.100212
Tuqa Haider Al-Zaalimiu , Anees Ali Al-Hamzawi
Uranium (U) is a heavy metal with chemical toxicity and radiological hazards. Chronic exposure, even at low concentrations, may contribute to serious health risks, including cancer. For this reason, it was necessary to measure the uranium content (UC) in blood samples of two groups of women (healthy and cancer patients) residing in the city center of Al-Muthanna Governorate. The Fission Track Analysis (FTA) technique with a CR-39 detector was applied to evaluate the UC in blood samples. Statistical comparisons between concentrations were performed using an independent t-test (p ≤ 0.05). The result illustrates that the UC in blood samples of the healthy women ranged from (0.74 ± 0.04 to 2.22 ± 0.04) with an average value equal to 1.14 ± 0.06 μg/l. In contrast, the UC for the cancer group ranged from (1.70 ± 0.04 to 4.22 ± 0.06) μg/l, with the mean value equal to 2.93 ± 0.05 μg/l. The findings revealed statistically significant differences (p < 0.001) in UC between the two groups, suggesting a correlation between the incidence of cancer in Iraqi women and elevated levels of UC in their blood. Preliminary observation showed higher UC among women working in the health sector (1.50 μg/l for healthy women and 3.59 μg/l for patients) compared to women in other occupations included in this study. Indicating a potential relationship between occupation type and increased UC. However, this association remains unconfirmed and requires further studies.
{"title":"Estimating the uranium content in blood samples of healthy and cancer-affected women in the city center of Al-Muthanna governorate, Iraq","authors":"Tuqa Haider Al-Zaalimiu , Anees Ali Al-Hamzawi","doi":"10.1016/j.nucana.2025.100212","DOIUrl":"10.1016/j.nucana.2025.100212","url":null,"abstract":"<div><div>Uranium (U) is a heavy metal with chemical toxicity and radiological hazards. Chronic exposure, even at low concentrations, may contribute to serious health risks, including cancer. For this reason, it was necessary to measure the uranium content (UC) in blood samples of two groups of women (healthy and cancer patients) residing in the city center of Al-Muthanna Governorate. The Fission Track Analysis (FTA) technique with a CR-39 detector was applied to evaluate the UC in blood samples. Statistical comparisons between concentrations were performed using an independent <em>t</em>-test (p ≤ 0.05). The result illustrates that the UC in blood samples of the healthy women ranged from (0.74 ± 0.04 to 2.22 ± 0.04) with an average value equal to 1.14 ± 0.06 μg/l. In contrast, the UC for the cancer group ranged from (1.70 ± 0.04 to 4.22 ± 0.06) μg/l, with the mean value equal to 2.93 ± 0.05 μg/l. The findings revealed statistically significant differences (p < 0.001) in UC between the two groups, suggesting a correlation between the incidence of cancer in Iraqi women and elevated levels of UC in their blood. Preliminary observation showed higher UC among women working in the health sector (1.50 μg/l for healthy women and 3.59 μg/l for patients) compared to women in other occupations included in this study. Indicating a potential relationship between occupation type and increased UC. However, this association remains unconfirmed and requires further studies.</div></div>","PeriodicalId":100965,"journal":{"name":"Nuclear Analysis","volume":"5 1","pages":"Article 100212"},"PeriodicalIF":0.0,"publicationDate":"2025-12-12","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145790611","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2025-12-11DOI: 10.1016/j.nucana.2025.100205
O.V. Chakilev, S.V. Kolesnikov, S.G. Rudakov
The determination of gadolinium in aqueous solution was carried out using a DT portable pulsed neutron generator and a 7.6 × 7.6 cm detector. The pulse mode of the acquisition process allows the separation of the registration of radiation capture, inelastic scattering and induced activity. The technique is based on the registration of secondary gamma radiation of the sample from the thermal neutron capture reaction. After correction of the neutron self-absorption effect, the nonlinear response between peak areas and Gd concentrations was converted to a linear response, and calibration curves were used to determine the minimum detection concentration (MDC). Significant improvements in gadolinium detection are achieved, and the MDC of Gd in 300 ml of aqueous solution was 11 ppm.
采用DT便携式脉冲中子发生器和∅7.6 × 7.6 cm LaBr3探测器对水溶液中的钆进行测定。采集过程的脉冲模式允许分离辐射捕获、非弹性散射和诱导活度的登记。该技术是基于从热中子捕获反应的样品的二次伽马辐射的登记。校正中子自吸收效应后,将峰面积与Gd浓度之间的非线性响应转化为线性响应,利用标定曲线确定最小检测浓度(MDC)。在300 ml水溶液中,钆的检测得到了显著的改进,其MDC为11 ppm。
{"title":"Determination of gadolinium in leachate by PGNAA","authors":"O.V. Chakilev, S.V. Kolesnikov, S.G. Rudakov","doi":"10.1016/j.nucana.2025.100205","DOIUrl":"10.1016/j.nucana.2025.100205","url":null,"abstract":"<div><div>The determination of gadolinium in aqueous solution was carried out using a DT portable pulsed neutron generator and a <span><math><mi>∅</mi></math></span>7.6 × 7.6 cm <span><math><mi>L</mi><mi>a</mi><mi>B</mi><msub><mi>r</mi><mn>3</mn></msub></math></span> detector. The pulse mode of the acquisition process allows the separation of the registration of radiation capture, inelastic scattering and induced activity. The technique is based on the registration of secondary gamma radiation of the sample from the thermal neutron capture reaction. After correction of the neutron self-absorption effect, the nonlinear response between peak areas and Gd concentrations was converted to a linear response, and calibration curves were used to determine the minimum detection concentration (MDC). Significant improvements in gadolinium detection are achieved, and the MDC of Gd in 300 ml of aqueous solution was 11 ppm.</div></div>","PeriodicalId":100965,"journal":{"name":"Nuclear Analysis","volume":"5 1","pages":"Article 100205"},"PeriodicalIF":0.0,"publicationDate":"2025-12-11","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145790612","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2025-12-01DOI: 10.1016/j.nucana.2025.100202
Ranjbar Hassan , Bagheri Reza , Janjani Iman
Objective
For many years, different ligands have been combined with rhenium therapeutic radioisotopes, specifically rhenium-186 and 188, to create radiopharmaceuticals for the treatment of various illnesses. Because of the unique qualities that set each of these radioisotopes apart, they can all be used to eradicate different kinds of cancers. Large cancers can be effectively removed in 188Re thanks to the use of great-energy, long-distance beta particles. However, 186Re's short range, low energy beta particles are a sufficient weapon to destroy tiny tumors with a high yield and little side effects. As a result, the properties of each of these radioisotopes can only partially address the therapy on their own. Therefore, we reasoned that 188Re and 186Re in conjunction must provide the greatest results when treating tumors of different sizes. One possible outcome of neutron-irradiation of natural rhenium is the simultaneous production of 186Re and 188Re.
Methods
We want to know if the natural irradiation of rhenium, together with the simultaneous synthesis of these radioisotopes, provides us with the right amounts of radioactivity to make compositional radiopharmaceuticals. This study examines the kind and quantity of impurities created, as well as the practical and theoretical evaluations of the simultaneous generation of 188Re and 186R to achieve compositional radiopharmaceuticals by neutron irradiation of natural rhenium in 5MWt pool-type light water research reactor.
Results
The outcomes demonstrated that the theoretical computations and experimental data correlate well. The data's greatest relative error has been determined to be 8 %.
Conclusion
The findings shown that 186Re and 188Re could be produced simultaneously with suitable and almost equal activities with irradiating natural rhenium for 100–120 h and considering 24 h for cooling. Also, the levels of impurities in the simultaneous manufacture of 186Re and 188Re using the neutron irradiation of natural rhenium are negligible in comparison to the primary products, and the primary products' activities are sufficient to make compositional radiopharmaceuticals.
{"title":"Theoretical and experimental validation of dual rhenium radioisotope production for enhanced targeted cancer therapy","authors":"Ranjbar Hassan , Bagheri Reza , Janjani Iman","doi":"10.1016/j.nucana.2025.100202","DOIUrl":"10.1016/j.nucana.2025.100202","url":null,"abstract":"<div><h3>Objective</h3><div>For many years, different ligands have been combined with rhenium therapeutic radioisotopes, specifically rhenium-186 and 188, to create radiopharmaceuticals for the treatment of various illnesses. Because of the unique qualities that set each of these radioisotopes apart, they can all be used to eradicate different kinds of cancers. Large cancers can be effectively removed in 188Re thanks to the use of great-energy, long-distance beta particles. However, <sup>186</sup>Re's short range, low energy beta particles are a sufficient weapon to destroy tiny tumors with a high yield and little side effects. As a result, the properties of each of these radioisotopes can only partially address the therapy on their own. Therefore, we reasoned that <sup>188</sup>Re and <sup>186</sup>Re in conjunction must provide the greatest results when treating tumors of different sizes. One possible outcome of neutron-irradiation of natural rhenium is the simultaneous production of <sup>186</sup>Re and <sup>188</sup>Re.</div></div><div><h3>Methods</h3><div>We want to know if the natural irradiation of rhenium, together with the simultaneous synthesis of these radioisotopes, provides us with the right amounts of radioactivity to make compositional radiopharmaceuticals. This study examines the kind and quantity of impurities created, as well as the practical and theoretical evaluations of the simultaneous generation of <sup>188</sup>Re and <sup>186</sup>R to achieve compositional radiopharmaceuticals by neutron irradiation of natural rhenium in 5MWt pool-type light water research reactor.</div></div><div><h3>Results</h3><div>The outcomes demonstrated that the theoretical computations and experimental data correlate well. The data's greatest relative error has been determined to be 8 %.</div></div><div><h3>Conclusion</h3><div>The findings shown that <sup>186</sup>Re and <sup>188</sup>Re could be produced simultaneously with suitable and almost equal activities with irradiating natural rhenium for 100–120 h and considering 24 h for cooling. Also, the levels of impurities in the simultaneous manufacture of <sup>186</sup>Re and <sup>188</sup>Re using the neutron irradiation of natural rhenium are negligible in comparison to the primary products, and the primary products' activities are sufficient to make compositional radiopharmaceuticals.</div></div>","PeriodicalId":100965,"journal":{"name":"Nuclear Analysis","volume":"4 4","pages":"Article 100202"},"PeriodicalIF":0.0,"publicationDate":"2025-12-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145617979","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2025-11-26DOI: 10.1016/j.nucana.2025.100204
Farhad Zolfagharpour, Zeinab Tayyari-Sadegh
In this work, the two assemblies named 16B36 and 36B20, and two arrangements named B and C, were introduced. The current arrangement of assemblies (named arrangement A) in the core of the BNPP reactor, was changed and the new assemblies were replaced, while the main characteristics of the core were maintained unchanged. The new arrangements and new assemblies were simulated in the MCNPX.2.6.0 code. For each arrangement, some parameters were calculated like: the effective multiplication factor, power peaking factor (PPF), energy deposition, average linear power density, maximum linear heat rate in hot rod, and the burnup after 300 operation days. According to the obtained results, arrangement C was suggested for use in BNPP at the first cycle of reactor operation, because in arrangement C, the burnup increases to about 3.3 GWd/MTU, the linear power density increases about 29 %, and the radial power distribution becomes significantly flattened, while the safety margin, including the maximum heat rate in hot rod, is maintained. The maximum heat rate in the hot rod was 35.95 kw/m which is below the allowed value (44.8 kw/m) reported in FSAR.
{"title":"New arrangements of FAs at BNPP's reactor: PPF and burnup calculations","authors":"Farhad Zolfagharpour, Zeinab Tayyari-Sadegh","doi":"10.1016/j.nucana.2025.100204","DOIUrl":"10.1016/j.nucana.2025.100204","url":null,"abstract":"<div><div>In this work, the two assemblies named 16B36 and 36B20, and two arrangements named B and C, were introduced. The current arrangement of assemblies (named arrangement A) in the core of the BNPP reactor, was changed and the new assemblies were replaced, while the main characteristics of the core were maintained unchanged. The new arrangements and new assemblies were simulated in the MCNPX.2.6.0 code. For each arrangement, some parameters were calculated like: the effective multiplication factor, power peaking factor (PPF), energy deposition, average linear power density, maximum linear heat rate in hot rod, and the burnup after 300 operation days. According to the obtained results, arrangement C was suggested for use in BNPP at the first cycle of reactor operation, because in arrangement C, the burnup increases to about 3.3 GWd/MTU, the linear power density increases about 29 %, and the radial power distribution becomes significantly flattened, while the safety margin, including the maximum heat rate in hot rod, is maintained. The maximum heat rate in the hot rod was 35.95 kw/m which is below the allowed value (44.8 kw/m) reported in FSAR.</div></div>","PeriodicalId":100965,"journal":{"name":"Nuclear Analysis","volume":"5 1","pages":"Article 100204"},"PeriodicalIF":0.0,"publicationDate":"2025-11-26","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145738019","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2025-11-24DOI: 10.1016/j.nucana.2025.100203
Ali K. Al-Muttairi , Norlaili A. Kabir
Lead (Pb) is widely used for radiation shielding due to its high atomic number, density, affordability, and availability. However, its toxicity poses serious environmental and health risks. This study aims to evaluate the gamma-ray shielding performance of polyvinyl alcohol (PVA)-based shielding composites in the attenuation of 60Co, 137Cs, and 241Am sources. A PVA-based shielding material incorporating Pb, Bi2O3, and Sn were evaluated for its radiation attenuation properties, using Pb as the benchmark standard for comparison of shielding effectiveness. PVA was selected for its hydrophilicity, ease of mixing, and light-weight property. A total of 18 shielding samples were fabricated, with six samples for each metal. The variables include metal percentages of 10 %, 20 %, and 30 %, as well as thicknesses of 0.6, 0.8, and 1.0 cm. Pb composites showed the highest attenuation among all samples, while Bi2O3 and Sn composites also demonstrated strong shielding performance. The results showed that increasing the metal percentage per unit thickness has a much greater effect on shielding performance than simply increasing thickness. Increasing metal percentage at constant thickness significantly increases both linear and mass attenuation coefficients for all samples while reducing their HVL. At a constant thickness of 0.8 cm, increasing the metal composition from 10 % to 30 % results in a rise in the linear attenuation coefficient. For PVA/Pb, it increases from 1.75 cm−1 to 2.7 cm−1, for PVA/Bi2O3, from 1.8 cm−1 to 1.9 cm−1, and for PVA/Sn, from 1.3 cm−1 to 1.5 cm−1. In summary, optimal shielding efficiency is primarily determined by the metal percentage per unit thickness, as photon attenuation depends more on the concentration of heavy atoms along the radiation path than on overall shielding thickness.
{"title":"Polyvinyl alcohol composites (PVA) with added Pb, Bi, and Sn: A study on radiation shielding and gamma ray attenuation","authors":"Ali K. Al-Muttairi , Norlaili A. Kabir","doi":"10.1016/j.nucana.2025.100203","DOIUrl":"10.1016/j.nucana.2025.100203","url":null,"abstract":"<div><div>Lead (Pb) is widely used for radiation shielding due to its high atomic number, density, affordability, and availability. However, its toxicity poses serious environmental and health risks. This study aims to evaluate the gamma-ray shielding performance of polyvinyl alcohol (PVA)-based shielding composites in the attenuation of <sup>60</sup>Co, <sup>137</sup>Cs, and <sup>241</sup>Am sources. A PVA-based shielding material incorporating Pb, Bi<sub>2</sub>O<sub>3</sub>, and Sn were evaluated for its radiation attenuation properties, using Pb as the benchmark standard for comparison of shielding effectiveness. PVA was selected for its hydrophilicity, ease of mixing, and light-weight property. A total of 18 shielding samples were fabricated, with six samples for each metal. The variables include metal percentages of 10 %, 20 %, and 30 %, as well as thicknesses of 0.6, 0.8, and 1.0 cm. Pb composites showed the highest attenuation among all samples, while Bi<sub>2</sub>O<sub>3</sub> and Sn composites also demonstrated strong shielding performance. The results showed that increasing the metal percentage per unit thickness has a much greater effect on shielding performance than simply increasing thickness. Increasing metal percentage at constant thickness significantly increases both linear and mass attenuation coefficients for all samples while reducing their HVL. At a constant thickness of 0.8 cm, increasing the metal composition from 10 % to 30 % results in a rise in the linear attenuation coefficient. For PVA/Pb, it increases from 1.75 cm<sup>−1</sup> to 2.7 cm<sup>−1</sup>, for PVA/Bi<sub>2</sub>O<sub>3</sub>, from 1.8 cm<sup>−1</sup> to 1.9 cm<sup>−1</sup>, and for PVA/Sn, from 1.3 cm<sup>−1</sup> to 1.5 cm<sup>−1</sup>. In summary, optimal shielding efficiency is primarily determined by the metal percentage per unit thickness, as photon attenuation depends more on the concentration of heavy atoms along the radiation path than on overall shielding thickness.</div></div>","PeriodicalId":100965,"journal":{"name":"Nuclear Analysis","volume":"5 1","pages":"Article 100203"},"PeriodicalIF":0.0,"publicationDate":"2025-11-24","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145685080","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Fertilizers contain several radioactive elements of the decay series of 238U, 226Ra and 232Th and they can be a source of human exposure to gamma radiation when crops grown with fertilizers are consumed by human. The activity concentrations of 238U, 232Th and 40K in three brands of fertilizers were measured using gamma-ray spectrometry and the radiological indices [Radium Equivalent activity (Raeq), Absorbed Dose rate (DR), Annual Effective Dose rate (AED), External hazard (Hex), and Internal hazard (Hin)] were estimated. The average activity concentrations of 238U, 232Th and 40K were 4.98 ± 1.71, 12.35 ± 2.45 and 11.89.05 ± 288.91 Bqkg−1; 7.50 ± 1.84, 16.60 ± 3.32 and 2080.72 ± 251.25 Bqkg−1 and 2.46 ± 0.68, 5.96 ± 1.24 and 306.82 ± 70.46 Bqkg−1 for NPK 15-15-15, NPK 15-15-17 and Urea, respectively. The values of radiological indices were lower than the permissible limits stipulated by world average values except Raeq and absorbed dose rate. Therefore, it can be concluded that no significant radiological health risk occurs. However, the presence of radionuclides in the fertilizers could be an exposure pathway that gamma radiation enters the food chain and threaten food production with deleterious health implications on the consumers of the such crops.
{"title":"Activity levels and radiological hazards of chemical fertilizers used for farm crops in Ondo city, Southwest, Nigeria","authors":"Lasun Tunde Ogundele , Muyiwa Micheal Orosun , Similoluwa Akiniran , Patrick Oluwagbemiga Ayeku","doi":"10.1016/j.nucana.2025.100201","DOIUrl":"10.1016/j.nucana.2025.100201","url":null,"abstract":"<div><div>Fertilizers contain several radioactive elements of the decay series of <sup>238</sup>U, <sup>226</sup>Ra and <sup>232</sup>Th and they can be a source of human exposure to gamma radiation when crops grown with fertilizers are consumed by human. The activity concentrations of <sup>238</sup>U, <sup>232</sup>Th and <sup>40</sup>K in three brands of fertilizers were measured using gamma-ray spectrometry and the radiological indices [Radium Equivalent activity (Ra<sub>eq</sub>), Absorbed Dose rate (DR), Annual Effective Dose rate (AED), External hazard (H<sub>ex</sub>), and Internal hazard (H<sub>in</sub>)] were estimated. The average activity concentrations of <sup>238</sup>U, <sup>232</sup>Th and <sup>40</sup>K were 4.98 ± 1.71, 12.35 ± 2.45 and 11.89.05 ± 288.91 Bqkg<sup>−1</sup>; 7.50 ± 1.84, 16.60 ± 3.32 and 2080.72 ± 251.25 Bqkg<sup>−1</sup> and 2.46 ± 0.68, 5.96 ± 1.24 and 306.82 ± 70.46 Bqkg<sup>−1</sup> for NPK 15-15-15, NPK 15-15-17 and Urea, respectively. The values of radiological indices were lower than the permissible limits stipulated by world average values except Ra<sub>eq</sub> and absorbed dose rate. Therefore, it can be concluded that no significant radiological health risk occurs. However, the presence of radionuclides in the fertilizers could be an exposure pathway that gamma radiation enters the food chain and threaten food production with deleterious health implications on the consumers of the such crops.</div></div>","PeriodicalId":100965,"journal":{"name":"Nuclear Analysis","volume":"5 1","pages":"Article 100201"},"PeriodicalIF":0.0,"publicationDate":"2025-10-26","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145618351","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2025-10-15DOI: 10.1016/j.nucana.2025.100185
Zeenat Ullah , Abdelhamid Jalil , Xianpeng Yin , Yingming Sang , Javed Hussain , Muhammad Shoaib , Ghulam Hussan , Da Chen
Accurate calibration of NaI(Tl) scintillation detectors is essential for reliable gamma-ray spectrometry in nuclear safeguards and environmental radiation monitoring. This study investigates the full energy peak efficiency (FEPE) of a NaI(Tl) detector using experimental measurements and Monte Carlo simulation performed with FLUKA and MCNP. Standard point sources (, , and ) were measured at four source-detector distances (4, 8, 12, and 16 cm) covering photon energies from 356 to 1333 keV. Both simulation tools demonstrated an average deviation of less than 6 % and a maximum deviation of 18 % from the experimental results in all configurations. Furthermore, source misalignment was numerically evaluated and found to have a measurable impact only at short source-detector distance. This work represents the first integrated benchmarking of FLUKA and MCNP against experimental FEPE data across multiple geometries, offering a validated framework for accurate detector modeling and calibration.
{"title":"Benchmarking of the efficiency of the NaI(Tl) detector using FLUKA, MCNP, and experimental measurements at multiple source distances","authors":"Zeenat Ullah , Abdelhamid Jalil , Xianpeng Yin , Yingming Sang , Javed Hussain , Muhammad Shoaib , Ghulam Hussan , Da Chen","doi":"10.1016/j.nucana.2025.100185","DOIUrl":"10.1016/j.nucana.2025.100185","url":null,"abstract":"<div><div>Accurate calibration of NaI(Tl) scintillation detectors is essential for reliable gamma-ray spectrometry in nuclear safeguards and environmental radiation monitoring. This study investigates the full energy peak efficiency (FEPE) of a <span><math><msup><mn>2</mn><mrow><mi>′</mi><mi>′</mi></mrow></msup><mspace></mspace><mo>×</mo><mspace></mspace><msup><mn>2</mn><mrow><mi>′</mi><mi>′</mi></mrow></msup></math></span> NaI(Tl) detector using experimental measurements and Monte Carlo simulation performed with FLUKA and MCNP. Standard point sources (<span><math><mrow><msup><mrow></mrow><mrow><mn>133</mn></mrow></msup><mtext>Ba</mtext></mrow></math></span>, <span><math><mrow><msup><mrow></mrow><mrow><mn>137</mn></mrow></msup><mtext>Cs</mtext></mrow></math></span>, and <span><math><mrow><msup><mrow></mrow><mrow><mn>60</mn></mrow></msup><mtext>Co</mtext></mrow></math></span>) were measured at four source-detector distances (4, 8, 12, and 16 cm) covering photon energies from 356 to 1333 keV. Both simulation tools demonstrated an average deviation of less than 6 % and a maximum deviation of 18 % from the experimental results in all configurations. Furthermore, source misalignment was numerically evaluated and found to have a measurable impact only at short source-detector distance. This work represents the first integrated benchmarking of FLUKA and MCNP against experimental FEPE data across multiple geometries, offering a validated framework for accurate detector modeling and calibration.</div></div>","PeriodicalId":100965,"journal":{"name":"Nuclear Analysis","volume":"4 4","pages":"Article 100185"},"PeriodicalIF":0.0,"publicationDate":"2025-10-15","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145418218","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2025-10-14DOI: 10.1016/j.nucana.2025.100200
Khalid Nabaoui , Abdessamad Didi , El Mehdi Alibrahmi , Otmane Allaoui , Jamila Yousfi , El Mahjoub Chakir
This study focuses on the use of polyethylene as the primary material for the fabrication of an irradiation shuttle intended for the TRIGA Mark II reactor. Designed to accommodate multiple sample capsules, the shuttle is subjected to prolonged neutron irradiation under real operating conditions. The objective is to analyze the interactions between thermal neutrons and polymeric materials in order to better understand their structural and radiological behavior under irradiation. The dose distribution was numerically modeled using the PHITS code, enabling precise identification of the regions of maximum intensity within the shuttle. The results provide a basis for optimizing the materials employed in nuclear environments, integrating radiological safety requirements with durability and mechanical performance.
本研究的重点是使用聚乙烯作为制造用于TRIGA Mark II反应堆的辐照梭的主要材料。设计用于容纳多个样品胶囊,航天飞机在实际操作条件下受到长时间的中子辐照。目的是分析热中子与高分子材料之间的相互作用,以便更好地了解它们在辐照下的结构和放射行为。使用PHITS代码对剂量分布进行了数值模拟,从而能够精确识别航天飞机内最大强度的区域。研究结果为优化核环境中使用的材料提供了基础,将放射性安全要求与耐久性和机械性能相结合。
{"title":"Monte Carlo simulation of dose and residual activation in a polyethylene shuttle of the TRIGA Mark II reactor","authors":"Khalid Nabaoui , Abdessamad Didi , El Mehdi Alibrahmi , Otmane Allaoui , Jamila Yousfi , El Mahjoub Chakir","doi":"10.1016/j.nucana.2025.100200","DOIUrl":"10.1016/j.nucana.2025.100200","url":null,"abstract":"<div><div>This study focuses on the use of polyethylene as the primary material for the fabrication of an irradiation shuttle intended for the TRIGA Mark II reactor. Designed to accommodate multiple sample capsules, the shuttle is subjected to prolonged neutron irradiation under real operating conditions. The objective is to analyze the interactions between thermal neutrons and polymeric materials in order to better understand their structural and radiological behavior under irradiation. The dose distribution was numerically modeled using the PHITS code, enabling precise identification of the regions of maximum intensity within the shuttle. The results provide a basis for optimizing the materials employed in nuclear environments, integrating radiological safety requirements with durability and mechanical performance.</div></div>","PeriodicalId":100965,"journal":{"name":"Nuclear Analysis","volume":"4 4","pages":"Article 100200"},"PeriodicalIF":0.0,"publicationDate":"2025-10-14","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145418219","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2025-10-14DOI: 10.1016/j.nucana.2025.100199
V. Muthukumar , D. Elil Raja , P. Jayaprakash , A. Suresh Babu
This research focuses on the mechanical and thermal characterization of nano-sisal fiber-reinforced polymer composites, exploring the potential of incorporating nanomaterials to enhance the performance of traditional sisal fiber composites. Natural sisal fibers (NSF) serve as the starting point for the chemical and physical processes that produce sisal fibers. Several analytical techniques are used to describe the materials, such as Fourier transform infrared spectroscopy (FTIR), scanning electron microscopy (SEM), high-resolution transmission electron microscopy (HR-TEM), and field emission scanning electron microscopy (FE-SEM). This study investigates the synergistic effects of integrating nanoscale reinforcements into sisal fiber-reinforced polymer matrices. Mechanical properties, including tensile strength, flexural strength, and impact resistance, are systematically evaluated using standardized testing procedures. Fabricating epoxy polymer-based composites involves adding silver fibers in various weight percentages (1, 2, 3, 4, 5, 6, 7, and 8 %). The results highlight the influence of nanoscale additives on the overall mechanical performance and thermal stability of the composite materials. Furthermore, the study investigates the potential for improved load-bearing capacity, durability, flexural strength, tensile strength, impact resistance, thermal analysis, and heat resistance in sisal fiber composite samples, where these composites could exhibit utility. The findings of this research contribute to the understanding of nano-sisal fiber-reinforced polymer composites and their viability in various engineering applications.
{"title":"Nano-sisal fiber reinforced polymer composites for biocompatible lightweight structural applications","authors":"V. Muthukumar , D. Elil Raja , P. Jayaprakash , A. Suresh Babu","doi":"10.1016/j.nucana.2025.100199","DOIUrl":"10.1016/j.nucana.2025.100199","url":null,"abstract":"<div><div>This research focuses on the mechanical and thermal characterization of nano-sisal fiber-reinforced polymer composites, exploring the potential of incorporating nanomaterials to enhance the performance of traditional sisal fiber composites. Natural sisal fibers (NSF) serve as the starting point for the chemical and physical processes that produce sisal fibers. Several analytical techniques are used to describe the materials, such as Fourier transform infrared spectroscopy (FTIR), scanning electron microscopy (SEM), high-resolution transmission electron microscopy (HR-TEM), and field emission scanning electron microscopy (FE-SEM). This study investigates the synergistic effects of integrating nanoscale reinforcements into sisal fiber-reinforced polymer matrices. Mechanical properties, including tensile strength, flexural strength, and impact resistance, are systematically evaluated using standardized testing procedures. Fabricating epoxy polymer-based composites involves adding silver fibers in various weight percentages (1, 2, 3, 4, 5, 6, 7, and 8 %). The results highlight the influence of nanoscale additives on the overall mechanical performance and thermal stability of the composite materials. Furthermore, the study investigates the potential for improved load-bearing capacity, durability, flexural strength, tensile strength, impact resistance, thermal analysis, and heat resistance in sisal fiber composite samples, where these composites could exhibit utility. The findings of this research contribute to the understanding of nano-sisal fiber-reinforced polymer composites and their viability in various engineering applications.</div></div>","PeriodicalId":100965,"journal":{"name":"Nuclear Analysis","volume":"4 4","pages":"Article 100199"},"PeriodicalIF":0.0,"publicationDate":"2025-10-14","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145363235","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}