首页 > 最新文献

Nuclear Analysis最新文献

英文 中文
A comparative analysis of the NaI detector response function using GAMOS and FLUKA Monte Carlo simulations 利用 GAMOS 和 FLUKA 蒙特卡罗模拟对碘化钠探测器响应函数进行比较分析
Pub Date : 2024-09-23 DOI: 10.1016/j.nucana.2024.100138
This work aims to study the response function of a 2″×2″ NaI(Tl) scintillation detector using Monte Carlo simulations. A precise mathematical model of the NaI(Tl) scintillator was developed using both FLUKA and GAMOS Monte Carlo simulation software. The photon pulse height distributions of the NaI(Tl) without influence of its energy resolution, obtained with FLUKA and GAMOS codes, were converted into a real NaI(Tl) response function using the necessary conversion process. Spectral characteristics such as full-energy peak efficiency, energy resolution, peak-to-Compton ratio, and peak-to-total ratio were investigated by simulation at different gamma-ray energy obtained from 109Cd, 137Cs, 54Mn, 65Zn, and 60Co sources. The simulated spectra from the GAMOS code were consistent with those generated by the FLUKA code. Additionally, the comparison between simulated results and experimental data demonstrated good agreement. The validation of the computational models used for the NaI(Tl) detector in both FLUKA and GAMOS software was successfully achieved, confirming the accuracy of the simulations in replicating the detector's response.
这项工作旨在利用蒙特卡罗模拟研究 2″×2″ NaI(Tl)闪烁探测器的响应函数。利用 FLUKA 和 GAMOS 蒙特卡罗模拟软件建立了 NaI(Tl)闪烁体的精确数学模型。利用 FLUKA 和 GAMOS 代码获得的不受能量分辨率影响的 NaI(Tl)光子脉冲高度分布,通过必要的转换过程转换为真实的 NaI(Tl)响应函数。通过模拟从 109Cd、137Cs、54Mn、65Zn 和 60Co 源获得的不同伽马射线能量,研究了全能峰值效率、能量分辨率、峰值与康普顿比和峰值与总比等光谱特性。GAMOS 代码模拟的光谱与 FLUKA 代码生成的光谱一致。此外,模拟结果与实验数据的比较也显示出良好的一致性。在 FLUKA 和 GAMOS 软件中对 NaI(Tl)探测器所用计算模型的验证已成功实现,证实了模拟在复制探测器响应方面的准确性。
{"title":"A comparative analysis of the NaI detector response function using GAMOS and FLUKA Monte Carlo simulations","authors":"","doi":"10.1016/j.nucana.2024.100138","DOIUrl":"10.1016/j.nucana.2024.100138","url":null,"abstract":"<div><div>This work aims to study the response function of a 2″×2″ NaI(Tl) scintillation detector using Monte Carlo simulations. A precise mathematical model of the NaI(Tl) scintillator was developed using both FLUKA and GAMOS Monte Carlo simulation software. The photon pulse height distributions of the NaI(Tl) without influence of its energy resolution, obtained with FLUKA and GAMOS codes, were converted into a real NaI(Tl) response function using the necessary conversion process. Spectral characteristics such as full-energy peak efficiency, energy resolution, peak-to-Compton ratio, and peak-to-total ratio were investigated by simulation at different gamma-ray energy obtained from <sup>109</sup>Cd, <sup>137</sup>Cs, <sup>54</sup>Mn, <sup>65</sup>Zn, and <sup>60</sup>Co sources. The simulated spectra from the GAMOS code were consistent with those generated by the FLUKA code. Additionally, the comparison between simulated results and experimental data demonstrated good agreement. The validation of the computational models used for the NaI(Tl) detector in both FLUKA and GAMOS software was successfully achieved, confirming the accuracy of the simulations in replicating the detector's response.</div></div>","PeriodicalId":100965,"journal":{"name":"Nuclear Analysis","volume":null,"pages":null},"PeriodicalIF":0.0,"publicationDate":"2024-09-23","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142323148","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Coulomb interaction dependence of optimal energy to synthesize superheavy elements 合成超重元素的最佳能量与库仑相互作用的关系
Pub Date : 2024-09-21 DOI: 10.1016/j.nucana.2024.100137
The production of superheavy elements beyond Z = 118 remains unattained through both cold and hot fusion techniques, primarily due to inadequate fusion reaction optimization involving projectile–target combinations and energy. Past efforts employed various theories to optimize these combinations. In our current study, we have successfully identified optimal fusion energies for synthesizing superheavy elements, employing an advance statistical model and dinuclear system models. The establishment of optimal energy governing rule is achieved through a comprehensive examination of the Coulomb interaction parameter, enabling precise determination of the optimal energy for successful fusion reactions in synthesizing superheavy elements. The confidence level of predicting optimal energies using the present formula varies between 97% to 99%. The predicted optimal energy using the present formula for five fusion reactions such as 208Pb(50Ti,1n)257Rf, 208Pb(50Ti,2n)256Rf, 209Bi(50Ti,1n)258Db, 208Pb(58Fe,1n)265Hs, and 244Pu(48Ca,4n)288Fl were studied and are in good agreement with each other. Furthermore, we predicted the Optimal energies for fusion reactions leading to synthesize the superheavy element Z = 119 and 120. The presented empirical rule will certainly bring a revolution in the synthesis of superheavy elements.
通过冷核聚变和热核聚变技术仍无法生产 Z = 118 以上的超重元素,这主要是由于涉及射弹-目标组合和能量的核聚变反应优化不足。过去的工作采用了各种理论来优化这些组合。在目前的研究中,我们利用先进的统计模型和双核系统模型,成功地确定了合成超重元素的最佳聚变能量。通过对库仑相互作用参数的全面研究,建立了最佳能量调控规则,从而精确确定了成功合成超重元素的最佳聚变反应能量。使用本公式预测最佳能量的置信度在 97% 到 99% 之间。我们对 208Pb(50Ti,1n)257Rf、208Pb(50Ti,2n)256Rf、209Bi(50Ti,1n)258Db、208Pb(58Fe,1n)265Hs 和 244Pu(48Ca,4n)288Fl 等五个聚变反应使用本公式预测的最佳能量进行了研究,结果相互吻合。此外,我们还预测了导致合成超重元素 Z = 119 和 120 的核聚变反应的最佳能量。所提出的经验法则必将为超重元素的合成带来一场革命。
{"title":"Coulomb interaction dependence of optimal energy to synthesize superheavy elements","authors":"","doi":"10.1016/j.nucana.2024.100137","DOIUrl":"10.1016/j.nucana.2024.100137","url":null,"abstract":"<div><div>The production of superheavy elements beyond Z <span><math><mo>=</mo></math></span> 118 remains unattained through both cold and hot fusion techniques, primarily due to inadequate fusion reaction optimization involving projectile–target combinations and energy. Past efforts employed various theories to optimize these combinations. In our current study, we have successfully identified optimal fusion energies for synthesizing superheavy elements, employing an advance statistical model and dinuclear system models. The establishment of optimal energy governing rule is achieved through a comprehensive examination of the Coulomb interaction parameter, enabling precise determination of the optimal energy for successful fusion reactions in synthesizing superheavy elements. The confidence level of predicting optimal energies using the present formula varies between 97% to 99%. The predicted optimal energy using the present formula for five fusion reactions such as <sup>208</sup>Pb(<sup>50</sup>Ti,1n)<sup>257</sup>Rf, <sup>208</sup>Pb(<sup>50</sup>Ti,2n)<sup>256</sup>Rf, <sup>209</sup>Bi(<sup>50</sup>Ti,1n)<sup>258</sup>Db, <sup>208</sup>Pb(<sup>58</sup>Fe,1n)<sup>265</sup>Hs, and <sup>244</sup>Pu(<sup>48</sup>Ca,4n)<sup>288</sup>Fl were studied and are in good agreement with each other. Furthermore, we predicted the Optimal energies for fusion reactions leading to synthesize the superheavy element Z <span><math><mo>=</mo></math></span> 119 and 120. The presented empirical rule will certainly bring a revolution in the synthesis of superheavy elements.</div></div>","PeriodicalId":100965,"journal":{"name":"Nuclear Analysis","volume":null,"pages":null},"PeriodicalIF":0.0,"publicationDate":"2024-09-21","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142328252","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Major and trace elements determination in organic and conventional Moroccan vegetables using the k0-standardisation method of neutron activation analysis 利用中子活化分析 k0 标准化方法测定摩洛哥有机蔬菜和常规蔬菜中的主要元素和微量元素
Pub Date : 2024-08-16 DOI: 10.1016/j.nucana.2024.100127

The aim of the present work is the determination of different essential (minor and trace) elements found in five Moroccan vegetables collected from large commercial markets in Kenitra city, Morocco, and in some organic vegetables which were traditionally grown without the use of pesticides or chemical fertilizers, in a plot located in the rural commune of Dar Laaslouji, 48 km from Kenitra city. The k0-standardisation method of the Neutron Activation Analysis (k0-INAA) using the TRIGA Mark II research reactor of 2 MW at the National Centre for Nuclear Energy, Science and Technology (CNESTEN) and gamma-ray spectroscopy facility were employed. For quality control, the accuracy of measurements has been investigated using certified reference materials (IAEA-336 lichens, and NIST SRM 1547 peach leaves) which were analyzed simultaneously with the samples. Good agreement was found between certified and determined values. The primary results are presented and discussed for the concentration of minor and trace elements in some vegetables (tomatoes, carrots, green peppers, cilantro and mint), that are widely used in Moroccan meals.

本研究的目的是测定从摩洛哥凯尼特拉市大型商业市场上采集的五种摩洛哥蔬菜中的不同基本(次要和微量)元素,以及在距离凯尼特拉市 48 公里的 Dar Laaslouji 乡的一块地里发现的一些传统种植的不使用杀虫剂或化肥的有机蔬菜中的不同基本(次要和微量)元素。使用国家核能、科学和技术中心(CNESTEN)的 2 兆瓦 TRIGA Mark II 研究反应堆和伽马射线光谱设备,采用了中子活化分析 k0 标准化方法(k0-IAA)。在质量控制方面,使用与样品同时分析的认证参考材料(IAEA-336 地衣和 NIST SRM 1547 桃叶)对测量的准确性进行了研究。发现认证值和测定值之间的一致性很好。本报告介绍并讨论了摩洛哥膳食中广泛使用的一些蔬菜(西红柿、胡萝卜、青椒、香菜和薄荷)中微量元素的主要结果。
{"title":"Major and trace elements determination in organic and conventional Moroccan vegetables using the k0-standardisation method of neutron activation analysis","authors":"","doi":"10.1016/j.nucana.2024.100127","DOIUrl":"10.1016/j.nucana.2024.100127","url":null,"abstract":"<div><p>The aim of the present work is the determination of different essential (minor and trace) elements found in five Moroccan vegetables collected from large commercial markets in Kenitra city, Morocco, and in some organic vegetables which were traditionally grown without the use of pesticides or chemical fertilizers, in a plot located in the rural commune of Dar Laaslouji, 48 km from Kenitra city. The k0-standardisation method of the Neutron Activation Analysis (k0-INAA) using the TRIGA Mark II research reactor of 2 MW at the National Centre for Nuclear Energy, Science and Technology (CNESTEN) and gamma-ray spectroscopy facility were employed. For quality control, the accuracy of measurements has been investigated using certified reference materials (IAEA-336 lichens, and NIST SRM 1547 peach leaves) which were analyzed simultaneously with the samples. Good agreement was found between certified and determined values. The primary results are presented and discussed for the concentration of minor and trace elements in some vegetables (tomatoes, carrots, green peppers, cilantro and mint), that are widely used in Moroccan meals.</p></div>","PeriodicalId":100965,"journal":{"name":"Nuclear Analysis","volume":null,"pages":null},"PeriodicalIF":0.0,"publicationDate":"2024-08-16","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.sciencedirect.com/science/article/pii/S2773183924000272/pdfft?md5=b1d34d7429818ab97b003d1bac920b82&pid=1-s2.0-S2773183924000272-main.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142058495","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Structural insights into soft matter materials via spin echo small angle neutron scattering and small angle neutron scattering 通过自旋回波小角中子散射和小角中子散射洞察软物质材料的结构
Pub Date : 2024-08-16 DOI: 10.1016/j.nucana.2024.100128

The recent advancements in neutron scattering technologies in China, with the development of China's first Spin-Echo Small-Angle Neutron Scattering (SESANS) spectrometer at China Mianyang Research Reactor (CMRR) and the integration of a Very Small Angle Neutron Scattering (VSANS) instrument at China Spallation Neutron Source (CSNS), have significantly bolstered the nation's scientific capabilities. This review aims to highlight the distinctive features and applications of SESANS and SANS, and to offer a valuable contribution by demonstrating how SESANS and SANS can be leveraged for the study of soft matters and solid-state materials, with a particular emphasis on the benefits of techniques such as chain labeling, contrast variation, and contrast matching. We also aim to illustrate what types of information can be gleaned from these methods. The review is structured to first introduce the general concepts of SANS and SESANS, followed by a discussion on the information these techniques can provide. Then the applications of these techniques, in combination with other techniques, on various material investigations will be demonstrated. The review concludes with a summary and future perspectives, aiming to inspire further interdisciplinary research and collaboration, and beneficial to a broader audience.

随着中国绵阳中子研究堆(CMRR)研制出中国第一台自旋回波小角中子散射(SESANS)光谱仪,以及中国溅射中子源(CSNS)集成了甚小角中子散射(VSANS)仪器,中国中子散射技术的最新进展极大地增强了国家的科学能力。本综述旨在强调 SESANS 和 SANS 的独特功能和应用,并通过展示如何利用 SESANS 和 SANS 研究软物质和固态材料,特别强调链标记、对比度变化和对比度匹配等技术的益处,从而做出有价值的贡献。我们还旨在说明从这些方法中可以收集到哪些类型的信息。综述的结构是首先介绍 SANS 和 SESANS 的一般概念,然后讨论这些技术可以提供的信息。然后将展示这些技术与其他技术相结合在各种材料研究中的应用。综述的最后是总结和未来展望,旨在激励进一步的跨学科研究与合作,并使更多读者受益。
{"title":"Structural insights into soft matter materials via spin echo small angle neutron scattering and small angle neutron scattering","authors":"","doi":"10.1016/j.nucana.2024.100128","DOIUrl":"10.1016/j.nucana.2024.100128","url":null,"abstract":"<div><p>The recent advancements in neutron scattering technologies in China, with the development of China's first Spin-Echo Small-Angle Neutron Scattering (SESANS) spectrometer at China Mianyang Research Reactor (CMRR) and the integration of a Very Small Angle Neutron Scattering (VSANS) instrument at China Spallation Neutron Source (CSNS), have significantly bolstered the nation's scientific capabilities. This review aims to highlight the distinctive features and applications of SESANS and SANS, and to offer a valuable contribution by demonstrating how SESANS and SANS can be leveraged for the study of soft matters and solid-state materials, with a particular emphasis on the benefits of techniques such as chain labeling, contrast variation, and contrast matching. We also aim to illustrate what types of information can be gleaned from these methods. The review is structured to first introduce the general concepts of SANS and SESANS, followed by a discussion on the information these techniques can provide. Then the applications of these techniques, in combination with other techniques, on various material investigations will be demonstrated. The review concludes with a summary and future perspectives, aiming to inspire further interdisciplinary research and collaboration, and beneficial to a broader audience.</p></div>","PeriodicalId":100965,"journal":{"name":"Nuclear Analysis","volume":null,"pages":null},"PeriodicalIF":0.0,"publicationDate":"2024-08-16","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.sciencedirect.com/science/article/pii/S2773183924000284/pdfft?md5=35c8e99ee7a1b6e9645a922724fdd3ac&pid=1-s2.0-S2773183924000284-main.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142040717","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Gold nanoparticle effect on dose and DNA damage enhancement in the vicinity of gold nanoparticles 金纳米粒子对剂量和金纳米粒子附近 DNA 损伤增强的影响
Pub Date : 2024-08-13 DOI: 10.1016/j.nucana.2024.100126

This study uses Monte Carlo simulations to examine the dose enhancement effect of gold nanoparticles (AuNPs) in radiation therapy and its effects on DNA damage. Using the GATE- 9.0 and Geant4-DNA packages, Monte Carlo simulations were used to simulate a mathematical phantom and determine the energy deposition in the vicinity of AuNP. The simulations were conducted for various photon beam energies (50, 100, 250, and 6000 keV) with and without the presence of different-size AuNPs (10, 30, 50 and 100 nm). The dose enhancement factor (DER) was evaluated using Geant4-DNA to examine the effects AuNP sizes and photon beam energies on DNA damage. A multi-scale Monte Carlo simulation was conducted to evaluate enhanced DNA damage owing to nanoparticles in the proximity of cancer cells. The Monte Carlo simulations indicated that AuNPs boost the dose delivery, resulting in enhanced energy deposition and subsequent DNA damage. The DER analysis revealed a significant increase in the dose deposition within DNA, leading to single or double-strand breaks. Geant4-DNA simulations revealed information on the dosage enhancement factor for various AuNP sizes and photon beam intensities, enabling a deeper comprehension of the underlying mechanics. The outcomes of this study emphasize the potential of AuNPs as effective radiosensitizers in radiation therapy and contribute to the growing body of research on the use of nanotechnology in enhancing cancer treatment outcomes. Further investigations and experimental validations are necessary to optimize the usage of AuNPs for improved radiation therapy.

本研究利用蒙特卡罗模拟来研究金纳米粒子(AuNPs)在放射治疗中的剂量增强效应及其对 DNA 损伤的影响。利用 GATE- 9.0 和 Geant4-DNA 软件包,蒙特卡罗模拟法模拟了一个数学模型,并确定了 AuNP 附近的能量沉积。模拟针对不同光子束能量(50、100、250 和 6000 keV)、不同尺寸 AuNPs(10、30、50 和 100 nm)的存在和不存在进行。使用 Geant4-DNA 评估了剂量增强因子 (DER),以研究 AuNP 尺寸和光子束能量对 DNA 损伤的影响。进行了多尺度蒙特卡洛模拟,以评估纳米粒子在癌细胞附近造成的 DNA 损伤增强。蒙特卡洛模拟结果表明,金纳米粒子提高了剂量传递,从而增强了能量沉积和随后的DNA损伤。DER 分析显示,DNA 内的剂量沉积明显增加,导致单链或双链断裂。Geant4-DNA 模拟揭示了不同 AuNP 尺寸和光子束强度下剂量增强因子的信息,从而加深了对基本力学的理解。这项研究的成果强调了 AuNPs 在放射治疗中作为有效放射增敏剂的潜力,并为越来越多的利用纳米技术提高癌症治疗效果的研究做出了贡献。要优化 AuNPs 的使用,提高放射治疗效果,还需要进一步的研究和实验验证。
{"title":"Gold nanoparticle effect on dose and DNA damage enhancement in the vicinity of gold nanoparticles","authors":"","doi":"10.1016/j.nucana.2024.100126","DOIUrl":"10.1016/j.nucana.2024.100126","url":null,"abstract":"<div><p>This study uses Monte Carlo simulations to examine the dose enhancement effect of gold nanoparticles (AuNPs) in radiation therapy and its effects on DNA damage. Using the GATE- 9.0 and Geant4-DNA packages, Monte Carlo simulations were used to simulate a mathematical phantom and determine the energy deposition in the vicinity of AuNP. The simulations were conducted for various photon beam energies (50, 100, 250, and 6000 keV) with and without the presence of different-size AuNPs (10, 30, 50 and 100 nm). The dose enhancement factor (DER) was evaluated using Geant4-DNA to examine the effects AuNP sizes and photon beam energies on DNA damage. A multi-scale Monte Carlo simulation was conducted to evaluate enhanced DNA damage owing to nanoparticles in the proximity of cancer cells. The Monte Carlo simulations indicated that AuNPs boost the dose delivery, resulting in enhanced energy deposition and subsequent DNA damage. The DER analysis revealed a significant increase in the dose deposition within DNA, leading to single or double-strand breaks. Geant4-DNA simulations revealed information on the dosage enhancement factor for various AuNP sizes and photon beam intensities, enabling a deeper comprehension of the underlying mechanics. The outcomes of this study emphasize the potential of AuNPs as effective radiosensitizers in radiation therapy and contribute to the growing body of research on the use of nanotechnology in enhancing cancer treatment outcomes. Further investigations and experimental validations are necessary to optimize the usage of AuNPs for improved radiation therapy.</p></div>","PeriodicalId":100965,"journal":{"name":"Nuclear Analysis","volume":null,"pages":null},"PeriodicalIF":0.0,"publicationDate":"2024-08-13","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.sciencedirect.com/science/article/pii/S2773183924000260/pdfft?md5=28fbf1d35df9f3b5d4b49c66adb0a166&pid=1-s2.0-S2773183924000260-main.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142011368","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Fusion mechanism involved in the synthesis of superheavy element Z>118 using Mn projectiles 利用锰射弹合成超重元素 Z>118 所涉及的聚变机制
Pub Date : 2024-08-06 DOI: 10.1016/j.nucana.2024.100124
<div><div>We conducted an in-depth investigation of Mn-induced fusion reactions aimed at synthesizing superheavy elements with atomic numbers Z=119 to Z=123. Our analysis considers the total potential, which combines Coulomb and nuclear potentials. The nuclear potential was calculated using the Thomas–Fermi approach, a valuable method for modeling the behavior of nucleons in atomic nuclei. within the framework of advanced statistical model, the evaporation residue cross-sections were determined. At optimal energies, we have calculated capture, fusion, and evaporation residue cross-sections for the reactions of all the projectile–target combinations. All <span><math><msup><mrow></mrow><mrow><mn>53</mn><mo>−</mo><mn>55</mn></mrow></msup></math></span>Mn isotopes with larger half-lives were taken into consideration as projectiles. Fusion reactions between <span><math><msup><mrow></mrow><mrow><mn>53</mn><mo>−</mo><mn>55</mn></mrow></msup></math></span>Mn projectiles with <span><math><msup><mrow></mrow><mrow><mn>238</mn><mo>−</mo><mn>242</mn><mo>,</mo><mn>244</mn></mrow></msup></math></span>Pu, <span><math><msup><mrow></mrow><mrow><mn>241</mn><mo>−</mo><mn>243</mn></mrow></msup></math></span>Am, <span><math><msup><mrow></mrow><mrow><mn>242</mn><mo>−</mo><mn>248</mn><mo>,</mo><mn>250</mn></mrow></msup></math></span>Cm, <span><math><msup><mrow></mrow><mrow><mn>247</mn><mo>−</mo><mn>249</mn></mrow></msup></math></span>Bk, and <span><math><msup><mrow></mrow><mrow><mn>248</mn><mo>−</mo><mn>254</mn></mrow></msup></math></span>Cf. Detailed investigations were made and promising reactions viz. <span><math><mrow><msup><mrow></mrow><mrow><mn>241</mn></mrow></msup><mi>Pu</mi></mrow></math></span> (<span><math><mrow><msup><mrow></mrow><mrow><mn>55</mn></mrow></msup><mi>Mn</mi></mrow></math></span>, 3n)<sup>293</sup>119, <span><math><mrow><msup><mrow></mrow><mrow><mn>242</mn></mrow></msup><mi>Am</mi></mrow></math></span> (<span><math><mrow><msup><mrow></mrow><mrow><mn>55</mn></mrow></msup><mi>Mn</mi></mrow></math></span>, 3n)<sup>294</sup>120, <span><math><mrow><msup><mrow></mrow><mrow><mn>247</mn></mrow></msup><mi>Cm</mi></mrow></math></span> (<span><math><mrow><msup><mrow></mrow><mrow><mn>55</mn></mrow></msup><mi>Mn</mi></mrow></math></span>, 3n)<sup>299</sup>121, <span><math><mrow><msup><mrow></mrow><mrow><mn>248</mn></mrow></msup><mi>Bk</mi></mrow></math></span> (<span><math><mrow><msup><mrow></mrow><mrow><mn>55</mn></mrow></msup><mi>Mn</mi></mrow></math></span>, 3n)<sup>300</sup>122 and <span><math><mrow><msup><mrow></mrow><mrow><mn>251</mn></mrow></msup><mi>Cf</mi></mrow></math></span> (<span><math><mrow><msup><mrow></mrow><mrow><mn>53</mn></mrow></msup><mi>Mn</mi></mrow></math></span>, 3n)<sup>301</sup>123 with maximum <span><math><msub><mrow><mi>σ</mi></mrow><mrow><mi>E</mi><mi>R</mi></mrow></msub></math></span> are found to be 415.1 fb at 240 MeV, 115.4 fb at 244 MeV, 36.5 fb at 245 MeV, 13.6 fb at 249 MeV, 5.4 fb at 250 MeV for Z=119-123 respectively. Th
我们对旨在合成原子序数为 Z=119 至 Z=123 的超重元素的锰诱导聚变反应进行了深入研究。我们的分析考虑了库仑势和核势相结合的总势能。核势能是用托马斯-费米方法计算的,这是一种模拟原子核中核子行为的重要方法。在最佳能量下,我们计算了所有射弹-靶组合反应的俘获、聚变和蒸发残余截面。所有具有较大半衰期的 53-55Mn 同位素都被视为射弹。对 53-55Mn 射弹与 238-242、244Pu、241-243Am、242-248、250Cm、247-249Bk 和 248-254Cf 之间的聚变反应进行了详细的研究,发现有希望的反应包括241Pu (55Mn, 3n)293119, 242Am (55Mn, 3n)294120, 247Cm (55Mn, 3n)299121, 248Bk (55Mn, 3n)300122 和 251Cf (53Mn, 3n)301123 的最大 σER 为 415.1 fb,244 MeV 时为 115.4 fb,245 MeV 时为 36.5 fb,249 MeV 时为 13.6 fb,250 MeV 时为 5.4 fb。这些预测可能有助于未来的实验人员探索元素周期表中的第 8 行。
{"title":"Fusion mechanism involved in the synthesis of superheavy element Z>118 using Mn projectiles","authors":"","doi":"10.1016/j.nucana.2024.100124","DOIUrl":"10.1016/j.nucana.2024.100124","url":null,"abstract":"&lt;div&gt;&lt;div&gt;We conducted an in-depth investigation of Mn-induced fusion reactions aimed at synthesizing superheavy elements with atomic numbers Z=119 to Z=123. Our analysis considers the total potential, which combines Coulomb and nuclear potentials. The nuclear potential was calculated using the Thomas–Fermi approach, a valuable method for modeling the behavior of nucleons in atomic nuclei. within the framework of advanced statistical model, the evaporation residue cross-sections were determined. At optimal energies, we have calculated capture, fusion, and evaporation residue cross-sections for the reactions of all the projectile–target combinations. All &lt;span&gt;&lt;math&gt;&lt;msup&gt;&lt;mrow&gt;&lt;/mrow&gt;&lt;mrow&gt;&lt;mn&gt;53&lt;/mn&gt;&lt;mo&gt;−&lt;/mo&gt;&lt;mn&gt;55&lt;/mn&gt;&lt;/mrow&gt;&lt;/msup&gt;&lt;/math&gt;&lt;/span&gt;Mn isotopes with larger half-lives were taken into consideration as projectiles. Fusion reactions between &lt;span&gt;&lt;math&gt;&lt;msup&gt;&lt;mrow&gt;&lt;/mrow&gt;&lt;mrow&gt;&lt;mn&gt;53&lt;/mn&gt;&lt;mo&gt;−&lt;/mo&gt;&lt;mn&gt;55&lt;/mn&gt;&lt;/mrow&gt;&lt;/msup&gt;&lt;/math&gt;&lt;/span&gt;Mn projectiles with &lt;span&gt;&lt;math&gt;&lt;msup&gt;&lt;mrow&gt;&lt;/mrow&gt;&lt;mrow&gt;&lt;mn&gt;238&lt;/mn&gt;&lt;mo&gt;−&lt;/mo&gt;&lt;mn&gt;242&lt;/mn&gt;&lt;mo&gt;,&lt;/mo&gt;&lt;mn&gt;244&lt;/mn&gt;&lt;/mrow&gt;&lt;/msup&gt;&lt;/math&gt;&lt;/span&gt;Pu, &lt;span&gt;&lt;math&gt;&lt;msup&gt;&lt;mrow&gt;&lt;/mrow&gt;&lt;mrow&gt;&lt;mn&gt;241&lt;/mn&gt;&lt;mo&gt;−&lt;/mo&gt;&lt;mn&gt;243&lt;/mn&gt;&lt;/mrow&gt;&lt;/msup&gt;&lt;/math&gt;&lt;/span&gt;Am, &lt;span&gt;&lt;math&gt;&lt;msup&gt;&lt;mrow&gt;&lt;/mrow&gt;&lt;mrow&gt;&lt;mn&gt;242&lt;/mn&gt;&lt;mo&gt;−&lt;/mo&gt;&lt;mn&gt;248&lt;/mn&gt;&lt;mo&gt;,&lt;/mo&gt;&lt;mn&gt;250&lt;/mn&gt;&lt;/mrow&gt;&lt;/msup&gt;&lt;/math&gt;&lt;/span&gt;Cm, &lt;span&gt;&lt;math&gt;&lt;msup&gt;&lt;mrow&gt;&lt;/mrow&gt;&lt;mrow&gt;&lt;mn&gt;247&lt;/mn&gt;&lt;mo&gt;−&lt;/mo&gt;&lt;mn&gt;249&lt;/mn&gt;&lt;/mrow&gt;&lt;/msup&gt;&lt;/math&gt;&lt;/span&gt;Bk, and &lt;span&gt;&lt;math&gt;&lt;msup&gt;&lt;mrow&gt;&lt;/mrow&gt;&lt;mrow&gt;&lt;mn&gt;248&lt;/mn&gt;&lt;mo&gt;−&lt;/mo&gt;&lt;mn&gt;254&lt;/mn&gt;&lt;/mrow&gt;&lt;/msup&gt;&lt;/math&gt;&lt;/span&gt;Cf. Detailed investigations were made and promising reactions viz. &lt;span&gt;&lt;math&gt;&lt;mrow&gt;&lt;msup&gt;&lt;mrow&gt;&lt;/mrow&gt;&lt;mrow&gt;&lt;mn&gt;241&lt;/mn&gt;&lt;/mrow&gt;&lt;/msup&gt;&lt;mi&gt;Pu&lt;/mi&gt;&lt;/mrow&gt;&lt;/math&gt;&lt;/span&gt; (&lt;span&gt;&lt;math&gt;&lt;mrow&gt;&lt;msup&gt;&lt;mrow&gt;&lt;/mrow&gt;&lt;mrow&gt;&lt;mn&gt;55&lt;/mn&gt;&lt;/mrow&gt;&lt;/msup&gt;&lt;mi&gt;Mn&lt;/mi&gt;&lt;/mrow&gt;&lt;/math&gt;&lt;/span&gt;, 3n)&lt;sup&gt;293&lt;/sup&gt;119, &lt;span&gt;&lt;math&gt;&lt;mrow&gt;&lt;msup&gt;&lt;mrow&gt;&lt;/mrow&gt;&lt;mrow&gt;&lt;mn&gt;242&lt;/mn&gt;&lt;/mrow&gt;&lt;/msup&gt;&lt;mi&gt;Am&lt;/mi&gt;&lt;/mrow&gt;&lt;/math&gt;&lt;/span&gt; (&lt;span&gt;&lt;math&gt;&lt;mrow&gt;&lt;msup&gt;&lt;mrow&gt;&lt;/mrow&gt;&lt;mrow&gt;&lt;mn&gt;55&lt;/mn&gt;&lt;/mrow&gt;&lt;/msup&gt;&lt;mi&gt;Mn&lt;/mi&gt;&lt;/mrow&gt;&lt;/math&gt;&lt;/span&gt;, 3n)&lt;sup&gt;294&lt;/sup&gt;120, &lt;span&gt;&lt;math&gt;&lt;mrow&gt;&lt;msup&gt;&lt;mrow&gt;&lt;/mrow&gt;&lt;mrow&gt;&lt;mn&gt;247&lt;/mn&gt;&lt;/mrow&gt;&lt;/msup&gt;&lt;mi&gt;Cm&lt;/mi&gt;&lt;/mrow&gt;&lt;/math&gt;&lt;/span&gt; (&lt;span&gt;&lt;math&gt;&lt;mrow&gt;&lt;msup&gt;&lt;mrow&gt;&lt;/mrow&gt;&lt;mrow&gt;&lt;mn&gt;55&lt;/mn&gt;&lt;/mrow&gt;&lt;/msup&gt;&lt;mi&gt;Mn&lt;/mi&gt;&lt;/mrow&gt;&lt;/math&gt;&lt;/span&gt;, 3n)&lt;sup&gt;299&lt;/sup&gt;121, &lt;span&gt;&lt;math&gt;&lt;mrow&gt;&lt;msup&gt;&lt;mrow&gt;&lt;/mrow&gt;&lt;mrow&gt;&lt;mn&gt;248&lt;/mn&gt;&lt;/mrow&gt;&lt;/msup&gt;&lt;mi&gt;Bk&lt;/mi&gt;&lt;/mrow&gt;&lt;/math&gt;&lt;/span&gt; (&lt;span&gt;&lt;math&gt;&lt;mrow&gt;&lt;msup&gt;&lt;mrow&gt;&lt;/mrow&gt;&lt;mrow&gt;&lt;mn&gt;55&lt;/mn&gt;&lt;/mrow&gt;&lt;/msup&gt;&lt;mi&gt;Mn&lt;/mi&gt;&lt;/mrow&gt;&lt;/math&gt;&lt;/span&gt;, 3n)&lt;sup&gt;300&lt;/sup&gt;122 and &lt;span&gt;&lt;math&gt;&lt;mrow&gt;&lt;msup&gt;&lt;mrow&gt;&lt;/mrow&gt;&lt;mrow&gt;&lt;mn&gt;251&lt;/mn&gt;&lt;/mrow&gt;&lt;/msup&gt;&lt;mi&gt;Cf&lt;/mi&gt;&lt;/mrow&gt;&lt;/math&gt;&lt;/span&gt; (&lt;span&gt;&lt;math&gt;&lt;mrow&gt;&lt;msup&gt;&lt;mrow&gt;&lt;/mrow&gt;&lt;mrow&gt;&lt;mn&gt;53&lt;/mn&gt;&lt;/mrow&gt;&lt;/msup&gt;&lt;mi&gt;Mn&lt;/mi&gt;&lt;/mrow&gt;&lt;/math&gt;&lt;/span&gt;, 3n)&lt;sup&gt;301&lt;/sup&gt;123 with maximum &lt;span&gt;&lt;math&gt;&lt;msub&gt;&lt;mrow&gt;&lt;mi&gt;σ&lt;/mi&gt;&lt;/mrow&gt;&lt;mrow&gt;&lt;mi&gt;E&lt;/mi&gt;&lt;mi&gt;R&lt;/mi&gt;&lt;/mrow&gt;&lt;/msub&gt;&lt;/math&gt;&lt;/span&gt; are found to be 415.1 fb at 240 MeV, 115.4 fb at 244 MeV, 36.5 fb at 245 MeV, 13.6 fb at 249 MeV, 5.4 fb at 250 MeV for Z=119-123 respectively. Th","PeriodicalId":100965,"journal":{"name":"Nuclear Analysis","volume":null,"pages":null},"PeriodicalIF":0.0,"publicationDate":"2024-08-06","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142327640","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Evaluation of Potassium-40 and Uranium-238 activities and radiological risk in Missour, Morocco soils using gamma spectrometry 利用伽马能谱仪评估摩洛哥米苏尔土壤中钾-40 和铀-238 的放射性活度及辐射风险
Pub Date : 2024-08-05 DOI: 10.1016/j.nucana.2024.100125

The objective of this study is to assess natural activity in soil to estimate potential radiological risks for the population. Given that soil is inherently radioactive and can reach hazardous levels, it is crucial to determine the activities of radionuclides such as Potassium-40 and Uranium-238 descendants at different depths and geographical positions. For this work, gamma spectrometry method was employed to analyze soil samples collected at three different positions in the Missour region. Each position was sampled at five different depths, spaced 5 cm apart, resulting in a total of 15 samples. The activity of Potassium-40 and Uranium238 descendants in the soil was accurately assessed using Lvis software, enabling the estimation of radiological doses.

这项研究的目的是评估土壤中的天然放射性活度,以估计对人口的潜在辐射风险。鉴于土壤本身具有放射性,并可达到危险水平,因此确定不同深度和地理位置的放射性核素(如钾-40 和铀-238 后裔)的放射性活度至关重要。在这项工作中,采用了伽马能谱法分析在米苏尔地区三个不同位置采集的土壤样本。每个位置采集了五个不同深度的样本,样本间距为 5 厘米,共采集了 15 个样本。利用 Lvis 软件对土壤中钾-40 和铀-238 后裔的活度进行了准确评估,从而估算出辐射剂量。
{"title":"Evaluation of Potassium-40 and Uranium-238 activities and radiological risk in Missour, Morocco soils using gamma spectrometry","authors":"","doi":"10.1016/j.nucana.2024.100125","DOIUrl":"10.1016/j.nucana.2024.100125","url":null,"abstract":"<div><p>The objective of this study is to assess natural activity in soil to estimate potential radiological risks for the population. Given that soil is inherently radioactive and can reach hazardous levels, it is crucial to determine the activities of radionuclides such as Potassium-40 and Uranium-238 descendants at different depths and geographical positions. For this work, gamma spectrometry method was employed to analyze soil samples collected at three different positions in the Missour region. Each position was sampled at five different depths, spaced 5 cm apart, resulting in a total of 15 samples. The activity of Potassium-40 and Uranium238 descendants in the soil was accurately assessed using Lvis software, enabling the estimation of radiological doses.</p></div>","PeriodicalId":100965,"journal":{"name":"Nuclear Analysis","volume":null,"pages":null},"PeriodicalIF":0.0,"publicationDate":"2024-08-05","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.sciencedirect.com/science/article/pii/S2773183924000259/pdfft?md5=b064fa8f6785305a19ec020d1f7ebcfe&pid=1-s2.0-S2773183924000259-main.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141964342","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Compound nucleus formation probability of heavy and superheavy nuclei synthesized using heavy ion fusion reactions 利用重离子聚变反应合成的重核和超重核的复合核形成概率
Pub Date : 2024-07-31 DOI: 10.1016/j.nucana.2024.100123
The role of entrance channel parameters such as Z2/A, charge asymmetry αz, mass-asymmetry (ηA), charge product (Z1Z2), mean fissility χm, Coulomb interaction parameter and (NZ)/(N+Z) on compound nucleus formation of actinide nuclei using heavy ion fusion reactions were investigated. For the formation of compound nuclei, the considered atomic number range of the projectile varies between 5Z14 and the mass number lies between 10A34. Similarly, the studied target atomic number varies between 78Z92 and the mass number range is 197A238. Among these entrance channel parameters, PCN is more systematic for (NZ)(N+Z), Z2/A and αz. In addition to entrance channel parameters, the Ecm and EBass also play a significant role in the prediction of PCN. The proposed empirical formulae are applicable to the compound nuclei from Fr to Sg. These findings are significant for the PCN prediction from Fr to Sg.
研究了入口通道参数,如 Z2/A、电荷不对称性 αz、质量不对称性 (ηA)、电荷乘积 (Z1Z2)、平均裂变率 χm、库仑相互作用参数和 (N-Z)/(N+Z) 对利用重离子聚变反应形成锕系核的复合核的作用。为了形成复合核,考虑的射弹原子序数范围在 5≤Z≤14 之间,质量数在 10≤A≤34 之间。同样,研究的靶原子序数在 78≤Z≤92 之间变化,质量数范围为 197≤A≤238。在这些入口通道参数中,(N-Z)(N+Z)、Z2/A 和 αz 的 PCN 更有系统性。除入口通道参数外,Ecm 和 EBass 对 PCN 的预测也起着重要作用。所提出的经验公式适用于从 Fr 到 Sg 的化合物核。这些发现对于从 Fr 到 Sg 的 PCN 预测具有重要意义。
{"title":"Compound nucleus formation probability of heavy and superheavy nuclei synthesized using heavy ion fusion reactions","authors":"","doi":"10.1016/j.nucana.2024.100123","DOIUrl":"10.1016/j.nucana.2024.100123","url":null,"abstract":"<div><div>The role of entrance channel parameters such as <span><math><mrow><msup><mrow><mi>Z</mi></mrow><mrow><mn>2</mn></mrow></msup><mo>/</mo><mi>A</mi></mrow></math></span>, charge asymmetry <span><math><msub><mrow><mi>α</mi></mrow><mrow><mi>z</mi></mrow></msub></math></span>, mass-asymmetry (<span><math><msub><mrow><mi>η</mi></mrow><mrow><mi>A</mi></mrow></msub></math></span>), charge product (<span><math><mrow><msub><mrow><mi>Z</mi></mrow><mrow><mn>1</mn></mrow></msub><msub><mrow><mi>Z</mi></mrow><mrow><mn>2</mn></mrow></msub></mrow></math></span>), mean fissility <span><math><msub><mrow><mi>χ</mi></mrow><mrow><mi>m</mi></mrow></msub></math></span>, Coulomb interaction parameter and <span><math><mrow><mrow><mo>(</mo><mi>N</mi><mo>−</mo><mi>Z</mi><mo>)</mo></mrow><mo>/</mo><mrow><mo>(</mo><mi>N</mi><mo>+</mo><mi>Z</mi><mo>)</mo></mrow></mrow></math></span> on compound nucleus formation of actinide nuclei using heavy ion fusion reactions were investigated. For the formation of compound nuclei, the considered atomic number range of the projectile varies between <span><math><mrow><mn>5</mn><mo>≤</mo><mi>Z</mi><mo>≤</mo><mn>14</mn></mrow></math></span> and the mass number lies between <span><math><mrow><mn>10</mn><mo>≤</mo><mi>A</mi><mo>≤</mo><mn>34</mn></mrow></math></span>. Similarly, the studied target atomic number varies between <span><math><mrow><mn>78</mn><mo>≤</mo><mi>Z</mi><mo>≤</mo><mn>92</mn></mrow></math></span> and the mass number range is <span><math><mrow><mn>197</mn><mo>≤</mo><mi>A</mi><mo>≤</mo><mn>238</mn></mrow></math></span>. Among these entrance channel parameters, <span><math><msub><mrow><mi>P</mi></mrow><mrow><mi>C</mi><mi>N</mi></mrow></msub></math></span> is more systematic for <span><math><mfrac><mrow><mrow><mo>(</mo><mi>N</mi><mo>−</mo><mi>Z</mi><mo>)</mo></mrow></mrow><mrow><mrow><mo>(</mo><mi>N</mi><mo>+</mo><mi>Z</mi><mo>)</mo></mrow></mrow></mfrac></math></span>, <span><math><mrow><msup><mrow><mi>Z</mi></mrow><mrow><mn>2</mn></mrow></msup><mo>/</mo><mi>A</mi></mrow></math></span> and <span><math><msub><mrow><mi>α</mi></mrow><mrow><mi>z</mi></mrow></msub></math></span>. In addition to entrance channel parameters, the <span><math><msub><mrow><mi>E</mi></mrow><mrow><mi>c</mi><mi>m</mi></mrow></msub></math></span> and <span><math><msub><mrow><mi>E</mi></mrow><mrow><mi>B</mi><mi>a</mi><mi>s</mi><mi>s</mi></mrow></msub></math></span> also play a significant role in the prediction of <span><math><msub><mrow><mi>P</mi></mrow><mrow><mi>C</mi><mi>N</mi></mrow></msub></math></span>. The proposed empirical formulae are applicable to the compound nuclei from Fr to Sg. These findings are significant for the <span><math><msub><mrow><mi>P</mi></mrow><mrow><mi>C</mi><mi>N</mi></mrow></msub></math></span> prediction from Fr to Sg.</div></div>","PeriodicalId":100965,"journal":{"name":"Nuclear Analysis","volume":null,"pages":null},"PeriodicalIF":0.0,"publicationDate":"2024-07-31","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142358342","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Feasibility of producing 225Ac via thermal neutron irradiation of 226Ra: A systematic theoretical study 通过热中子辐照 226Ra 生产 225Ac 的可行性:系统理论研究
Pub Date : 2024-07-20 DOI: 10.1016/j.nucana.2024.100122

With a suitable half-life and abundant radiolabeling strategy, 225Ac has become one of the most promising radionuclides in the area of targeted alpha therapy. However, limited radionuclide supply is threatening the development of 225Ac related endoradiotherapy dramatically. As the parent nuclide of 225Ac, 229Th can be produced via 226Ra(3n, 2β)229Th reaction in a nuclear reactor. However, related practice has not been conducted in large scale, since the nuclear reaction pathway for producing 229Th is complicated. In this work, the feasibility of producing 225Ac/229Th in a reactor was confirmed by systematic theoretical calculations, and a procedure that combines irradiation with separation process was proposed. The results show that 176 MBq of 229Th can be produced by irradiating 1.0 g of 226Ra with a neutron flux density of 1 × 1015 n cm−2 s−1 for 90 days. This will generate 150 MBq of 225Ac monthly from a radionuclide generator, which is sufficient for the single treatment cycle of 200 patients each year considering the radioactivity loss in radiochemical separation, transfer and radiolabeling process. In addition, this irradiation process will also produce 37.8 GBq 227Ac for the preparation of 227Ac-227Th-223Ra generator. In general, the production of 225Ac by neutron irradiation of 226Ra in reactor is practicable and holds potential to alleviate the shortage of current supply of 225Ac.

225Ac 具有合适的半衰期和丰富的放射性标记策略,已成为α靶向治疗领域最有前途的放射性核素之一。然而,有限的放射性核素供应正极大地威胁着与 225Ac 相关的放射治疗的发展。作为 225Ac 的母核素,229Th 可在核反应堆中通过 226Ra(3n,2β)229Th 反应生成。然而,由于产生 229Th 的核反应途径复杂,相关实践尚未大规模开展。在这项工作中,通过系统的理论计算证实了在反应堆中生产 225Ac/229Th 的可行性,并提出了一种将辐照与分离过程相结合的程序。结果表明,用 1 × 1015 n cm-2 s-1 的中子通量密度对 1.0 克 226Ra 进行辐照 90 天,可产生 176 MBq 的 229Th。考虑到放射化学分离、转移和放射性标记过程中的放射性损失,这足以满足每年 200 名患者一个治疗周期的需要。此外,这一辐照过程还将产生 37.8 GBq 227Ac 用于制备 227Ac-227Th-223Ra 发生器。总之,在反应堆中用中子辐照 226Ra 生产 225Ac 是切实可行的,并有可能缓解目前 225Ac 供应短缺的问题。
{"title":"Feasibility of producing 225Ac via thermal neutron irradiation of 226Ra: A systematic theoretical study","authors":"","doi":"10.1016/j.nucana.2024.100122","DOIUrl":"10.1016/j.nucana.2024.100122","url":null,"abstract":"<div><p>With a suitable half-life and abundant radiolabeling strategy, <sup>225</sup>Ac has become one of the most promising radionuclides in the area of targeted alpha therapy. However, limited radionuclide supply is threatening the development of <sup>225</sup>Ac related endoradiotherapy dramatically. As the parent nuclide of <sup>225</sup>Ac, <sup>229</sup>Th can be produced via <sup>226</sup>Ra(3n, 2β)<sup>229</sup>Th reaction in a nuclear reactor. However, related practice has not been conducted in large scale, since the nuclear reaction pathway for producing <sup>229</sup>Th is complicated. In this work, the feasibility of producing <sup>225</sup>Ac/<sup>229</sup>Th in a reactor was confirmed by systematic theoretical calculations, and a procedure that combines irradiation with separation process was proposed. The results show that 176 MBq of <sup>229</sup>Th can be produced by irradiating 1.0 g of <sup>226</sup>Ra with a neutron flux density of 1 × 10<sup>15</sup> n cm<sup>−2</sup> s<sup>−1</sup> for 90 days. This will generate 150 MBq of <sup>225</sup>Ac monthly from a radionuclide generator, which is sufficient for the single treatment cycle of 200 patients each year considering the radioactivity loss in radiochemical separation, transfer and radiolabeling process. In addition, this irradiation process will also produce 37.8 GBq <sup>227</sup>Ac for the preparation of <sup>227</sup>Ac-<sup>227</sup>Th-<sup>223</sup>Ra generator. In general, the production of <sup>225</sup>Ac by neutron irradiation of <sup>226</sup>Ra in reactor is practicable and holds potential to alleviate the shortage of current supply of <sup>225</sup>Ac.</p></div>","PeriodicalId":100965,"journal":{"name":"Nuclear Analysis","volume":null,"pages":null},"PeriodicalIF":0.0,"publicationDate":"2024-07-20","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.sciencedirect.com/science/article/pii/S2773183924000223/pdfft?md5=459ab0fb9ccb924e8ab5a6fed4199880&pid=1-s2.0-S2773183924000223-main.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141839148","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Radiological impact of hydrocarbon waste release on drinking water of ughievwen and udu communities, delta state Nigeria 碳氢化合物废物排放对尼日利亚三角洲州 Ughievwen 和 Udu 社区饮用水的辐射影响
Pub Date : 2024-07-16 DOI: 10.1016/j.nucana.2024.100121

Well water quality has been characterized with constant and continuous changes via the interaction of rock, soil and natural nano-filters which terminates at the aquiferous layer for clean well-water collection. The continuous exploration and production of crude oil has resulted significant increase of unwanted elements such as naturally occurring radionuclides in the water-bed which necessitates this study. The study determines the radionuclides based health impact or hazards associated with drinking water from crude oil exploration/production release in Ughievwen and Udu communities of Delta State, Nigeria. Sixty well water samples (three samples from each community) were collected and analyzed using sodium iodide (Nal (Tl)) detector. The obtained mean values of 238U, 232Th and 40K are 6.91 ± 1.62BqL−1, 4.39 ± 1.47 BqL−1 and 24.54 ± 1.59 BqL−1 respectively. The 238U, 232Th and 40K results showed that the measured values are higher than the world standard (UNSCEAR; WHO) and the control values The mean values of total annual effective dose of different age groups are: 11.08 mSvy−1, 2.54 mSvy−1, 1.93 mSvy−1, 2.52 mSvy−1, 7.03 mSvy−1 and 1.12 mSvy−1 respectively. While the mean committed effective dose of adult is 55.94 mSvy−1. The total annual effective dose, committed effective dose, cancer risks and hereditary effects are all lower than recommended limit (WHO; ICRP; USEPA) and reported scientific values except 11.08 mSvy−1 and 7.03 mSvy−1 that are higher than limit. It is evident from obtained results that the drinking water may not be radiologically safe for use by the public, which necessitates routine monitoring and caution to circumvent increase in radiation and the radiological of the studied communities’ drinking water. This is to avoid long term radiological risk arising from accumulation of such release in the studied communities.

井水水质的特点是通过岩石、土壤和天然纳米过滤器的相互作用不断发生持续变化,最终在含水层收集清洁的井水。原油的不断勘探和生产导致水床中的有害元素(如天然放射性核素)显著增加,因此有必要进行这项研究。本研究确定了尼日利亚三角洲州 Ughievwen 和 Udu 社区原油勘探/生产释放的饮用水中放射性核素对健康的影响或危害。研究人员收集了 60 份井水样本(每个社区 3 份),并使用碘化钠(Nal (Tl))检测器进行了分析。获得的 238U、232Th 和 40K 平均值分别为 6.91 ± 1.62BqL-1 、 4.39 ± 1.47 BqL-1 和 24.54 ± 1.59 BqL-1。238U、232Th 和 40K 的测量结果表明,测量值高于世界标准值(UNSCEAR;WHO)和对照值:11.08 mSvy-1、2.54 mSvy-1、1.93 mSvy-1、2.52 mSvy-1、7.03 mSvy-1 和 1.12 mSvy-1。成人的平均承诺有效剂量为 55.94 mSvy-1。除 11.08 mSvy-1 和 7.03 mSvy-1 高于推荐限值外,其余的年总有效剂量、承诺有效剂量、癌症风险和遗传影响均低于推荐限值(世界卫生组织、国际癌症研究委员会、美国环保局)和报告的科学值。从获得的结果可以看出,公众使用的饮用水在辐射方面可能并不安全,因此有必要进行例行监测并采取谨慎措施,以避免辐射的增加和所研究社区饮用水的辐射性。这样做是为了避免在所研究的社区中因这种释放的累积而产生长期的辐射风险。
{"title":"Radiological impact of hydrocarbon waste release on drinking water of ughievwen and udu communities, delta state Nigeria","authors":"","doi":"10.1016/j.nucana.2024.100121","DOIUrl":"10.1016/j.nucana.2024.100121","url":null,"abstract":"<div><p>Well water quality has been characterized with constant and continuous changes via the interaction of rock, soil and natural nano-filters which terminates at the aquiferous layer for clean well-water collection. The continuous exploration and production of crude oil has resulted significant increase of unwanted elements such as naturally occurring radionuclides in the water-bed which necessitates this study. The study determines the radionuclides based health impact or hazards associated with drinking water from crude oil exploration/production release in Ughievwen and Udu communities of Delta State, Nigeria. Sixty well water samples (three samples from each community) were collected and analyzed using sodium iodide (Nal (Tl)) detector. The obtained mean values of <sup>238</sup>U, <sup>232</sup>Th and <sup>40</sup>K are 6.91 <span><math><mrow><mo>±</mo></mrow></math></span> 1.62BqL<sup>−1</sup>, 4.39 <span><math><mrow><mo>±</mo></mrow></math></span> 1.47 BqL<sup>−1</sup> and 24.54 <span><math><mrow><mo>±</mo></mrow></math></span> 1.59 BqL<sup>−1</sup> respectively. The <sup>238</sup>U, <sup>232</sup>Th and <sup>40</sup>K results showed that the measured values are higher than the world standard (UNSCEAR; WHO) and the control values The mean values of total annual effective dose of different age groups are: 11.08 mSvy<sup>−1</sup>, 2.54 mSvy<sup>−1</sup>, 1.93 mSvy<sup>−1</sup>, 2.52 mSvy<sup>−1</sup>, 7.03 mSvy<sup>−1</sup> and 1.12 mSvy<sup>−1</sup> respectively. While the mean committed effective dose of adult is 55.94 mSvy<sup>−1</sup>. The total annual effective dose, committed effective dose, cancer risks and hereditary effects are all lower than recommended limit (WHO; ICRP; USEPA) and reported scientific values except 11.08 mSvy<sup>−1</sup> and 7.03 mSvy<sup>−1</sup> that are higher than limit. It is evident from obtained results that the drinking water may not be radiologically safe for use by the public, which necessitates routine monitoring and caution to circumvent increase in radiation and the radiological of the studied communities’ drinking water. This is to avoid long term radiological risk arising from accumulation of such release in the studied communities.</p></div>","PeriodicalId":100965,"journal":{"name":"Nuclear Analysis","volume":null,"pages":null},"PeriodicalIF":0.0,"publicationDate":"2024-07-16","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.sciencedirect.com/science/article/pii/S2773183924000211/pdfft?md5=869ab386a09f2b2eca91c3c05f0eb686&pid=1-s2.0-S2773183924000211-main.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141850667","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
期刊
Nuclear Analysis
全部 Acc. Chem. Res. ACS Applied Bio Materials ACS Appl. Electron. Mater. ACS Appl. Energy Mater. ACS Appl. Mater. Interfaces ACS Appl. Nano Mater. ACS Appl. Polym. Mater. ACS BIOMATER-SCI ENG ACS Catal. ACS Cent. Sci. ACS Chem. Biol. ACS Chemical Health & Safety ACS Chem. Neurosci. ACS Comb. Sci. ACS Earth Space Chem. ACS Energy Lett. ACS Infect. Dis. ACS Macro Lett. ACS Mater. Lett. ACS Med. Chem. Lett. ACS Nano ACS Omega ACS Photonics ACS Sens. ACS Sustainable Chem. Eng. ACS Synth. Biol. Anal. Chem. BIOCHEMISTRY-US Bioconjugate Chem. BIOMACROMOLECULES Chem. Res. Toxicol. Chem. Rev. Chem. Mater. CRYST GROWTH DES ENERG FUEL Environ. Sci. Technol. Environ. Sci. Technol. Lett. Eur. J. Inorg. Chem. IND ENG CHEM RES Inorg. Chem. J. Agric. Food. Chem. J. Chem. Eng. Data J. Chem. Educ. J. Chem. Inf. Model. J. Chem. Theory Comput. J. Med. Chem. J. Nat. Prod. J PROTEOME RES J. Am. Chem. Soc. LANGMUIR MACROMOLECULES Mol. Pharmaceutics Nano Lett. Org. Lett. ORG PROCESS RES DEV ORGANOMETALLICS J. Org. Chem. J. Phys. Chem. J. Phys. Chem. A J. Phys. Chem. B J. Phys. Chem. C J. Phys. Chem. Lett. Analyst Anal. Methods Biomater. Sci. Catal. Sci. Technol. Chem. Commun. Chem. Soc. Rev. CHEM EDUC RES PRACT CRYSTENGCOMM Dalton Trans. Energy Environ. Sci. ENVIRON SCI-NANO ENVIRON SCI-PROC IMP ENVIRON SCI-WAT RES Faraday Discuss. Food Funct. Green Chem. Inorg. Chem. Front. Integr. Biol. J. Anal. At. Spectrom. J. Mater. Chem. A J. Mater. Chem. B J. Mater. Chem. C Lab Chip Mater. Chem. Front. Mater. Horiz. MEDCHEMCOMM Metallomics Mol. Biosyst. Mol. Syst. Des. Eng. Nanoscale Nanoscale Horiz. Nat. Prod. Rep. New J. Chem. Org. Biomol. Chem. Org. Chem. Front. PHOTOCH PHOTOBIO SCI PCCP Polym. Chem.
×
引用
GB/T 7714-2015
复制
MLA
复制
APA
复制
导出至
BibTeX EndNote RefMan NoteFirst NoteExpress
×
0
微信
客服QQ
Book学术公众号 扫码关注我们
反馈
×
意见反馈
请填写您的意见或建议
请填写您的手机或邮箱
×
提示
您的信息不完整,为了账户安全,请先补充。
现在去补充
×
提示
您因"违规操作"
具体请查看互助需知
我知道了
×
提示
现在去查看 取消
×
提示
确定
Book学术官方微信
Book学术文献互助
Book学术文献互助群
群 号:481959085
Book学术
文献互助 智能选刊 最新文献 互助须知 联系我们:info@booksci.cn
Book学术提供免费学术资源搜索服务,方便国内外学者检索中英文文献。致力于提供最便捷和优质的服务体验。
Copyright © 2023 Book学术 All rights reserved.
ghs 京公网安备 11010802042870号 京ICP备2023020795号-1