{"title":"绝热预成型中催化剂失活:性能预测的实验方法和模型","authors":"T. Christensen, J. Rostrup-Nielsen","doi":"10.1021/bk-1996-0634.ch013","DOIUrl":null,"url":null,"abstract":"Adiabatic prereforming is a low-temperature steam reforming process used in modern syngas production. Catalyst deactivation plays an important role in design of adiabatic prereforming and the low-temperature operation requires a high-activity catalyst with resistance to poisoning. This paper presents a model for the complex interaction of chemical reactions, poisoning mechanisms and pore diffusion that results in deactivation of prereforming catalyst","PeriodicalId":20402,"journal":{"name":"Preprints-American Chemical Society Division of Petroleum Chemistry","volume":"C-24 1","pages":"433-436"},"PeriodicalIF":0.0000,"publicationDate":"1995-12-31","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"5","resultStr":"{\"title\":\"Catalyst deactivation in adiabatic prereforming: Experimental methods and models for prediction of performance\",\"authors\":\"T. Christensen, J. Rostrup-Nielsen\",\"doi\":\"10.1021/bk-1996-0634.ch013\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"Adiabatic prereforming is a low-temperature steam reforming process used in modern syngas production. Catalyst deactivation plays an important role in design of adiabatic prereforming and the low-temperature operation requires a high-activity catalyst with resistance to poisoning. This paper presents a model for the complex interaction of chemical reactions, poisoning mechanisms and pore diffusion that results in deactivation of prereforming catalyst\",\"PeriodicalId\":20402,\"journal\":{\"name\":\"Preprints-American Chemical Society Division of Petroleum Chemistry\",\"volume\":\"C-24 1\",\"pages\":\"433-436\"},\"PeriodicalIF\":0.0000,\"publicationDate\":\"1995-12-31\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"5\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Preprints-American Chemical Society Division of Petroleum Chemistry\",\"FirstCategoryId\":\"1085\",\"ListUrlMain\":\"https://doi.org/10.1021/bk-1996-0634.ch013\",\"RegionNum\":0,\"RegionCategory\":null,\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"\",\"JCRName\":\"\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Preprints-American Chemical Society Division of Petroleum Chemistry","FirstCategoryId":"1085","ListUrlMain":"https://doi.org/10.1021/bk-1996-0634.ch013","RegionNum":0,"RegionCategory":null,"ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"","JCRName":"","Score":null,"Total":0}
Catalyst deactivation in adiabatic prereforming: Experimental methods and models for prediction of performance
Adiabatic prereforming is a low-temperature steam reforming process used in modern syngas production. Catalyst deactivation plays an important role in design of adiabatic prereforming and the low-temperature operation requires a high-activity catalyst with resistance to poisoning. This paper presents a model for the complex interaction of chemical reactions, poisoning mechanisms and pore diffusion that results in deactivation of prereforming catalyst