非平衡态激子凝聚体WSe2的超快生成和熔化

E. Perfetto, G. Stefanucci
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引用次数: 3

摘要

本文研究了在以最低能量激子共振的相干光照射下,体WSe$_{2}$中非平衡激子凝聚形成的屏蔽动力学。谷间散射导致电子从光填充的K谷迁移到传导带最小值$\Sigma$。由于K点的电子-空穴不平衡,产生了准自由空穴等离子体,有效地屏蔽了剩余激子的相互作用。我们发现这种等离子体筛选导致非平衡态的超快熔化,并且在熔化过程中相干激子和准自由电子-空穴对共存。时间分辨谱函数确实表现出相反凸性的传导和激子边带以及随时间变化的相对谱权。随时间变化的导通密度与激光强度的关系以及随时间变化的谱函数与最近的实验结果一致。
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Ultrafast creation and melting of nonequilibrium excitonic condensates in bulk WSe2
We study the screened dynamics of the nonequilibrium excitonic consensate forming in a bulk WSe$_{2}$ when illuminated by coherent light resonant with the lowest-energy exciton. Intervalley scattering causes electron migration from the optically populated K valley to the conduction band minimum at $\Sigma$. Due to the electron-hole unbalance at the K point a plasma of quasi-free holes develops, which efficiently screens the interaction of the remaining excitons. We show that this plasma screening causes an ultrafast melting of the nonequilibrium consensate and that during melting coherent excitons and quasi-free electron-hole pairs coexist. The time-resolved spectral function does exhibit a conduction and excitonic sidebands of opposite convexity and relative spectral weight that changes in time. Both the dependence of the time-dependent conduction density on the laser intensity and the time-resolved spectral function agree with recent experiments.
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