利用Hydrus-3d进行Sr-90在变饱和土中的迁移试验和数值模拟

Anchang Deng, Jun Zhu, Yunfeng Shi, Chao Chen, Tian Xie, Ting Li, A. Zhang
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摘要

核废料填埋场土壤中Sr-90的迁移数据将为填埋场的安全性评估和事故响应措施提供科学依据。想得到Sr-90的纵向(或横向)色散和配分系数等运移参数是准确预测Sr-90运移的关键。本文尝试采用试验与数值模拟相结合的方法估算变饱和土中Sr-90的迁移参数,并以山西粉质壤土中Sr-90的迁移为例进行了探讨。采用柱法进行Sr-90的迁移实验,入液水流量为375 mL/d,室温pH值为7左右。结果表明:Sr-90的中心流向迁移距离为3.9 cm,峰值浓度为1.04×104 Bq/cm3;根据Sr-90在土柱中的浓度分布,结合核素迁移三维数值模型(Hydrus-3d),拟合得到粉质壤土中的分配系数为79 ml/g,纵向弥散度为0.7 cm,横向弥散度为0.8 cm。该方法考虑了静态实验无法覆盖的固体孔隙率和水速度,同时得到了固体的纵向和横向分散度,使结果更符合实际情况。
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The migration experiment of Sr-90 in variable saturated soils and numerical simulation used Hydrus-3d
There is a scientific support that migration data of Sr-90 in the nuclear waste landfill soil will provide for safety estimation and accident response measures in landfill.In order to make a more accurate prediction of the migration of Sr-90, it is critical to get the migration parameters such as longitudinal (or transverse) dispersivity and partition coefficient. This article try to use a method for estimating the migration parameters of Sr-90 in variable saturated soils combining experiment and numerical simulation, then explores the method with the migration of Sr-90 in silty loam in Shanxi province as an example. The migration experiment of Sr-90 was carried by column method , the water flow in is 375 mL/d, the pH value was about 7 at room temperature. The results show that the migration distance of central flow direction for Sr-90 is 3.9 cm and the peak concentration is 1.04×104 Bq/cm3. According to the concentration distribution of Sr-90 in the soil column combined with three-dimensional numerical model of nuclide migration (Hydrus-3d), the partition coefficient in the silty loam is 79 ml/g while the longitudinal dispersivity is 0.7 cm and the transverse dispersivity is 0.8 cm by fitting. This method takes the porosity and water velocity of solid into consideration that static experiments fail to cover and obtains the longitudinal and transverse dispersivity at the same time, which making the results more tally with the actual situation.
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