基于AIRS数据的东北多年冻土区甲烷柱浓度时空分布及排放源分析

Zhichao Xu, Yunshan Chen, W. Shan, Yuexing Wu
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摘要

东北地区是中国高纬多年冻土带分布面积最大的地区。随着全球变暖的加剧,多年冻土中储存的碳将逐渐解冻,以甲烷气体的形式释放到空气中,从而增加了近地面对流层的甲烷柱浓度。然而,目前对流层近地表甲烷柱浓度的时空分布和排放源尚不清楚。本文利用Aqua卫星AIRS (Atmospheric Infrared Sounder)遥感数据,分析了2003 - 2021年东北地区近地面对流层甲烷柱浓度的分布和变化趋势,并结合国家气象和野外监测资料,研究了东北多年冻土区地表甲烷的排放机理和排放源。研究结果表明:东北地区多年冻土带具有较高的四季甲烷排放能力,甲烷柱浓度呈显著的双峰季节变化;第一个高峰出现在夏季(6 ~ 8月),8月出现最大值;第二个高峰出现在冬季(12 ~ 2月),12月出现最大值。东北地区近地表甲烷柱浓度的平均增长率最大出现在春季(5.378ppbv/a),这是由于多年冻土下储存的碳逐渐以甲烷的形式暴露释放所致。排放源包括微生物作用、湿地地下水输送的甲烷、冰冻层储存的地质甲烷(亚稳态甲烷水合物、稳态甲烷水合物和地下深层或煤层产热源甲烷)。该研究为东北多年冻土区碳排放估算提供了数据和技术支持。
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Analysis of spatiotemporal distribution of methane column concentration and emission source in permafrost area of Northeast China based on AIRS data
Northeast China has the largest high-latitude permafrost distribution zone in China. With the intensification of global warming, the carbon stored in the permafrost will gradually thaw and release in the form of methane gas to air, thus increasing the methane column concentration in the near-surface troposphere. However, at present, the spatiotemporal distribution and emission source of methane column concentration in the near-surface troposphere are not clear. In this paper, using the AIRS (Atmospheric Infrared Sounder) remote sensing data from Aqua satellite, we analyzed the distribution and change trend of the methane column concentration in the near-surface troposphere in Northeast China from 2003 to 2021, and combined with the national meteorological and field monitoring data, we studied the emission mechanism and emission source of surface methane in the permafrost area of Northeast China. Study results show that: the permafrost zone in Northeast China has a high methane emission capacity in four seasons, and the methane column concentration shows a significant double-peak seasonal variation. The first peak appears in summer (June to August) and the maximum appears in August, the second peak appears in winter (December to February) and the maximum appears in December. However, the maximum average growth rate of near-surface methane column concentration in Northeast China appeared in spring (5.378ppbv/a), the reason is that the carbon stored under the permafrost is gradually exposed and released in the form of methane. The emission sources include microbial action, methane transported by wetland groundwater, geological methane (metastable methane hydrate, steady-state methane hydrate and thermogenic methane produced in the deep underground or coal seams) stored in frozen layer. The study provide data and technical support for the estimation of carbon emissions in permafrost areas in Northeast China.
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