光谱学

IF 19 1区 物理与天体物理 Q1 PHYSICS, MULTIDISCIPLINARY Reports on Progress in Physics Pub Date : 2020-04-18 DOI:10.1088/0034-4885/1/1/306
R. Schlögl, Y. Joseph
{"title":"光谱学","authors":"R. Schlögl, Y. Joseph","doi":"10.1088/0034-4885/1/1/306","DOIUrl":null,"url":null,"abstract":"We introduce the notion, and develop the theory of local-noise spectroscopy (LNS) - a tool to study the properties of systems far from equilibrium by means of flux density correlations. As a test bed, we apply it to biased molecular junctions. This tool naturally extends those based on local fluxes, while providing complementary information on the system. As examples of the rich phenomenology that one can study with this approach, we show that LNS can be used to yield information on microscopic properties of bias-induced light emission in junctions, provide local resolution of intra-system interactions, and employed as a nano-thermometry tool. Although LNS may, at the moment, be difficult to realize experimentally, it can nonetheless be used as a powerful theoretical tool to infer a wide range of physical properties on a variety of systems of present interest.","PeriodicalId":21110,"journal":{"name":"Reports on Progress in Physics","volume":"17 1","pages":"102 - 130"},"PeriodicalIF":19.0000,"publicationDate":"2020-04-18","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"406","resultStr":"{\"title\":\"Spectroscopy\",\"authors\":\"R. Schlögl, Y. Joseph\",\"doi\":\"10.1088/0034-4885/1/1/306\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"We introduce the notion, and develop the theory of local-noise spectroscopy (LNS) - a tool to study the properties of systems far from equilibrium by means of flux density correlations. As a test bed, we apply it to biased molecular junctions. This tool naturally extends those based on local fluxes, while providing complementary information on the system. As examples of the rich phenomenology that one can study with this approach, we show that LNS can be used to yield information on microscopic properties of bias-induced light emission in junctions, provide local resolution of intra-system interactions, and employed as a nano-thermometry tool. Although LNS may, at the moment, be difficult to realize experimentally, it can nonetheless be used as a powerful theoretical tool to infer a wide range of physical properties on a variety of systems of present interest.\",\"PeriodicalId\":21110,\"journal\":{\"name\":\"Reports on Progress in Physics\",\"volume\":\"17 1\",\"pages\":\"102 - 130\"},\"PeriodicalIF\":19.0000,\"publicationDate\":\"2020-04-18\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"406\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Reports on Progress in Physics\",\"FirstCategoryId\":\"101\",\"ListUrlMain\":\"https://doi.org/10.1088/0034-4885/1/1/306\",\"RegionNum\":1,\"RegionCategory\":\"物理与天体物理\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q1\",\"JCRName\":\"PHYSICS, MULTIDISCIPLINARY\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Reports on Progress in Physics","FirstCategoryId":"101","ListUrlMain":"https://doi.org/10.1088/0034-4885/1/1/306","RegionNum":1,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"PHYSICS, MULTIDISCIPLINARY","Score":null,"Total":0}
引用次数: 406

摘要

我们引入了局域噪声谱的概念,并发展了局域噪声谱(LNS)理论,这是一种利用通量密度相关来研究远离平衡态的系统特性的工具。作为测试平台,我们将其应用于偏置分子结。这个工具自然地扩展了那些基于局部通量的工具,同时提供了关于系统的补充信息。作为可以用这种方法研究的丰富现象学的例子,我们表明LNS可以用来获得结中偏置引起的光发射的微观特性的信息,提供系统内相互作用的局部分辨率,并用作纳米测温工具。虽然LNS目前可能难以在实验上实现,但它仍然可以作为一种强大的理论工具来推断当前感兴趣的各种系统的广泛物理性质。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
查看原文
分享 分享
微信好友 朋友圈 QQ好友 复制链接
本刊更多论文
Spectroscopy
We introduce the notion, and develop the theory of local-noise spectroscopy (LNS) - a tool to study the properties of systems far from equilibrium by means of flux density correlations. As a test bed, we apply it to biased molecular junctions. This tool naturally extends those based on local fluxes, while providing complementary information on the system. As examples of the rich phenomenology that one can study with this approach, we show that LNS can be used to yield information on microscopic properties of bias-induced light emission in junctions, provide local resolution of intra-system interactions, and employed as a nano-thermometry tool. Although LNS may, at the moment, be difficult to realize experimentally, it can nonetheless be used as a powerful theoretical tool to infer a wide range of physical properties on a variety of systems of present interest.
求助全文
通过发布文献求助,成功后即可免费获取论文全文。 去求助
来源期刊
Reports on Progress in Physics
Reports on Progress in Physics 物理-物理:综合
CiteScore
31.90
自引率
0.00%
发文量
45
审稿时长
6-12 weeks
期刊介绍: Reports on Progress in Physics is a highly selective journal with a mission to publish ground-breaking new research and authoritative invited reviews of the highest quality and significance across all areas of physics and related areas. Articles must be essential reading for specialists, and likely to be of broader multidisciplinary interest with the expectation for long-term scientific impact and influence on the current state and/or future direction of a field.
期刊最新文献
Key Issues Review: Useful autonomous quantum machines. Recent developments in tornado theory and observations. A comprehensive review of quantum machine learning: from NISQ to fault tolerance. Physics and technology of Laser Lightning Control. Realization of chiral two-mode Lipkin-Meshkov-Glick models via acoustics.
×
引用
GB/T 7714-2015
复制
MLA
复制
APA
复制
导出至
BibTeX EndNote RefMan NoteFirst NoteExpress
×
×
提示
您的信息不完整,为了账户安全,请先补充。
现在去补充
×
提示
您因"违规操作"
具体请查看互助需知
我知道了
×
提示
现在去查看 取消
×
提示
确定
0
微信
客服QQ
Book学术公众号 扫码关注我们
反馈
×
意见反馈
请填写您的意见或建议
请填写您的手机或邮箱
已复制链接
已复制链接
快去分享给好友吧!
我知道了
×
扫码分享
扫码分享
Book学术官方微信
Book学术文献互助
Book学术文献互助群
群 号:481959085
Book学术
文献互助 智能选刊 最新文献 互助须知 联系我们:info@booksci.cn
Book学术提供免费学术资源搜索服务,方便国内外学者检索中英文文献。致力于提供最便捷和优质的服务体验。
Copyright © 2023 Book学术 All rights reserved.
ghs 京公网安备 11010802042870号 京ICP备2023020795号-1