Near Field Radiative Heat Transfer in a Chain of Metallic Particles

Minggang Luo, Junming Zhao, L. Liu
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Abstract

Heat transport mediated by near-field interaction in particulate system (e.g. chain of particles) is one of the research focuses in thermal transport in micro-nanoscale. Near field radiative heat transfer (NFRHT) characteristics of metallic nanoparticle chains (separation distance between neighboring particles is h) are analyzed by means of both coupled electric-magnetic dipole approximation and quadrupole approximation. Thermal conductance (G) between the central particle and other particle with different separation gaps (Δx) is calculated at both 300K and 1200K. Corrected polarizability is used to take quadrupole effect into consideration when calculating the NFRHT in extreme near field where dipole approximation ceases to be valid. Temperature distributions along several different chains of particles due to NFRHT are also predicted. Results show that, according to the asymptotic behavior of distribution of G along metallic chains similar as that observed in SiC chains, heat super-diffusion is demonstrated at both 300K and 1200K in metallic nanoparticle chains. At 300K, the contribution of quadrupole results in that thermal conductance responses to h in different way in metallic and dielectric particle chains. Temperature distribution and heat flow are the two key parameters used to characterize the heat transport in chains of particles. Ag particles in SiC chain act as barriers during the radiative heat transport process. Heat super-diffusion, as well as some other characteristics of NFRHT, observed in metallic nanoparticle chains may help for insight of heat transport in particulate system and new design of device in micro-nanoscale.
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金属颗粒链中的近场辐射传热
颗粒系统(如颗粒链)中近场相互作用介导的热传递是微纳尺度热传递研究的热点之一。采用耦合电-磁偶极近似和四极近似分析了金属纳米颗粒链(相邻颗粒之间的分离距离为h)的近场辐射传热特性。在300K和1200K时,计算中心粒子与其他不同分离间隙粒子(Δx)之间的热导率(G)。在偶极子近似失效的极近场计算中,采用校正极化率来考虑四极子效应。还预测了几种不同颗粒链的温度分布。结果表明,金属纳米颗粒链在300K和1200K温度下均表现出热超扩散,G沿金属链的分布与SiC链相似。在300K时,四极子的贡献导致金属和介电粒子链的热导率对h的响应方式不同。温度分布和热流是表征颗粒链中热传递的两个关键参数。碳化硅链中的银粒子在辐射热传递过程中起屏障作用。在金属纳米颗粒链中观察到的热超扩散以及NFRHT的其他一些特性,有助于在微纳尺度上了解颗粒系统的热传递和新器件的设计。
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