Chirped Pulses Meet Quantum Dots: Innovations, Challenges, and Future Perspectives

Florian Kappe, Yusuf Karli, Grant Wilbur, Ria G. Krämer, Sayan Ghosh, René Schwarz, Moritz Kaiser, Thomas K. Bracht, Doris E. Reiter, Stefan Nolte, Kimberley C. Hall, Gregor Weihs, Vikas Remesh
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Abstract

Shaped laser pulses have been remarkably effective in investigating various aspects of light–matter interactions spanning a broad range of research. Chirped laser pulses exhibiting a time-varying frequency, or quadratic spectral phase, form a crucial category in the group of shaped laser pulses. This type of pulses have made a ubiquitous presence from spectroscopic applications to developments in high-power laser technology, and from nanophotonics to quantum optical communication, ever since their introduction. In the case of quantum technologies recently, substantial efforts are being invested toward achieving a truly scalable architecture. Concurrently, it is important to develop methods to produce robust photon sources. In this context, semiconductor quantum dots hold great potential, due to their exceptional photophysical properties and on-demand operating nature. Concerning the scalability aspect of semiconductor quantum dots, it is advantageous to develop a simple, yet robust method to generate photon states from it. Chirped pulse excitation has been widely demonstrated as a robust and efficient state preparation scheme in quantum dots, thereby boosting its applicability as a stable photon source in a real-world scenario. Despite the rapid growth and advancements in laser technologies, the generation and control of chirped laser pulses can be demanding. Here, an overview of a selected few approaches is presented to tailor and characterize chirped pulses for the efficient excitation of a quantum dot source. By taking the chirped-pulse-induced adiabatic rapid passage process in quantum dot as an example, numerical design examples are presented along with experimental advantages and challenges in each method and conclude with an outlook on future perspectives.

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啁啾脉冲与量子点:创新、挑战与未来展望
异形激光脉冲在研究光与物质相互作用的各个方面有着显著的效果,其研究范围十分广泛。啁啾激光脉冲具有时变频率或二次光谱相位,是异形激光脉冲中的一个重要类别。自问世以来,从光谱应用到高功率激光技术的发展,从纳米光子学到量子光通信,这类脉冲无处不在。就量子技术而言,最近正在投入大量精力,以实现真正可扩展的架构。与此同时,重要的是要开发出生产稳健光子源的方法。在这种情况下,半导体量子点因其卓越的光物理特性和按需运行的性质而具有巨大的潜力。考虑到半导体量子点的可扩展性,开发一种简单而稳健的方法来生成光子态是非常有利的。啁啾脉冲激发已被广泛证明是量子点中一种稳健高效的状态制备方案,从而提高了其作为稳定光子源在现实世界中的适用性。尽管激光技术发展迅速、日新月异,但啁啾激光脉冲的产生和控制仍然要求很高。在此,我们将概述几种精选的方法,以定制和表征用于量子点源高效激发的啁啾脉冲。以量子点中啁啾脉冲诱导的绝热快速通过过程为例,介绍了数值设计实例以及每种方法的实验优势和挑战,最后对未来前景进行了展望。
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