{"title":"Magnetic Field Enabled Ultrahigh-Rate Zn Metal Anodes","authors":"Yizhou Wang, Chen Liu, Jianyu Chen, Tianchao Guo, Zhengnan Tian, Zhiming Zhao, Yunpei Zhu, Xixiang Zhang, Jin Zhao, Yanwen Ma, Husam N. Alshareef","doi":"10.1016/j.mtener.2024.101509","DOIUrl":null,"url":null,"abstract":"<p>Aqueous Zn-based flow batteries receive tremendous attention toward future grid-scale energy storage, but the uncontrollable dendrite growth and limited plating current density at the Zn anode severely hinder their application prospects. Herein, we realize non-dendritic Zn growth at an ultrahigh current density of 100 mA cm<sup>-2</sup> via the application of an external magnetic field. Through in-situ observation, morphology characterization, and electrochemical performance explorations, we find that the magnetic field can effectively inhibit the savage growth of dendrites. We believe this work can provide new inspiration for high-rate Zn metal anode research and promote the future applications of Zn-based flow batteries.</p>","PeriodicalId":18277,"journal":{"name":"Materials Today Energy","volume":"198 1","pages":""},"PeriodicalIF":9.0000,"publicationDate":"2024-01-24","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":null,"platform":"Semanticscholar","paperid":null,"PeriodicalName":"Materials Today Energy","FirstCategoryId":"88","ListUrlMain":"https://doi.org/10.1016/j.mtener.2024.101509","RegionNum":2,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"CHEMISTRY, PHYSICAL","Score":null,"Total":0}
引用次数: 0
Abstract
Aqueous Zn-based flow batteries receive tremendous attention toward future grid-scale energy storage, but the uncontrollable dendrite growth and limited plating current density at the Zn anode severely hinder their application prospects. Herein, we realize non-dendritic Zn growth at an ultrahigh current density of 100 mA cm-2 via the application of an external magnetic field. Through in-situ observation, morphology characterization, and electrochemical performance explorations, we find that the magnetic field can effectively inhibit the savage growth of dendrites. We believe this work can provide new inspiration for high-rate Zn metal anode research and promote the future applications of Zn-based flow batteries.
基于锌的水基液流电池在未来电网规模的能源存储方面受到极大关注，但锌阳极不可控的枝晶生长和有限的电镀电流密度严重阻碍了其应用前景。在本文中，我们通过施加外部磁场，在 100 mA cm-2 的超高电流密度下实现了非树枝状锌生长。通过原位观察、形态表征和电化学性能探索，我们发现磁场能有效抑制树枝状的野蛮生长。我们相信这项工作能为高倍率锌金属阳极的研究提供新的启发，并促进锌基液流电池的未来应用。
期刊介绍：
Materials Today Energy is a multi-disciplinary, rapid-publication journal focused on all aspects of materials for energy.
Materials Today Energy provides a forum for the discussion of high quality research that is helping define the inclusive, growing field of energy materials.
Part of the Materials Today family, Materials Today Energy offers authors rigorous peer review, rapid decisions, and high visibility. The editors welcome comprehensive articles, short communications and reviews on both theoretical and experimental work in relation to energy harvesting, conversion, storage and distribution, on topics including but not limited to:
-Solar energy conversion
-Hydrogen generation
-Photocatalysis
-Thermoelectric materials and devices
-Materials for nuclear energy applications
-Materials for Energy Storage
-Environment protection
-Sustainable and green materials
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