Biopolymer‐based gel electrolytes for electrochemical energy Storage: Advances and prospects

IF 33.6 1区材料科学 Q1 MATERIALS SCIENCE, MULTIDISCIPLINARY Progress in Materials Science Pub Date : 2024-02-28 DOI:10.1016/j.pmatsci.2024.101264

Wu Yang , Wang Yang , Jiaming Zeng , Yuling Chen , Yongfa Huang , Juan Liu , Jianyun Gan , Tingzhen Li , Hao Zhang , Linxin Zhong , Xinwen Peng

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Abstract

With the rapid development of wearable electronics, safety hazards and operational stability have drawn widespread attention in recent years. Biopolymers with low cost, eco‐friendly and biocompatibility are competitive candidates to replace traditional petroleum‐based materials in constructing gel polymer electrolytes. Biopolymer-based gel electrolytes (BGPEs) have exhibited broad application prospects through suitable structural designs and functionalization in flexible and smart electrochemical energy storage devices. This review summarized the recent advances of BGPEs with characteristic physicochemical properties and smart functionalities for application in electrochemical energy storage devices. The crosslinking methods and performance validation of BGPEs are also comprehensively reviewed and analyzed. Significantly, the functionalized BGPEs with self‐healing, stretchability, and thermotolerant abilities are emphasized. Finally, the remaining challenges and future directions of BGPEs for application in advanced electrochemical energy storage devices are outlined to provide guidance for their further development.

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用于电化学储能的生物聚合物凝胶电解质：进展与前景

近年来，随着可穿戴电子设备的快速发展，其安全隐患和运行稳定性引起了广泛关注。生物聚合物具有成本低、生态友好和生物相容性等特点，是替代传统石油基材料构建凝胶聚合物电解质的有力候选材料。基于生物聚合物的凝胶电解质（BGPEs）通过适当的结构设计和功能化，在柔性和智能电化学储能装置中展现出广阔的应用前景。本综述总结了具有特色理化特性和智能功能的生物聚合物基凝胶电解质在电化学储能装置中应用的最新进展。此外，还全面综述和分析了 BGPE 的交联方法和性能验证。特别强调了具有自愈、拉伸和耐热能力的功能化 BGPE。最后，概述了 BGPE 在先进电化学储能设备中应用所面临的挑战和未来发展方向，为其进一步发展提供指导。

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来源期刊

Progress in Materials Science 工程技术-材料科学：综合

CiteScore

59.60

自引率

0.80%

发文量

101

审稿时长

11.4 months

期刊介绍： Progress in Materials Science is a journal that publishes authoritative and critical reviews of recent advances in the science of materials. The focus of the journal is on the fundamental aspects of materials science, particularly those concerning microstructure and nanostructure and their relationship to properties. Emphasis is also placed on the thermodynamics, kinetics, mechanisms, and modeling of processes within materials, as well as the understanding of material properties in engineering and other applications. The journal welcomes reviews from authors who are active leaders in the field of materials science and have a strong scientific track record. Materials of interest include metallic, ceramic, polymeric, biological, medical, and composite materials in all forms. Manuscripts submitted to Progress in Materials Science are generally longer than those found in other research journals. While the focus is on invited reviews, interested authors may submit a proposal for consideration. Non-invited manuscripts are required to be preceded by the submission of a proposal. Authors publishing in Progress in Materials Science have the option to publish their research via subscription or open access. Open access publication requires the author or research funder to meet a publication fee (APC). Abstracting and indexing services for Progress in Materials Science include Current Contents, Science Citation Index Expanded, Materials Science Citation Index, Chemical Abstracts, Engineering Index, INSPEC, and Scopus.