Epitaxial tantalum‐doped β‐Ga2O3 thin films grown on MgO (001) substrate by pulsed laser deposition

IF 2.5 4区 物理与天体物理 Q3 MATERIALS SCIENCE, MULTIDISCIPLINARY Physica Status Solidi-Rapid Research Letters Pub Date : 2024-03-02 DOI:10.1002/pssr.202400023
Haobo Lin, Ningtao Liu, Wei Wang, Xiaoli Zhang, Dongyang Han, Wenrui Zhang, Jichun Ye
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Abstract

Epitaxial thin films of tantalum‐doped β‐Ga2O3 (Ta‐Ga2O3) were grown on MgO (001) substrates to study the effect of Ta doping on the electrical properties of β‐Ga2O3 films. X‐ray diffraction measurements show that the films with different Ta doping concentrations are (00l)‐oriented single‐crystalline β‐Ga2O3 without impurity phases. The incorporation of the Ta element modifies the electrical properties of Ta‐Ga2O3 films significantly. At a very low doping ratio of 0.05 mol%, the Ta‐Ga2O3 film showed a minimum resistivity of 2.32 Ω·cm and a carrier concentration of 2.48×1017 cm‐3. The corresponding activation energy of Ta element in the film was 16.8 meV, suggesting that the Ta element is a promising shallow donor dopant. The XPS analysis confirms that the Fermi level of the Ga2O3 films shifts towards the conduction band minimum after the introduction of Ta ions. These results indicate that the transition metal element Ta could be an effective n‐type dopant for modulating the carrier transport behavior of β‐Ga2O3 films.This article is protected by copyright. All rights reserved.
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利用脉冲激光沉积法在氧化镁(001)基底上生长的掺杂钽的外延β-Ga2O3 薄膜
在氧化镁(001)基底上生长了掺杂钽的β-Ga2O3(Ta-Ga2O3)外延薄膜,以研究掺杂Ta对β-Ga2O3薄膜电性能的影响。X 射线衍射测量结果表明,不同掺杂浓度 Ta 的薄膜都是取向 (00l) 的单晶 β-Ga2O3 ,没有杂质相。Ta元素的掺入极大地改变了Ta-Ga2O3薄膜的电学特性。在 0.05 摩尔%的极低掺杂率下,Ta-Ga2O3 薄膜的最小电阻率为 2.32 Ω-cm,载流子浓度为 2.48×1017 cm-3。薄膜中 Ta 元素的相应活化能为 16.8 meV,表明 Ta 元素是一种很有前途的浅供体掺杂剂。XPS 分析证实,在引入 Ta 离子后,Ga2O3 薄膜的费米级向导带最低点移动。这些结果表明,过渡金属元素 Ta 可以作为一种有效的 n 型掺杂剂来调节 β-Ga2O3 薄膜的载流子输运行为。本文受版权保护。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
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来源期刊
Physica Status Solidi-Rapid Research Letters
Physica Status Solidi-Rapid Research Letters 物理-材料科学:综合
CiteScore
5.20
自引率
3.60%
发文量
208
审稿时长
1.4 months
期刊介绍: Physica status solidi (RRL) - Rapid Research Letters was designed to offer extremely fast publication times and is currently one of the fastest double peer-reviewed publication media in solid state and materials physics. Average times are 11 days from submission to first editorial decision, and 12 days from acceptance to online publication. It communicates important findings with a high degree of novelty and need for express publication, as well as other results of immediate interest to the solid-state physics and materials science community. Published Letters require approval by at least two independent reviewers. The journal covers topics such as preparation, structure and simulation of advanced materials, theoretical and experimental investigations of the atomistic and electronic structure, optical, magnetic, superconducting, ferroelectric and other properties of solids, nanostructures and low-dimensional systems as well as device applications. Rapid Research Letters particularly invites papers from interdisciplinary and emerging new areas of research.
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