Contribution of individual sources of volatile organic compounds to their cancer and non-cancer risks in the multi-industrial city of Ulsan, South Korea

IF 2.9 4区 环境科学与生态学 Q3 ENVIRONMENTAL SCIENCES Air Quality Atmosphere and Health Pub Date : 2024-03-25 DOI:10.1007/s11869-024-01554-x
Seong-Joon Kim, Sang-Jin Lee, Hyunjoo Kim, Youwei Hong, Sung-Deuk Choi
{"title":"Contribution of individual sources of volatile organic compounds to their cancer and non-cancer risks in the multi-industrial city of Ulsan, South Korea","authors":"Seong-Joon Kim,&nbsp;Sang-Jin Lee,&nbsp;Hyunjoo Kim,&nbsp;Youwei Hong,&nbsp;Sung-Deuk Choi","doi":"10.1007/s11869-024-01554-x","DOIUrl":null,"url":null,"abstract":"<div><p>Previous studies have investigated the major sources and health risks associated with atmospheric volatile organic compounds (VOCs). However, the spatial variability of the impact of their emission sources on health risks has rarely been studied. In this study, passive air sampling of VOCs was conducted at 24 sites in Ulsan, the largest industrial city in South Korea. Toluene exhibited the highest time-averaged concentration (6.37 µg/m<sup>3</sup>), followed by m,p,o-xylenes (4.69 µg/m<sup>3</sup>), ethyl acetate (3.26 µg/m<sup>3</sup>), and ethylbenzene (2.70 µg/m<sup>3</sup>). Higher concentrations of total (Σ<sub>59</sub>) VOCs and BTEX (benzene, toluene, ethylbenzene, and m,p,o-xylenes) were observed near industrial complexes. The mean cumulative (Σ<sub>11</sub>) cancer risk was 9.1E-6, with the highest contribution from benzene (4.7E-6), while the mean cumulative (Σ<sub>17</sub>) non-cancer risk was 2.6E-1, primarily driven by naphthalene (1.7E-1), suggesting the importance of carcinogenic VOCs. Five major sources were identified using the positive matrix factorization model, revealing the dominance of industrial activities. Both cancer and non-cancer risks were elevated in the petrochemical industrial complex, which is located close to densely populated areas. Consequently, prioritized management of VOC exposure to workers and residents is necessary for the petrochemical industrial complex and nearby residential areas.</p></div>","PeriodicalId":49109,"journal":{"name":"Air Quality Atmosphere and Health","volume":"17 9","pages":"1937 - 1949"},"PeriodicalIF":2.9000,"publicationDate":"2024-03-25","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":null,"platform":"Semanticscholar","paperid":null,"PeriodicalName":"Air Quality Atmosphere and Health","FirstCategoryId":"93","ListUrlMain":"https://link.springer.com/article/10.1007/s11869-024-01554-x","RegionNum":4,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q3","JCRName":"ENVIRONMENTAL SCIENCES","Score":null,"Total":0}
引用次数: 0

Abstract

Previous studies have investigated the major sources and health risks associated with atmospheric volatile organic compounds (VOCs). However, the spatial variability of the impact of their emission sources on health risks has rarely been studied. In this study, passive air sampling of VOCs was conducted at 24 sites in Ulsan, the largest industrial city in South Korea. Toluene exhibited the highest time-averaged concentration (6.37 µg/m3), followed by m,p,o-xylenes (4.69 µg/m3), ethyl acetate (3.26 µg/m3), and ethylbenzene (2.70 µg/m3). Higher concentrations of total (Σ59) VOCs and BTEX (benzene, toluene, ethylbenzene, and m,p,o-xylenes) were observed near industrial complexes. The mean cumulative (Σ11) cancer risk was 9.1E-6, with the highest contribution from benzene (4.7E-6), while the mean cumulative (Σ17) non-cancer risk was 2.6E-1, primarily driven by naphthalene (1.7E-1), suggesting the importance of carcinogenic VOCs. Five major sources were identified using the positive matrix factorization model, revealing the dominance of industrial activities. Both cancer and non-cancer risks were elevated in the petrochemical industrial complex, which is located close to densely populated areas. Consequently, prioritized management of VOC exposure to workers and residents is necessary for the petrochemical industrial complex and nearby residential areas.

查看原文
分享 分享
微信好友 朋友圈 QQ好友 复制链接
本刊更多论文
韩国蔚山多工业城市挥发性有机化合物的个别来源对其癌症和非癌症风险的影响
摘要 以前的研究调查了大气中挥发性有机化合物(VOCs)的主要来源和相关健康风险。然而,有关其排放源对健康风险影响的空间变化的研究却很少。本研究在韩国最大的工业城市蔚山的 24 个地点对挥发性有机化合物进行了被动空气采样。甲苯的时间平均浓度最高(6.37 微克/立方米),其次是间,对,邻二甲苯(4.69 微克/立方米)、乙酸乙酯(3.26 微克/立方米)和乙苯(2.70 微克/立方米)。在工业综合体附近观察到的总 (Σ59) 挥发性有机化合物和 BTEX(苯、甲苯、乙苯和 m,p,o-二甲苯)浓度较高。平均累积(Σ11)癌症风险为 9.1E-6,其中苯的贡献最大(4.7E-6),而平均累积(Σ17)非癌症风险为 2.6E-1,主要由萘驱动(1.7E-1),这表明了致癌挥发性有机化合物的重要性。利用正矩阵因式分解模型确定了五个主要来源,揭示了工业活动的主导地位。在靠近人口稠密地区的石化工业综合体中,癌症和非癌症风险都很高。因此,有必要对石化工业综合体和附近居民区的工人和居民接触挥发性有机化合物的情况进行优先管理。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
求助全文
约1分钟内获得全文 去求助
来源期刊
Air Quality Atmosphere and Health
Air Quality Atmosphere and Health ENVIRONMENTAL SCIENCES-
CiteScore
8.80
自引率
2.00%
发文量
146
审稿时长
>12 weeks
期刊介绍: Air Quality, Atmosphere, and Health is a multidisciplinary journal which, by its very name, illustrates the broad range of work it publishes and which focuses on atmospheric consequences of human activities and their implications for human and ecological health. It offers research papers, critical literature reviews and commentaries, as well as special issues devoted to topical subjects or themes. International in scope, the journal presents papers that inform and stimulate a global readership, as the topic addressed are global in their import. Consequently, we do not encourage submission of papers involving local data that relate to local problems. Unless they demonstrate wide applicability, these are better submitted to national or regional journals. Air Quality, Atmosphere & Health addresses such topics as acid precipitation; airborne particulate matter; air quality monitoring and management; exposure assessment; risk assessment; indoor air quality; atmospheric chemistry; atmospheric modeling and prediction; air pollution climatology; climate change and air quality; air pollution measurement; atmospheric impact assessment; forest-fire emissions; atmospheric science; greenhouse gases; health and ecological effects; clean air technology; regional and global change and satellite measurements. This journal benefits a diverse audience of researchers, public health officials and policy makers addressing problems that call for solutions based in evidence from atmospheric and exposure assessment scientists, epidemiologists, and risk assessors. Publication in the journal affords the opportunity to reach beyond defined disciplinary niches to this broader readership.
期刊最新文献
AIRQ HARMO21 special issue—PREFACE Long-term changes of surface ozone and ozone sensitivity over the North China Plain based on 2015–2021 satellite retrievals Developing a novel hybrid model based on deep neural networks and discrete wavelet transform algorithm for prediction of daily air temperature The impact of respirable dust exposure on lung function parameters of motorcycle taxi drivers in Bangkok and adjacent provinces, Thailand Ozone production sensitivity in the highland city of Lhasa: a comparative analysis with Beijing
×
引用
GB/T 7714-2015
复制
MLA
复制
APA
复制
导出至
BibTeX EndNote RefMan NoteFirst NoteExpress
×
×
提示
您的信息不完整,为了账户安全,请先补充。
现在去补充
×
提示
您因"违规操作"
具体请查看互助需知
我知道了
×
提示
现在去查看 取消
×
提示
确定
0
微信
客服QQ
Book学术公众号 扫码关注我们
反馈
×
意见反馈
请填写您的意见或建议
请填写您的手机或邮箱
已复制链接
已复制链接
快去分享给好友吧!
我知道了
×
扫码分享
扫码分享
Book学术官方微信
Book学术文献互助
Book学术文献互助群
群 号:481959085
Book学术
文献互助 智能选刊 最新文献 互助须知 联系我们:info@booksci.cn
Book学术提供免费学术资源搜索服务,方便国内外学者检索中英文文献。致力于提供最便捷和优质的服务体验。
Copyright © 2023 Book学术 All rights reserved.
ghs 京公网安备 11010802042870号 京ICP备2023020795号-1