Characterisation of sealed radioactive source for nuclear forensic purposes

Z. Laili, Hishamudin Husin, Ahmad Hasnulhadi Che Kamaruddin, Muhamad Azfar Azman, Wilfred Sylvester Paulus, Nadira Kamarudin
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Abstract

A study characterized sealed radioactive sources (60Co, 137Cs, and 241Am) for nuclear forensic analysis, focusing on their physical, macroscopic, and radiological properties. Results revealed specific features, such as stamped or engraved information, that served as valuable signatures for nuclear forensic investigation. Corrosion observations provide valuable insights into the condition of the source and historical context. Gamma-ray spectra analysis revealed clear distinctions, including a scattering peak in cylindrical 60Co and 137Cs disk sources (200-500 keV), which was absent in the cup-style 241Am source. Unusual peaks in the gamma spectra of 60Co, 137Cs, and 241Am sources suggested potential impurities or background radiation. This was indicated by non-Gaussian shapes and significant counts per second at specific energy levels. X-ray radiography effectively highlights nuclear material characteristics, emphasizing density, uniformity, and internal structure. This analysis contributed to the development of a National Nuclear Forensic Library (NNFL) and enhanced Malaysia’s capability in nuclear forensic investigations related to radioactive sources found outside regulatory control.
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用于核鉴识目的的密封放射源的特征描述
一项研究描述了用于核鉴识分析的密封放射源(60Co、137Cs 和 241Am)的特征,重点关注其物理、宏观和放射性特性。研究结果揭示了一些特定特征,如印记或刻印信息,这些特征是核鉴识调查的宝贵标志。对腐蚀情况的观察为了解源的状况和历史背景提供了宝贵的信息。伽马射线光谱分析显示了明显的区别,包括圆柱形 60Co 和 137Cs 盘源(200-500keV)中的散射峰,而杯状 241Am 源中没有这种散射峰。60钴、137Cs和241Am源伽马能谱中的异常峰表明可能存在杂质或本底辐射。这表现为非高斯形状和特定能级上每秒大量的计数。X 射线射线照相术有效地突出了核材料的特征,强调了密度、均匀性和内部结构。这项分析有助于国家核鉴识图书馆(NNFL)的发展,并提高了马来西亚对在监管控制之外发现的放射源进行核鉴识调查的能力。
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