Conductive PEDOT-Dominant Surface of Transparent Electrode Patch via Selective Phase Transfer for Efficient Flexible Photoelectronic Devices.

IF 8.3 2区 材料科学 Q1 MATERIALS SCIENCE, MULTIDISCIPLINARY ACS Applied Materials & Interfaces Pub Date : 2024-07-24 Epub Date: 2024-07-11 DOI:10.1021/acsami.4c07526
Junmin Lee, Min Soo Kim, Woongsik Jang, Dong Hwan Wang
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Abstract

In this study, a conductive patch for a flexible organic optoelectronic device is proposed and implemented using a poly(3,4-ethylenedioxythiophene):polystyrenesulfonate (PEDOT:PSS) polymer electrode based on a transfer process to achieve its high conductivity with an efficient conductive pathway. This PEDOT-dominant surface is induced by phase inversion during the transfer process owing to the solvent affinity of the PSS phase. The PEDOT:PSS patch formed by the transfer process minimizes the power loss in a flexible optoelectronic device due to the improved charge collection and suppressed leakage current responses. In addition, the bending stability of the flexible photoelectronic device is also enhanced by maintaining performance for 1000 bending cycles. Therefore, in the fabrication of a transparent flexible conductive PEDOT:PSS patch, the transfer process of a conducting polymer constitutes an effective strategy that can improve conductivity and embellished morphology.

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通过选择性相转移实现透明电极贴片的导电 PEDOT 主导表面,从而实现高效柔性光电子器件。
本研究提出了一种用于柔性有机光电器件的导电贴片,该贴片采用聚(3,4-亚乙二氧基噻吩):聚苯乙烯磺酸盐(PEDOT:PSS)聚合物电极,基于转移过程实现其高效导电途径的高导电性。由于 PSS 相的溶剂亲和性,这种 PEDOT 主导表面是在转移过程中通过相反转诱发的。通过转移过程形成的 PEDOT:PSS 贴片可改善电荷收集并抑制漏电流反应,从而最大限度地降低柔性光电器件的功率损耗。此外,柔性光电器件的弯曲稳定性也得到了提高,可在 1000 次弯曲循环中保持性能不变。因此,在制造透明柔性导电 PEDOT:PSS 贴片时,导电聚合物的转移过程是一种有效的策略,可以提高导电性和美化形态。
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来源期刊
ACS Applied Materials & Interfaces
ACS Applied Materials & Interfaces 工程技术-材料科学:综合
CiteScore
16.00
自引率
6.30%
发文量
4978
审稿时长
1.8 months
期刊介绍: ACS Applied Materials & Interfaces is a leading interdisciplinary journal that brings together chemists, engineers, physicists, and biologists to explore the development and utilization of newly-discovered materials and interfacial processes for specific applications. Our journal has experienced remarkable growth since its establishment in 2009, both in terms of the number of articles published and the impact of the research showcased. We are proud to foster a truly global community, with the majority of published articles originating from outside the United States, reflecting the rapid growth of applied research worldwide.
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