Gas migration at the granite–bentonite interface under semirigid boundary conditions in the context of high‐level radioactive waste disposal

Jiangfeng Liu, Zhipeng Wang, Jingna Guo, A. Jivkov, Majid Sedighi, Jianfu Shao
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Abstract

The corrosion of waste canisters in the deep geological disposal facilities (GDFs) for high‐level radioactive waste (HLRW) can generate gas, which escapes from the engineered barrier system through the interfaces between the bentonite buffer blocks and the host rock and those between the bentonite blocks. In this study, a series of water infiltration and gas breakthrough experiments were conducted on granite and on granite–bentonite specimens with smooth and grooved interfaces. On this basis, this study presents new insights and a quantitative assessment of the impact of the interface between clay and host rock on gas transport. As the results show, the water permeability values from water infiltration tests on granite and granite–bentonite samples (10−19–10−20 m2) are found to be slightly higher than that of bentonite. The gas permeability of the mock‐up samples with smooth interfaces is one order of magnitude larger than that of the mock‐up with grooved interfaces. The gas results of breakthrough pressures for the granite and the granite–bentonite mock‐up samples are significantly lower than that of bentonite. The results highlight the potential existence of preferential gas migration channels between the rock and bentonite buffer that require further considerations in safety assessment.
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高放射性废物处置背景下半刚性边界条件下花岗岩-膨润土界面的气体迁移
高放射性废物(HLRW)深层地质处置设施(GDFs)中的废物罐腐蚀会产生气体,这些气体会通过膨润土缓冲块与主岩之间的界面以及膨润土块之间的界面从工程屏障系统中逸出。本研究在花岗岩以及界面光滑和开槽的花岗岩-膨润土试样上进行了一系列水渗透和气体突破实验。在此基础上,本研究对粘土和主岩之间的界面对气体输送的影响提出了新的见解和定量评估。结果表明,花岗岩和花岗膨润土样品(10-19-10-20 m2)的渗水试验得出的透水率值略高于膨润土。界面光滑的模拟样品的气体渗透率比界面有凹槽的模拟样品大一个数量级。花岗岩和花岗岩-膨润土模拟样品的气体突破压力结果明显低于膨润土。这些结果突出表明,岩石和膨润土缓冲区之间可能存在优先气体迁移通道,需要在安全评估中进一步考虑。
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