Carbon Dioxide Capture and Conversion Using Metal-Organic Framework (MOF) Materials: A Comprehensive Review.

IF 4.4 3区 材料科学 Q2 CHEMISTRY, MULTIDISCIPLINARY Nanomaterials Pub Date : 2024-08-12 DOI:10.3390/nano14161340
Fanyi Kong, Wenqian Chen
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Abstract

The escalating threat of anthropogenic climate change has spurred an urgent quest for innovative CO2 capture and utilization (CCU) technologies. Metal-organic frameworks (MOFs) have emerged as prominent candidates in CO2 capture and conversion due to their large specific surface area, well-defined porous structure, and tunable chemical properties. This review unveils the latest advancements in MOF-based materials specifically designed for superior CO2 adsorption, precise separation, advanced photocatalytic and electrocatalytic CO2 reduction, progressive CO2 hydrogenation, and dual functionalities. We explore the strategies that enhance MOF efficiency and examine the challenges of and opportunities afforded by transitioning from laboratory research to industrial application. Looking ahead, this review offers a visionary perspective on harnessing MOFs for the sustainable capture and conversion of CO2.

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使用金属有机框架 (MOF) 材料捕获和转化二氧化碳:全面回顾。
人为气候变化的威胁不断升级,促使人们迫切寻求创新的二氧化碳捕获和利用(CCU)技术。金属有机框架(MOFs)因其较大的比表面积、明确的多孔结构和可调整的化学特性,已成为二氧化碳捕获和转化的主要候选材料。本综述揭示了基于 MOF 的材料的最新进展,这些材料专为实现卓越的二氧化碳吸附、精确分离、先进的光催化和电催化二氧化碳还原、渐进式二氧化碳氢化和双重功能而设计。我们探讨了提高 MOF 效率的策略,并研究了从实验室研究过渡到工业应用所面临的挑战和带来的机遇。展望未来,本综述为利用 MOFs 实现二氧化碳的可持续捕获和转化提供了一个富有远见的视角。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
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来源期刊
Nanomaterials
Nanomaterials NANOSCIENCE & NANOTECHNOLOGY-MATERIALS SCIENCE, MULTIDISCIPLINARY
CiteScore
8.50
自引率
9.40%
发文量
3841
审稿时长
14.22 days
期刊介绍: Nanomaterials (ISSN 2076-4991) is an international and interdisciplinary scholarly open access journal. It publishes reviews, regular research papers, communications, and short notes that are relevant to any field of study that involves nanomaterials, with respect to their science and application. Thus, theoretical and experimental articles will be accepted, along with articles that deal with the synthesis and use of nanomaterials. Articles that synthesize information from multiple fields, and which place discoveries within a broader context, will be preferred. There is no restriction on the length of the papers. Our aim is to encourage scientists to publish their experimental and theoretical research in as much detail as possible. Full experimental or methodical details, or both, must be provided for research articles. Computed data or files regarding the full details of the experimental procedure, if unable to be published in a normal way, can be deposited as supplementary material. Nanomaterials is dedicated to a high scientific standard. All manuscripts undergo a rigorous reviewing process and decisions are based on the recommendations of independent reviewers.
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