Long-Range Non-Coulombic Coupling at the LaAlO3/SrTiO3 Interface

IF 4.3 3区 材料科学 Q2 CHEMISTRY, MULTIDISCIPLINARY Advanced Materials Interfaces Pub Date : 2024-08-13 DOI:10.1002/admi.202400223
Aditi Nethwewala, Kitae Eom, Muqing Yu, Ranjani Ramachandran, Chang-Beom Eom, Patrick Irvin, Jeremy Levy
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Abstract

The LaAlO3/SrTiO3 interface hosts a plethora of gate-tunable electronic phases. Gating of LaAlO3/SrTiO3 interfaces is usually assumed to occur electrostatically. However, increasing evidence suggests that non-local interactions can influence and, in some cases, dominate the coupling between applied gate voltages and electronic properties. Here, quasi-1D ballistic electron waveguides are sketched at the LaAlO3/SrTiO3 interface as a probe to understand how gate tunability varies as a function of spatial separation. Gate tunability measurements reveal the scaling law to be at odds with the pure electrostatic coupling observed in traditional semiconductor systems. The non-Coulombic gating at the interface is attributed to a long-range nanoelectromechanical coupling between the gate and electron waveguide, possibly mediated by the ferroelastic domains in SrTiO3. The long-range interactions at the LaAlO3/SrTiO3 interface add unexpected richness and complexity to this correlated electron system.

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LaAlO3/SrTiO3 界面的长程非库仑耦合
LaAlO3/SrTiO3 界面存在大量可门控调节的电子相。LaAlO3/SrTiO3 界面的门控通常被认为是静电发生的。然而,越来越多的证据表明,非局部相互作用会影响外加栅极电压与电子特性之间的耦合,并在某些情况下起主导作用。在此,我们在 LaAlO3/SrTiO3 界面上勾勒出准一维弹道电子波导,作为了解栅极可调谐性如何随空间隔离而变化的探针。栅极可调谐性测量结果表明,其缩放规律与传统半导体系统中观察到的纯静电耦合不一致。界面上的非库仑门控归因于栅极和电子波导之间的长程纳米机电耦合,这可能是由 SrTiO3 中的铁弹性域介导的。LaAlO3/SrTiO3 界面的长程相互作用为这一相关电子系统增添了意想不到的丰富性和复杂性。
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来源期刊
Advanced Materials Interfaces
Advanced Materials Interfaces CHEMISTRY, MULTIDISCIPLINARY-MATERIALS SCIENCE, MULTIDISCIPLINARY
CiteScore
8.40
自引率
5.60%
发文量
1174
审稿时长
1.3 months
期刊介绍: Advanced Materials Interfaces publishes top-level research on interface technologies and effects. Considering any interface formed between solids, liquids, and gases, the journal ensures an interdisciplinary blend of physics, chemistry, materials science, and life sciences. Advanced Materials Interfaces was launched in 2014 and received an Impact Factor of 4.834 in 2018. The scope of Advanced Materials Interfaces is dedicated to interfaces and surfaces that play an essential role in virtually all materials and devices. Physics, chemistry, materials science and life sciences blend to encourage new, cross-pollinating ideas, which will drive forward our understanding of the processes at the interface. Advanced Materials Interfaces covers all topics in interface-related research: Oil / water separation, Applications of nanostructured materials, 2D materials and heterostructures, Surfaces and interfaces in organic electronic devices, Catalysis and membranes, Self-assembly and nanopatterned surfaces, Composite and coating materials, Biointerfaces for technical and medical applications. Advanced Materials Interfaces provides a forum for topics on surface and interface science with a wide choice of formats: Reviews, Full Papers, and Communications, as well as Progress Reports and Research News.
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