Haoqiu Chen, Tingting Wang, Yanfen Sun, Zhiwei Chen, Juan Yuan, Lianxin Luo
{"title":"Study on the Improvement of the Degradation Efficiency of Methylene Blue Using Pulsed Direct-Current Self-Power Supply","authors":"Haoqiu Chen, Tingting Wang, Yanfen Sun, Zhiwei Chen, Juan Yuan, Lianxin Luo","doi":"10.1021/acs.langmuir.4c02576","DOIUrl":null,"url":null,"abstract":"Effective treatment of dye wastewater is currently a great concern and a research hotspot. Electrocatalysis has unique advantages in treating toxic and harmful refractory dye wastewater; however, it requires an external power supply, which increases energy consumption and cost. As a new energy collection technology, triboelectric nanogenerators (TENGs) have gained considerable attention. In this study, an origami multilayer spherical friction nanogenerator (Q-TENG) was developed for the removal of methylene blue (MB) from dye wastewater. The current and voltage output performances of Q-TENG were explored, and the removal and degradation mechanisms of MB were discussed. Results indicated that when the water wave acceleration <i>a</i> = 3 m/s<sup>2</sup>, the open-circuit voltage and short-circuit current reached the maximum values of 179 V and 9.4 μA, respectively. The self-powered catalytic degradation of MB using Q-TENG can produce more <sup>•</sup>OH and SO<sub>4</sub><sup>–•</sup>, and the free radicals increase with increasing action time of Q-TENG, thus increasing the degradation efficiency of MB. This study provides a new strategy for solving the problem of high energy consumption during electrochemical reactions in wastewater treatment.","PeriodicalId":50,"journal":{"name":"Langmuir","volume":null,"pages":null},"PeriodicalIF":3.7000,"publicationDate":"2024-09-18","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":null,"platform":"Semanticscholar","paperid":null,"PeriodicalName":"Langmuir","FirstCategoryId":"92","ListUrlMain":"https://doi.org/10.1021/acs.langmuir.4c02576","RegionNum":2,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q2","JCRName":"CHEMISTRY, MULTIDISCIPLINARY","Score":null,"Total":0}
引用次数: 0
Abstract
Effective treatment of dye wastewater is currently a great concern and a research hotspot. Electrocatalysis has unique advantages in treating toxic and harmful refractory dye wastewater; however, it requires an external power supply, which increases energy consumption and cost. As a new energy collection technology, triboelectric nanogenerators (TENGs) have gained considerable attention. In this study, an origami multilayer spherical friction nanogenerator (Q-TENG) was developed for the removal of methylene blue (MB) from dye wastewater. The current and voltage output performances of Q-TENG were explored, and the removal and degradation mechanisms of MB were discussed. Results indicated that when the water wave acceleration a = 3 m/s2, the open-circuit voltage and short-circuit current reached the maximum values of 179 V and 9.4 μA, respectively. The self-powered catalytic degradation of MB using Q-TENG can produce more •OH and SO4–•, and the free radicals increase with increasing action time of Q-TENG, thus increasing the degradation efficiency of MB. This study provides a new strategy for solving the problem of high energy consumption during electrochemical reactions in wastewater treatment.
期刊介绍:
Langmuir is an interdisciplinary journal publishing articles in the following subject categories:
Colloids: surfactants and self-assembly, dispersions, emulsions, foams
Interfaces: adsorption, reactions, films, forces
Biological Interfaces: biocolloids, biomolecular and biomimetic materials
Materials: nano- and mesostructured materials, polymers, gels, liquid crystals
Electrochemistry: interfacial charge transfer, charge transport, electrocatalysis, electrokinetic phenomena, bioelectrochemistry
Devices and Applications: sensors, fluidics, patterning, catalysis, photonic crystals
However, when high-impact, original work is submitted that does not fit within the above categories, decisions to accept or decline such papers will be based on one criteria: What Would Irving Do?
Langmuir ranks #2 in citations out of 136 journals in the category of Physical Chemistry with 113,157 total citations. The journal received an Impact Factor of 4.384*.
This journal is also indexed in the categories of Materials Science (ranked #1) and Multidisciplinary Chemistry (ranked #5).