Fusion mechanism involved in the synthesis of superheavy element Z>118 using Mn projectiles

{"title":"Fusion mechanism involved in the synthesis of superheavy element Z>118 using Mn projectiles","authors":"","doi":"10.1016/j.nucana.2024.100124","DOIUrl":null,"url":null,"abstract":"<div><div>We conducted an in-depth investigation of Mn-induced fusion reactions aimed at synthesizing superheavy elements with atomic numbers Z=119 to Z=123. Our analysis considers the total potential, which combines Coulomb and nuclear potentials. The nuclear potential was calculated using the Thomas–Fermi approach, a valuable method for modeling the behavior of nucleons in atomic nuclei. within the framework of advanced statistical model, the evaporation residue cross-sections were determined. At optimal energies, we have calculated capture, fusion, and evaporation residue cross-sections for the reactions of all the projectile–target combinations. All <span><math><msup><mrow></mrow><mrow><mn>53</mn><mo>−</mo><mn>55</mn></mrow></msup></math></span>Mn isotopes with larger half-lives were taken into consideration as projectiles. Fusion reactions between <span><math><msup><mrow></mrow><mrow><mn>53</mn><mo>−</mo><mn>55</mn></mrow></msup></math></span>Mn projectiles with <span><math><msup><mrow></mrow><mrow><mn>238</mn><mo>−</mo><mn>242</mn><mo>,</mo><mn>244</mn></mrow></msup></math></span>Pu, <span><math><msup><mrow></mrow><mrow><mn>241</mn><mo>−</mo><mn>243</mn></mrow></msup></math></span>Am, <span><math><msup><mrow></mrow><mrow><mn>242</mn><mo>−</mo><mn>248</mn><mo>,</mo><mn>250</mn></mrow></msup></math></span>Cm, <span><math><msup><mrow></mrow><mrow><mn>247</mn><mo>−</mo><mn>249</mn></mrow></msup></math></span>Bk, and <span><math><msup><mrow></mrow><mrow><mn>248</mn><mo>−</mo><mn>254</mn></mrow></msup></math></span>Cf. Detailed investigations were made and promising reactions viz. <span><math><mrow><msup><mrow></mrow><mrow><mn>241</mn></mrow></msup><mi>Pu</mi></mrow></math></span> (<span><math><mrow><msup><mrow></mrow><mrow><mn>55</mn></mrow></msup><mi>Mn</mi></mrow></math></span>, 3n)<sup>293</sup>119, <span><math><mrow><msup><mrow></mrow><mrow><mn>242</mn></mrow></msup><mi>Am</mi></mrow></math></span> (<span><math><mrow><msup><mrow></mrow><mrow><mn>55</mn></mrow></msup><mi>Mn</mi></mrow></math></span>, 3n)<sup>294</sup>120, <span><math><mrow><msup><mrow></mrow><mrow><mn>247</mn></mrow></msup><mi>Cm</mi></mrow></math></span> (<span><math><mrow><msup><mrow></mrow><mrow><mn>55</mn></mrow></msup><mi>Mn</mi></mrow></math></span>, 3n)<sup>299</sup>121, <span><math><mrow><msup><mrow></mrow><mrow><mn>248</mn></mrow></msup><mi>Bk</mi></mrow></math></span> (<span><math><mrow><msup><mrow></mrow><mrow><mn>55</mn></mrow></msup><mi>Mn</mi></mrow></math></span>, 3n)<sup>300</sup>122 and <span><math><mrow><msup><mrow></mrow><mrow><mn>251</mn></mrow></msup><mi>Cf</mi></mrow></math></span> (<span><math><mrow><msup><mrow></mrow><mrow><mn>53</mn></mrow></msup><mi>Mn</mi></mrow></math></span>, 3n)<sup>301</sup>123 with maximum <span><math><msub><mrow><mi>σ</mi></mrow><mrow><mi>E</mi><mi>R</mi></mrow></msub></math></span> are found to be 415.1 fb at 240 MeV, 115.4 fb at 244 MeV, 36.5 fb at 245 MeV, 13.6 fb at 249 MeV, 5.4 fb at 250 MeV for Z=119-123 respectively. These predictions may help the future experimentalist to explore the 8th row in the periodic table.</div></div>","PeriodicalId":100965,"journal":{"name":"Nuclear Analysis","volume":null,"pages":null},"PeriodicalIF":0.0000,"publicationDate":"2024-08-06","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":null,"platform":"Semanticscholar","paperid":null,"PeriodicalName":"Nuclear Analysis","FirstCategoryId":"1085","ListUrlMain":"https://www.sciencedirect.com/science/article/pii/S2773183924000247","RegionNum":0,"RegionCategory":null,"ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"","JCRName":"","Score":null,"Total":0}
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Abstract

We conducted an in-depth investigation of Mn-induced fusion reactions aimed at synthesizing superheavy elements with atomic numbers Z=119 to Z=123. Our analysis considers the total potential, which combines Coulomb and nuclear potentials. The nuclear potential was calculated using the Thomas–Fermi approach, a valuable method for modeling the behavior of nucleons in atomic nuclei. within the framework of advanced statistical model, the evaporation residue cross-sections were determined. At optimal energies, we have calculated capture, fusion, and evaporation residue cross-sections for the reactions of all the projectile–target combinations. All 5355Mn isotopes with larger half-lives were taken into consideration as projectiles. Fusion reactions between 5355Mn projectiles with 238242,244Pu, 241243Am, 242248,250Cm, 247249Bk, and 248254Cf. Detailed investigations were made and promising reactions viz. 241Pu (55Mn, 3n)293119, 242Am (55Mn, 3n)294120, 247Cm (55Mn, 3n)299121, 248Bk (55Mn, 3n)300122 and 251Cf (53Mn, 3n)301123 with maximum σER are found to be 415.1 fb at 240 MeV, 115.4 fb at 244 MeV, 36.5 fb at 245 MeV, 13.6 fb at 249 MeV, 5.4 fb at 250 MeV for Z=119-123 respectively. These predictions may help the future experimentalist to explore the 8th row in the periodic table.
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利用锰射弹合成超重元素 Z>118 所涉及的聚变机制
我们对旨在合成原子序数为 Z=119 至 Z=123 的超重元素的锰诱导聚变反应进行了深入研究。我们的分析考虑了库仑势和核势相结合的总势能。核势能是用托马斯-费米方法计算的,这是一种模拟原子核中核子行为的重要方法。在最佳能量下,我们计算了所有射弹-靶组合反应的俘获、聚变和蒸发残余截面。所有具有较大半衰期的 53-55Mn 同位素都被视为射弹。对 53-55Mn 射弹与 238-242、244Pu、241-243Am、242-248、250Cm、247-249Bk 和 248-254Cf 之间的聚变反应进行了详细的研究,发现有希望的反应包括241Pu (55Mn, 3n)293119, 242Am (55Mn, 3n)294120, 247Cm (55Mn, 3n)299121, 248Bk (55Mn, 3n)300122 和 251Cf (53Mn, 3n)301123 的最大 σER 为 415.1 fb,244 MeV 时为 115.4 fb,245 MeV 时为 36.5 fb,249 MeV 时为 13.6 fb,250 MeV 时为 5.4 fb。这些预测可能有助于未来的实验人员探索元素周期表中的第 8 行。
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