Shape-Dependent Aerosol Dynamics in Indoor Environments: Penetration, Deposition, and Dispersion

IF 12.2 1区 环境科学与生态学 Q1 ENGINEERING, ENVIRONMENTAL Journal of Hazardous Materials Pub Date : 2024-10-28 DOI:10.1016/j.jhazmat.2024.136305
Lipeng Lv, Bin Zhao
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The shape-induced deviations are associated with dynamical processes, showing a decrease trend among penetration, deposition, and dispersion of the non-spherical particles. The maximum discrepancy due to particle shape during the penetration process exceeds 1000%, observed with particles of approximately 0.02 <span><span style=\"\"></span><span data-mathml='&lt;math xmlns=\"http://www.w3.org/1998/Math/MathML\"&gt;&lt;mi is=\"true\"&gt;&amp;#x3BC;&lt;/mi&gt;&lt;mi is=\"true\"&gt;m&lt;/mi&gt;&lt;/math&gt;' role=\"presentation\" style=\"font-size: 90%; display: inline-block; position: relative;\" tabindex=\"0\"><svg aria-hidden=\"true\" focusable=\"false\" height=\"1.855ex\" role=\"img\" style=\"vertical-align: -0.697ex;\" viewbox=\"0 -498.8 1482 798.9\" width=\"3.442ex\" xmlns:xlink=\"http://www.w3.org/1999/xlink\"><g fill=\"currentColor\" stroke=\"currentColor\" stroke-width=\"0\" transform=\"matrix(1 0 0 -1 0 0)\"><g is=\"true\"><use xlink:href=\"#MJMATHI-3BC\"></use></g><g is=\"true\" transform=\"translate(603,0)\"><use xlink:href=\"#MJMATHI-6D\"></use></g></g></svg><span role=\"presentation\"><math xmlns=\"http://www.w3.org/1998/Math/MathML\"><mi is=\"true\">μ</mi><mi is=\"true\">m</mi></math></span></span><script type=\"math/mml\"><math><mi is=\"true\">μ</mi><mi is=\"true\">m</mi></math></script></span> in diameter interacting with straight cracks 4.5<!-- --> <!-- -->cm in length and 0.25<!-- --> <!-- -->mm in height. Moreover, there is a discrepancy of more than 70% in the deposition of particles with a diameter of approximately 10 <span><span style=\"\"></span><span data-mathml='&lt;math xmlns=\"http://www.w3.org/1998/Math/MathML\"&gt;&lt;mi is=\"true\"&gt;&amp;#x3BC;&lt;/mi&gt;&lt;mi is=\"true\"&gt;m&lt;/mi&gt;&lt;/math&gt;' role=\"presentation\" style=\"font-size: 90%; display: inline-block; position: relative;\" tabindex=\"0\"><svg aria-hidden=\"true\" focusable=\"false\" height=\"1.855ex\" role=\"img\" style=\"vertical-align: -0.697ex;\" viewbox=\"0 -498.8 1482 798.9\" width=\"3.442ex\" xmlns:xlink=\"http://www.w3.org/1999/xlink\"><g fill=\"currentColor\" stroke=\"currentColor\" stroke-width=\"0\" transform=\"matrix(1 0 0 -1 0 0)\"><g is=\"true\"><use xlink:href=\"#MJMATHI-3BC\"></use></g><g is=\"true\" transform=\"translate(603,0)\"><use xlink:href=\"#MJMATHI-6D\"></use></g></g></svg><span role=\"presentation\"><math xmlns=\"http://www.w3.org/1998/Math/MathML\"><mi is=\"true\">μ</mi><mi is=\"true\">m</mi></math></span></span><script type=\"math/mml\"><math><mi is=\"true\">μ</mi><mi is=\"true\">m</mi></math></script></span> on side walls when using side air supply ventilation. Similarly, a discrepancy of nearly 11% is noted for particles around 0.02 <span><span style=\"\"></span><span data-mathml='&lt;math xmlns=\"http://www.w3.org/1998/Math/MathML\"&gt;&lt;mi is=\"true\"&gt;&amp;#x3BC;&lt;/mi&gt;&lt;mi is=\"true\"&gt;m&lt;/mi&gt;&lt;/math&gt;' role=\"presentation\" style=\"font-size: 90%; display: inline-block; position: relative;\" tabindex=\"0\"><svg aria-hidden=\"true\" focusable=\"false\" height=\"1.855ex\" role=\"img\" style=\"vertical-align: -0.697ex;\" viewbox=\"0 -498.8 1482 798.9\" width=\"3.442ex\" xmlns:xlink=\"http://www.w3.org/1999/xlink\"><g fill=\"currentColor\" stroke=\"currentColor\" stroke-width=\"0\" transform=\"matrix(1 0 0 -1 0 0)\"><g is=\"true\"><use xlink:href=\"#MJMATHI-3BC\"></use></g><g is=\"true\" transform=\"translate(603,0)\"><use xlink:href=\"#MJMATHI-6D\"></use></g></g></svg><span role=\"presentation\"><math xmlns=\"http://www.w3.org/1998/Math/MathML\"><mi is=\"true\">μ</mi><mi is=\"true\">m</mi></math></span></span><script type=\"math/mml\"><math><mi is=\"true\">μ</mi><mi is=\"true\">m</mi></math></script></span> in diameter during dispersion under displacement ventilation within indoor settings. The interaction between shape-related particle dynamics, particularly their diffusion characteristics, and the properties of the flow field leads to these shape-dependent dynamical discrepancies. These findings offer a comprehensive understanding of how the shape of particles affects their indoor dynamic behavior, thereby supporting the control of hazardous particles in indoor environments.","PeriodicalId":361,"journal":{"name":"Journal of Hazardous Materials","volume":null,"pages":null},"PeriodicalIF":12.2000,"publicationDate":"2024-10-28","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":null,"platform":"Semanticscholar","paperid":null,"PeriodicalName":"Journal of Hazardous Materials","FirstCategoryId":"93","ListUrlMain":"https://doi.org/10.1016/j.jhazmat.2024.136305","RegionNum":1,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"ENGINEERING, ENVIRONMENTAL","Score":null,"Total":0}
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Abstract

Particle shape exerts a significant influence on their dynamic behavior, and it is imperative to elucidate these effects given the potential for severe environmental toxicity associated with shaped particles. Despite extensive research on the dynamical processes of spherical particles, the behaviors of non-spherical particles have been insufficiently investigated. In this study, we have developed a suite of computation-based models that account for particle shape and have reported on the typical dynamical behaviors of non-spherical particles within indoor environments. We have explored three typical scenarios, i.e., particle penetration into indoor spaces through building cracks, indoor particle deposition, and indoor particle dispersion. The shape-induced deviations are associated with dynamical processes, showing a decrease trend among penetration, deposition, and dispersion of the non-spherical particles. The maximum discrepancy due to particle shape during the penetration process exceeds 1000%, observed with particles of approximately 0.02 μm in diameter interacting with straight cracks 4.5 cm in length and 0.25 mm in height. Moreover, there is a discrepancy of more than 70% in the deposition of particles with a diameter of approximately 10 μm on side walls when using side air supply ventilation. Similarly, a discrepancy of nearly 11% is noted for particles around 0.02 μm in diameter during dispersion under displacement ventilation within indoor settings. The interaction between shape-related particle dynamics, particularly their diffusion characteristics, and the properties of the flow field leads to these shape-dependent dynamical discrepancies. These findings offer a comprehensive understanding of how the shape of particles affects their indoor dynamic behavior, thereby supporting the control of hazardous particles in indoor environments.

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室内环境中与形状有关的气溶胶动力学:渗透、沉积和扩散
颗粒的形状对其动态行为有重大影响,鉴于异形颗粒可能对环境造成严重危害,因此必须阐明这些影响。尽管对球形颗粒的动态过程进行了广泛研究,但对非球形颗粒的行为研究还不够。在这项研究中,我们开发了一套基于计算的模型,其中考虑到了颗粒的形状,并报告了非球形颗粒在室内环境中的典型动力学行为。我们探讨了三种典型情况,即粒子通过建筑裂缝渗入室内空间、室内粒子沉积和室内粒子扩散。形状引起的偏差与动态过程有关,在非球形粒子的穿透、沉积和扩散过程中呈现出下降趋势。在穿透过程中,直径约为 0.02 μm μm 的颗粒与长 4.5 厘米、高 0.25 毫米的直线裂缝相互作用时,由于颗粒形状造成的最大偏差超过了 1000%。此外,在使用侧送风通风时,直径约为 10 μm μm 的颗粒在侧壁上的沉积量相差超过 70%。同样,在室内环境中使用置换通风时,直径约为 0.02 μm μm 的颗粒在扩散过程中的差异也接近 11%。与形状相关的颗粒动力学(尤其是其扩散特性)和流场特性之间的相互作用导致了这些与形状相关的动力学差异。这些发现提供了对颗粒形状如何影响其室内动态行为的全面理解,从而为控制室内环境中的有害颗粒提供了支持。
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来源期刊
Journal of Hazardous Materials
Journal of Hazardous Materials 工程技术-工程:环境
CiteScore
25.40
自引率
5.90%
发文量
3059
审稿时长
58 days
期刊介绍: The Journal of Hazardous Materials serves as a global platform for promoting cutting-edge research in the field of Environmental Science and Engineering. Our publication features a wide range of articles, including full-length research papers, review articles, and perspectives, with the aim of enhancing our understanding of the dangers and risks associated with various materials concerning public health and the environment. It is important to note that the term "environmental contaminants" refers specifically to substances that pose hazardous effects through contamination, while excluding those that do not have such impacts on the environment or human health. Moreover, we emphasize the distinction between wastes and hazardous materials in order to provide further clarity on the scope of the journal. We have a keen interest in exploring specific compounds and microbial agents that have adverse effects on the environment.
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