Al/AlN-based thermal paste fillers prepared by self-propagating high-temperature synthesis (SHS)

IF 2.8 4区 工程技术 Q2 ENGINEERING, ELECTRICAL & ELECTRONIC Journal of Materials Science: Materials in Electronics Pub Date : 2024-11-04 DOI:10.1007/s10854-024-13703-0
Anton Reger, Alexander Akulinkin
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Abstract

This paper describes the synthesis of material with different aluminum and aluminum nitride concentrations through the nitriding combustion of aluminum. The effect of pre-nitrided additives on combustion rate, maximum combustion temperature, and nitrogen and oxygen content in the synthesized products is analyzed. Additionally, the phase composition and microstructure of the synthesized materials are presented. The synthesized material is used as filler for thermal paste with an organosilicon binder (polymethylsiloxane). The thermal paste with filler, produced by one-step combustion of aluminum with the highest amount of unreacted aluminum, exhibited the highest thermal conductivity coefficient. With increasing the aluminum concentration, the thermal paste maintained its dielectric properties. The thermal paste demonstrated high efficiency in dissipating heat when applied between the heatsink and the heated body. The CPU stress test confirmed its effectiveness.

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通过自蔓延高温合成(SHS)制备铝/氮化铝基导热膏填料
本文介绍了通过铝氮化燃烧合成不同铝和氮化铝浓度的材料。分析了预氮化添加剂对燃烧速率、最高燃烧温度以及合成产物中氮和氧含量的影响。此外,还介绍了合成材料的相组成和微观结构。合成材料被用作有机硅粘合剂(聚甲基硅氧烷)导热膏的填料。通过铝的一步燃烧制得的带有填料的导热膏具有最高的导热系数,其中未反应铝的含量最高。随着铝浓度的增加,导热膏保持了其介电特性。在散热器和发热体之间使用导热膏时,导热膏表现出很高的散热效率。CPU 压力测试证实了其有效性。
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来源期刊
Journal of Materials Science: Materials in Electronics
Journal of Materials Science: Materials in Electronics 工程技术-材料科学:综合
CiteScore
5.00
自引率
7.10%
发文量
1931
审稿时长
2 months
期刊介绍: The Journal of Materials Science: Materials in Electronics is an established refereed companion to the Journal of Materials Science. It publishes papers on materials and their applications in modern electronics, covering the ground between fundamental science, such as semiconductor physics, and work concerned specifically with applications. It explores the growth and preparation of new materials, as well as their processing, fabrication, bonding and encapsulation, together with the reliability, failure analysis, quality assurance and characterization related to the whole range of applications in electronics. The Journal presents papers in newly developing fields such as low dimensional structures and devices, optoelectronics including III-V compounds, glasses and linear/non-linear crystal materials and lasers, high Tc superconductors, conducting polymers, thick film materials and new contact technologies, as well as the established electronics device and circuit materials.
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