Structural and magnetic properties of Co2FeGa full-Heusler alloy thin films with low Gilbert damping

IF 2.5 3区 材料科学 Q3 MATERIALS SCIENCE, MULTIDISCIPLINARY Journal of Magnetism and Magnetic Materials Pub Date : 2024-11-30 DOI:10.1016/j.jmmm.2024.172691
Bruno L.D. Santos , Alisson C. Krohling , Klaus Krambrock , Edson C. Passamani , Waldemar A.A. Macedo
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Abstract

Highly ordered Co2FeGa thin films were successfully prepared using direct current magnetron sputtering by adjusting the film growth conditions. This involved making modifications to substrate and annealing temperatures. Structural, chemical, and magnetic properties were systematically studied using global and surface techniques. The results showed a transition from a partially ordered film grown at 300 °C to a highly ordered L21 full-Heusler phase at 600 °C. X-ray photoelectron spectroscopy confirmed a stoichiometric Co2FeGa alloy for the films, while 57Fe conversion electron Mössbauer spectroscopy revealed the atomic disorder–order transition induced by high substrate temperatures and/or annealing temperatures. The magnetic properties were found to be strongly influenced by the thermal history of the films. Saturation magnetization reached 1200 kA/m and coercivity was as low as 0.8 mT for the film growth at 600 °C. Ferromagnetic resonance showed that the α-Gilbert damping parameter was significantly affected by growth conditions with a value of 0.0015(3) measured in films grown at the highest temperature. This study demonstrates that precise control over film crystallinity and atomic ordering can lead to low α-damping values in polycrystalline Co2FeGa thin films, making them promising materials for use in spintronic devices.
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低吉尔伯特阻尼Co2FeGa全heusler合金薄膜的结构和磁性能
通过调整薄膜生长条件,采用直流磁控溅射法制备了高有序的Co2FeGa薄膜。这涉及到对衬底和退火温度的修改。结构,化学和磁性性能系统地研究使用全局和表面技术。结果表明,在300℃下生长的部分有序膜在600℃下转变为高度有序的L21 full-Heusler相。x射线光电子能谱证实了薄膜为Co2FeGa合金,而57Fe转换电子Mössbauer能谱显示了高衬底温度和/或退火温度诱导的原子无序-有序转变。发现薄膜的磁性能受热历史的强烈影响。在600℃下,薄膜的饱和磁化强度达到1200 kA/m,矫顽力低至0.8 mT。铁磁共振结果表明,生长条件对α-Gilbert阻尼参数有显著影响,在最高温度下生长的薄膜α-Gilbert阻尼参数值为0.0015(3)。该研究表明,对薄膜结晶度和原子有序度的精确控制可以导致多晶Co2FeGa薄膜的α-阻尼值较低,使其成为用于自旋电子器件的有前途的材料。
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来源期刊
Journal of Magnetism and Magnetic Materials
Journal of Magnetism and Magnetic Materials 物理-材料科学:综合
CiteScore
5.30
自引率
11.10%
发文量
1149
审稿时长
59 days
期刊介绍: The Journal of Magnetism and Magnetic Materials provides an important forum for the disclosure and discussion of original contributions covering the whole spectrum of topics, from basic magnetism to the technology and applications of magnetic materials. The journal encourages greater interaction between the basic and applied sub-disciplines of magnetism with comprehensive review articles, in addition to full-length contributions. In addition, other categories of contributions are welcome, including Critical Focused issues, Current Perspectives and Outreach to the General Public. Main Categories: Full-length articles: Technically original research documents that report results of value to the communities that comprise the journal audience. The link between chemical, structural and microstructural properties on the one hand and magnetic properties on the other hand are encouraged. In addition to general topics covering all areas of magnetism and magnetic materials, the full-length articles also include three sub-sections, focusing on Nanomagnetism, Spintronics and Applications. The sub-section on Nanomagnetism contains articles on magnetic nanoparticles, nanowires, thin films, 2D materials and other nanoscale magnetic materials and their applications. The sub-section on Spintronics contains articles on magnetoresistance, magnetoimpedance, magneto-optical phenomena, Micro-Electro-Mechanical Systems (MEMS), and other topics related to spin current control and magneto-transport phenomena. The sub-section on Applications display papers that focus on applications of magnetic materials. The applications need to show a connection to magnetism. Review articles: Review articles organize, clarify, and summarize existing major works in the areas covered by the Journal and provide comprehensive citations to the full spectrum of relevant literature.
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