A fabric-based multi-functional solar evaporator with all-weather efficient continuous evaporating capability through photothermal and electrothermal effects†
Chuanliang Chen, Minhan Cheng, Yuliang Qu, Ke Tian, Qianyang Li, Qiang Fu and Hua Deng
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引用次数: 0
Abstract
Solar-driven desalination is a promising strategy to alleviate the water crisis. However, the intermittent nature of solar irradiation presents a significant challenge in achieving continuous steam generation under all conditions. Most existing methods for fabricating solar evaporators lack scalability, flexibility, and convenience. This study presents an all-weather fabric-based solar evaporation system that integrates carbon nanotubes and in situ anchored copper sulfide nanostructures. The system collects solar energy, leveraging the strong light absorption and excellent conductivity of the fabric, and enables continuous steam generation through alternating photothermal and electrothermal conversion both during the day and at night. Thanks to the synergistic effects of photothermal (1 sun) and electrothermal (5 V) methods, the evaporation system achieves an evaporation rate of up to 5.03 kg m−2 h−1 in 3.5 wt% NaCl solution, while also reaching 1.93 kg m−2 h−1 at night. Additionally, during a continuous 7 day test, the system demonstrates excellent stability. Importantly, the evaporation system collects 46.36 kg m−2 of high-flux condensate during a day of real seawater testing under weak outdoor illumination. Furthermore, this evaporator encompasses antibacterial and UV resistance functions. This study provides a promising approach for efficient, all-weather seawater desalination in complex environments.
太阳能驱动的海水淡化是缓解水危机的一个很有前途的策略。然而,在所有条件下,太阳辐照的间歇性对实现连续蒸汽产生提出了重大挑战。大多数现有的制造太阳能蒸发器的方法缺乏可扩展性、灵活性和便利性。本研究提出了一种基于织物的全天候太阳能蒸发系统,该系统集成了碳纳米管和原位锚定硫化铜纳米结构。该系统收集太阳能,利用织物的强光吸收和优异的导电性,并在白天和晚上通过交替的光热和电热转换实现连续的蒸汽产生。由于光热(1个太阳)和电热(5 V)方法的协同作用,蒸发系统在3.5 wt% NaCl溶液中实现了高达5.03 kg m−2 h−1的蒸发速率,而在夜间也达到了1.93 kg m−2 h−1。此外,在连续7天的测试中,系统表现出出色的稳定性。重要的是,在室外光照较弱的真实海水测试中,蒸发系统在一天内收集了46.36 kg m−2的高通量冷凝水。此外,该蒸发器还具有抗菌和抗紫外线功能。该研究为复杂环境下的高效、全天候海水淡化提供了一条有前景的途径。
期刊介绍:
The Journal of Materials Chemistry A, B & C covers a wide range of high-quality studies in the field of materials chemistry, with each section focusing on specific applications of the materials studied. Journal of Materials Chemistry A emphasizes applications in energy and sustainability, including topics such as artificial photosynthesis, batteries, and fuel cells. Journal of Materials Chemistry B focuses on applications in biology and medicine, while Journal of Materials Chemistry C covers applications in optical, magnetic, and electronic devices. Example topic areas within the scope of Journal of Materials Chemistry A include catalysis, green/sustainable materials, sensors, and water treatment, among others.