Quantum Efficiency and Vertical Position of Quantum Emitters in hBN Determined by Purcell Effect in Hybrid Metal-Dielectric Planar Photonic Structures

IF 6.5 1区 物理与天体物理 Q1 MATERIALS SCIENCE, MULTIDISCIPLINARY ACS Photonics Pub Date : 2024-12-06 DOI:10.1021/acsphotonics.4c01416
Domitille Gérard, Aurélie Pierret, Helmi Fartas, Bruno Berini, Stéphanie Buil, Jean-Pierre Hermier, Aymeric Delteil
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Abstract

Color centers in hexagonal boron nitride (hBN) advantageously combine excellent photophysical properties with the potential for integration in highly compact devices. Progress toward scalable integration necessitates a high quantum efficiency and an efficient photon collection. In this context, we compare the optical characteristics of individual hBN color centers generated by electron irradiation in two different electromagnetic environments. We keep track of well-identified emitters that we characterize before and after the dry transfer of exfoliated crystals. This comparison provides information about their quantum efficiency, which we find close to unity, as well as their vertical position in the crystal with nanometric precision, which we find away from the flake surfaces. Our work suggests hybrid dielectric-metal planar structures as an efficient tool for characterizing quantum emitters in addition to improving the count rate and can be generalized to other emitters in 2D materials or in planar photonic structures.

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利用金属-介电杂化平面光子结构中的Purcell效应确定hBN中量子发射体的量子效率和垂直位置
六方氮化硼(hBN)的色心有利地结合了优异的光物理性质和集成在高度紧凑器件中的潜力。向可扩展集成的进展需要高量子效率和有效的光子收集。在这种情况下,我们比较了在两种不同的电磁环境下电子辐照产生的单个hBN色心的光学特性。我们跟踪在剥离晶体干燥转移之前和之后我们表征的识别良好的发射器。这种比较提供了关于它们的量子效率的信息,我们发现它们接近于一致,以及它们在晶体中的垂直位置,我们发现它们具有纳米精度,远离薄片表面。我们的工作表明,除了提高计数率外,混合介质-金属平面结构作为表征量子发射体的有效工具,可以推广到二维材料或平面光子结构中的其他发射体。
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来源期刊
ACS Photonics
ACS Photonics NANOSCIENCE & NANOTECHNOLOGY-MATERIALS SCIENCE, MULTIDISCIPLINARY
CiteScore
11.90
自引率
5.70%
发文量
438
审稿时长
2.3 months
期刊介绍: Published as soon as accepted and summarized in monthly issues, ACS Photonics will publish Research Articles, Letters, Perspectives, and Reviews, to encompass the full scope of published research in this field.
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