Ultra-fast, cost-effective and scale-up preparation of lightweight electromagnetic interference shielding graphite worm-based aerogel

IF 13.3 1区 工程技术 Q1 ENGINEERING, CHEMICAL Chemical Engineering Journal Pub Date : 2024-12-23 DOI:10.1016/j.cej.2024.158793
Xin Yan, Jianming Yang, Chenghan Huang, Ziyin Yu, He-Xin Zhang, Liang Fang, Keun-Byoung Yoon
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Abstract

Lightweight aerogels with conductive properties have been widely considered promising materials for electromagnetic interference (EMI) shielding. However, there are still challenges to achieve large-scale preparation of aerogels through simple, convenient and economical methods. In this study, graphite worm-based aerogel (GWA) with high electrical conductivity was prepared by one-step mixing graphite worms with a gel-like product made of polyvinyl alcohol (PVA), glycerol and borax. The phase separation between the hydrophobic graphite worm and the hydrophilic polymer enables excellent retention of the pore structure. The “worm-like” porous structural framework promotes the scattering and reflection of EM waves, effectively attenuating EM energy. The results indicate that the developed GWA material exhibits a high shielding performance of 58.0 dB. The existence of a three-dimensional conductive network endows the GWA material with excellent Joule heating performance (146.1 °C) at 10 V. In addition, the GWA material exhibited EMI shielding effectiveness (SE) retention of 98.1 % after three recycling cycles, which guarantees its service life in practical applications. This study provides a feasible solution for the large-scale preparation of aerogels with excellent EMI shielding performance, effectively alleviating the contradiction between the construction of porous structures and large-scale production.

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来源期刊
Chemical Engineering Journal
Chemical Engineering Journal 工程技术-工程:化工
CiteScore
21.70
自引率
9.30%
发文量
6781
审稿时长
2.4 months
期刊介绍: The Chemical Engineering Journal is an international research journal that invites contributions of original and novel fundamental research. It aims to provide an international platform for presenting original fundamental research, interpretative reviews, and discussions on new developments in chemical engineering. The journal welcomes papers that describe novel theory and its practical application, as well as those that demonstrate the transfer of techniques from other disciplines. It also welcomes reports on carefully conducted experimental work that is soundly interpreted. The main focus of the journal is on original and rigorous research results that have broad significance. The Catalysis section within the Chemical Engineering Journal focuses specifically on Experimental and Theoretical studies in the fields of heterogeneous catalysis, molecular catalysis, and biocatalysis. These studies have industrial impact on various sectors such as chemicals, energy, materials, foods, healthcare, and environmental protection.
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