Bottle Aging of Smoke-Affected Wines: Changes in Smoke Flavor and Chemical Composition

IF 6.2 1区 农林科学 Q1 AGRICULTURE, MULTIDISCIPLINARY Journal of Agricultural and Food Chemistry Pub Date : 2025-01-07 DOI:10.1021/acs.jafc.4c10590
Mango Parker, Eleanor Bilogrevic, WenWen Jiang, Eric Wilkes, I. Leigh Francis, Markus J. Herderich
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Abstract

Winegrapes exposed to environmental wildfire smoke during ripening can be identified through analysis of volatile phenols and phenolic glycosides. While elevated concentrations of these smoke marker compounds in grapes have been shown to be predictive of composition and smoke flavor in young wines, recent research has demonstrated that not every wine produced from smoke-exposed grapes will inevitably have discernible smoke flavor when assessed as young wine 6 weeks after bottling. This is supported by anecdotal reports from wine producers that wines that do not appear noticeably smoky when young become noticeably smoky during aging. Yet there is little data available to date on the chemical composition and sensory attributes of aged wines produced from grapes exposed to environmental wildfire smoke. Data are largely limited to smoke-affected wines from model studies with deliberately smoked vines, and suggest that the concentrations of volatile phenols and glycosides may remain relatively unchanged after 5 to 6 years of bottle aging. To address the gap in knowledge, this study followed 49 wines made from grapes exposed to wildfire smoke during the 2019–2020 ripening season and reports the results obtained from monitoring chemical composition and smoke flavor intensity up for to three years after bottling. Notably, the concentrations of volatile phenols and glycosides did not change significantly over 39 months in the bottle, with the exception of syringol, which increased in both smoke-affected and control wines. Significant smoke flavor ratings were consistent over the three years for the majority of the wines (73%). For nine mildly smoke-affected wines, smoke flavor became apparent in older wines, while it had not been apparent in the young wines, likely due to masking by other attributes. These data represent a substantial database of smoke marker concentrations in wine and smoke flavor to provide context when interpreting smoke marker analysis in the future.

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烟熏葡萄酒的瓶内陈酿:烟味和化学成分的变化
在成熟过程中暴露于环境野火烟雾中的酿酒葡萄可以通过分析挥发性酚和酚类苷来识别。虽然葡萄中这些烟雾标记化合物的浓度升高已被证明可以预测年轻葡萄酒的成分和烟味,但最近的研究表明,在装瓶后6周评估年轻葡萄酒时,并非所有由暴露于烟雾中的葡萄生产的葡萄酒都不可避免地具有可识别的烟味。这得到了葡萄酒生产商的轶事报道的支持,即年轻时没有明显烟雾的葡萄酒在陈年过程中会变得明显烟雾。然而,迄今为止,关于暴露在野火烟雾中的葡萄酿造的陈年葡萄酒的化学成分和感官属性的数据很少。数据很大程度上局限于烟雾影响葡萄酒的模型研究,这些研究采用故意熏过的葡萄藤,并表明挥发性酚和苷的浓度在瓶中陈化5到6年后可能保持相对不变。为了解决知识上的差距,这项研究跟踪了49种葡萄酒,这些葡萄酒是由2019-2020年成熟季节暴露在野火烟雾中的葡萄制成的,并报告了装瓶后长达三年的化学成分和烟雾风味强度监测结果。值得注意的是,挥发性酚和糖苷的浓度在39个月内没有明显变化,除了丁香醇,在烟雾影响和对照葡萄酒中都有所增加。在过去的三年里,大多数葡萄酒(73%)的烟味评级都是一致的。对于九种轻度烟雾影响的葡萄酒,烟雾味在较老的葡萄酒中变得明显,而在年轻的葡萄酒中则不明显,可能是由于其他属性的掩盖。这些数据代表了葡萄酒和烟味中烟雾标记物浓度的大量数据库,为将来解释烟雾标记物分析提供了背景。
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来源期刊
Journal of Agricultural and Food Chemistry
Journal of Agricultural and Food Chemistry 农林科学-农业综合
CiteScore
9.90
自引率
8.20%
发文量
1375
审稿时长
2.3 months
期刊介绍: The Journal of Agricultural and Food Chemistry publishes high-quality, cutting edge original research representing complete studies and research advances dealing with the chemistry and biochemistry of agriculture and food. The Journal also encourages papers with chemistry and/or biochemistry as a major component combined with biological/sensory/nutritional/toxicological evaluation related to agriculture and/or food.
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