Unveiling the role of NiFeM hydroxide (M = Pt, Ru, Ir, Rh) cocatalysts for robust H2 production in photocatalytic water splitting

IF 4.3 2区 化学 Q2 CHEMISTRY, MULTIDISCIPLINARY Chemical Communications Pub Date : 2025-01-20 DOI:10.1039/d4cc06199c
Mengmeng Shao, Wei Shi, Junhui Jiang, Shihua Tan, Xuehan Wang, Jiawei Fei, Jinhua Li, Zhangjing Zhang
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Abstract

In this study, the NiFe-LDH doped with different Pt group metals (Pt, Ru, Ir, Rh) was prepared as a cocatalyst for photocatalytic H2 production over g-C3N4. It is found that the doped NiFe-LDH loaded g-C3N4 generally displays higher photocatalytic activity than the raw NiFe-LDH modified one, where the NiFeRu-LDH loaded g-C3N4 shows the optimal H2 evolution rate of 77.4 μmol h−1, about 5.5 times that of the NiFe-LDH system.

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揭示氢氧化NiFeM (M = Pt, Ru, Ir, Rh)助催化剂在光催化水裂解中强劲产氢的作用
本研究制备了不同Pt族金属(Pt, Ru, Ir, Rh)掺杂的NiFe-LDH作为g-C3N4光催化制氢的助催化剂。结果表明,掺杂NiFe-LDH后的g-C3N4的光催化活性普遍高于未经NiFe-LDH修饰的g-C3N4,其中NiFeRu-LDH负载的g-C3N4的最佳析氢速率为77.4 μmol h−1,约为NiFe-LDH体系的5.5倍。
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来源期刊
Chemical Communications
Chemical Communications 化学-化学综合
CiteScore
8.60
自引率
4.10%
发文量
2705
审稿时长
1.4 months
期刊介绍: ChemComm (Chemical Communications) is renowned as the fastest publisher of articles providing information on new avenues of research, drawn from all the world''s major areas of chemical research.
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