Non-destructive prediction and pixel-level visualization of polysaccharide-based properties in ancient paper using SWNIR hyperspectral imaging and machine learning

IF 12.5 1区 化学 Q1 CHEMISTRY, APPLIED Carbohydrate Polymers Pub Date : 2025-03-15 Epub Date: 2024-12-30 DOI:10.1016/j.carbpol.2024.123198
Yan Wu , Bin Wang , Jian Chen , Xinkang Huang , Jun Xu , Wenguang Wei , Kefu Chen
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Abstract

Ancient documents and artworks are invaluable cultural heritage artworks that require careful preservation. Traditional methods for assessing their physical and chemical properties—such as tearing index, tensile index, water absorption, and pH—are often destructive, risking irreversible damage. This study introduces a novel, non-destructive approach using Short-Wave Near-Infrared (SWNIR) hyperspectral imaging (HSI) combined with advanced machine learning models. By integrating spectral preprocessing, feature selection, and machine learning techniques—including Back Propagation Neural Networks (BPNN), Long Short-Term Memory Networks (LSTM), and Convolutional Neural Networks (CNN)—with Sparrow Search Algorithm (SSA) optimization and Gray Level Co-occurrence Matrix (GLCM) texture feature extraction, the resulting SSA-BP-UVE-GLCM model achieved high predictive accuracy (R2 ≥ 0.98). This framework enables precise, pixel-level predictions of paper properties, influenced by polysaccharides like cellulose, offering a non-invasive analysis that supports targeted restoration strategies and advances the conservation of cultural heritage. The findings enhance non-invasive testing and classification methods for polysaccharide-based materials, providing a foundation for further exploration of environmental impacts on artwork integrity using sophisticated machine learning algorithms.

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基于SWNIR高光谱成像和机器学习的古代纸张中多糖性质的无损预测和像素级可视化。
古代文献和艺术品是宝贵的文化遗产,需要精心保护。评估其物理和化学性质的传统方法(如撕裂指数、拉伸指数、吸水率和ph值)往往具有破坏性,有可能造成不可逆转的损害。本研究介绍了一种新颖的、非破坏性的方法,使用短波近红外(SWNIR)高光谱成像(HSI)结合先进的机器学习模型。通过将光谱预处理、特征选择和机器学习技术(包括反向传播神经网络(BPNN)、长短期记忆网络(LSTM)和卷积神经网络(CNN))与Sparrow搜索算法(SSA)优化和灰度共生矩阵(GLCM)纹理特征提取相结合,得到的SSA- bp - uve -GLCM模型具有较高的预测精度(R2≥0.98)。该框架能够精确地、像素级地预测受纤维素等多糖影响的纸张特性,提供非侵入性分析,支持有针对性的修复策略,并促进文化遗产的保护。研究结果增强了多糖基材料的非侵入性测试和分类方法,为使用复杂的机器学习算法进一步探索环境对艺术品完整性的影响提供了基础。
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来源期刊
Carbohydrate Polymers
Carbohydrate Polymers 化学-高分子科学
CiteScore
22.40
自引率
8.00%
发文量
1286
审稿时长
47 days
期刊介绍: Carbohydrate Polymers stands as a prominent journal in the glycoscience field, dedicated to exploring and harnessing the potential of polysaccharides with applications spanning bioenergy, bioplastics, biomaterials, biorefining, chemistry, drug delivery, food, health, nanotechnology, packaging, paper, pharmaceuticals, medicine, oil recovery, textiles, tissue engineering, wood, and various aspects of glycoscience. The journal emphasizes the central role of well-characterized carbohydrate polymers, highlighting their significance as the primary focus rather than a peripheral topic. Each paper must prominently feature at least one named carbohydrate polymer, evident in both citation and title, with a commitment to innovative research that advances scientific knowledge.
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