Broadband and High-Resolution Mid-Infrared Spectroscopy Enabled by a Single Phase Change Metasurface

IF 10 1区 物理与天体物理 Q1 OPTICS Laser & Photonics Reviews Pub Date : 2025-01-25 DOI:10.1002/lpor.202401473
Yi Xu, Yan Li, Ruifeng Zhong, Yu-Ru Li, Qiang Li, Dawei Wang, Zhenshi Chen, Jingshun Pan, Zhaohui Li
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Abstract

The mid-infrared (MIR) spectral region is crucial for various applications due to its unique properties, but traditional spectrometers are often bulky. Miniaturized spectrometers face a trade-off between spectral and spatial resolution. Here, a novel approach to MIR spectroscopy is numerically demonstrated by employing an electrically controlled phase-change metasurface. This method fully exploits the high optical contrast and the quasi-continuous phase change characteristics of chalcogenide phase change materials, enabling the construction of a set of spectral responses that provide broad spectral coverage with low correlation, utilizing a single metasurface pixel. With this innovative strategy, a broadband and high-resolution spectral reconstruction is numerically demonstrated with a full width at half maximum (FWHM) resolution of 20 nm and a dual-peak resolution of 160 nm within a 2400 nm bandwidth. Furthermore, the potential of the spectral detection scheme is underscored by the successful numerical reconstruction of the absorption peaks of methane and carbon dioxide, highlighting its capability for gas analysis and molecular identification. The integration of the spectral detection method into the field of spectral imaging is anticipated to have significant implications, suggesting substantial improvements in chemical process monitoring, and rapid diagnostic techniques in combustion environments.

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由单一相变超表面实现的宽带和高分辨率中红外光谱
中红外(MIR)光谱区域由于其独特的性能对各种应用至关重要,但传统的光谱仪往往体积庞大。小型化光谱仪面临着光谱分辨率和空间分辨率之间的权衡。在这里,MIR光谱的一种新方法是通过采用电控相变超表面进行数值演示。该方法充分利用硫系相变材料的高光学对比度和准连续相变特性,利用单个超表面像元,构建了一组具有低相关性、宽光谱覆盖的光谱响应。利用这一创新的策略,宽带和高分辨率的光谱重建在数值上得到了验证,其中全宽度半最大(FWHM)分辨率为20 nm,双峰分辨率为160 nm,带宽为2400 nm。此外,通过对甲烷和二氧化碳吸收峰的成功数值重建,强调了光谱检测方案的潜力,突出了其气体分析和分子识别的能力。光谱检测方法与光谱成像领域的整合预计将产生重大影响,表明化学过程监测和燃烧环境中的快速诊断技术的实质性改进。
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来源期刊
CiteScore
14.20
自引率
5.50%
发文量
314
审稿时长
2 months
期刊介绍: Laser & Photonics Reviews is a reputable journal that publishes high-quality Reviews, original Research Articles, and Perspectives in the field of photonics and optics. It covers both theoretical and experimental aspects, including recent groundbreaking research, specific advancements, and innovative applications. As evidence of its impact and recognition, Laser & Photonics Reviews boasts a remarkable 2022 Impact Factor of 11.0, according to the Journal Citation Reports from Clarivate Analytics (2023). Moreover, it holds impressive rankings in the InCites Journal Citation Reports: in 2021, it was ranked 6th out of 101 in the field of Optics, 15th out of 161 in Applied Physics, and 12th out of 69 in Condensed Matter Physics. The journal uses the ISSN numbers 1863-8880 for print and 1863-8899 for online publications.
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