Effects of hydraulic circulation induced by gravel lenses of varying sizes on nitrobenzene removal in heterogeneous aquifers during air sparging remediation

IF 11.3 1区 环境科学与生态学 Q1 ENGINEERING, ENVIRONMENTAL Journal of Hazardous Materials Pub Date : 2025-02-04 DOI:10.1016/j.jhazmat.2025.137461
Meng Yao , Yitao Xu , Xuyang Chen , Kaiqi Zhang , Chao Guo , Wei Wang , Bowen Li , Mingxin Wang
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Abstract

Air sparging (AS) technology is widely used in groundwater remediation of organic contaminants. In this study, using a two-dimensional physical model, the research explores how varying sizes of gravel lenses affect airflow distribution, hydraulic circulation, and contaminant removal efficiency. The presence of gravel lenses was found to significantly enhance hydraulic circulation, thereby improving the removal of nitrobenzene. The study revealed that the length and height of the gravel lenses play crucial roles in determining the airflow pattern and the extent of hydraulic circulation. A lens length of 5 cm was sufficient to form a hydraulic circulation zone, while a lens height of 4 cm was necessary for effective bubble migration. As the lens thickness increased, the bubble migration path extended, enhancing the bubble pulsation effect and the remediation zone. However, beyond the thickness of 10 cm, further increases in lens thickness did not significantly improve removal efficiency, likely due to stable gas-liquid mass transfer rates. The study concluded that gravel lenses were essential for establishing hydraulic circulation in AS processes, which could lead to more effective remediation strategies in heterogeneous aquifers. These findings provide valuable insights for optimizing AS system designs in complex geological settings.

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空气雾化修复过程中不同尺寸砾石透镜诱导的水力循环对非均质含水层中硝基苯去除的影响
空气喷射技术在地下水有机污染物的修复中得到了广泛的应用。在本研究中,采用二维物理模型,研究了不同尺寸的砾石透镜对气流分布、水力循环和污染物去除效率的影响。砾石透镜的存在显著增强了液压循环,从而提高了硝基苯的去除率。研究表明,砾石透镜的长度和高度对气流形态和水力循环程度起着至关重要的作用。5 cm的透镜长度足以形成水力循环区,而4 cm的透镜高度则需要有效的气泡迁移。随着透镜厚度的增加,气泡迁移路径延长,气泡脉动效应增强,修复带增强。然而,在厚度超过10 cm时,进一步增加透镜厚度并没有显著提高去除效率,这可能是由于稳定的气液传质速率。研究表明,砾石透镜对于建立AS过程中的水力循环至关重要,可以为非均质含水层提供更有效的修复策略。这些发现为在复杂地质环境中优化AS系统设计提供了有价值的见解。
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来源期刊
Journal of Hazardous Materials
Journal of Hazardous Materials 工程技术-工程:环境
CiteScore
25.40
自引率
5.90%
发文量
3059
审稿时长
58 days
期刊介绍: The Journal of Hazardous Materials serves as a global platform for promoting cutting-edge research in the field of Environmental Science and Engineering. Our publication features a wide range of articles, including full-length research papers, review articles, and perspectives, with the aim of enhancing our understanding of the dangers and risks associated with various materials concerning public health and the environment. It is important to note that the term "environmental contaminants" refers specifically to substances that pose hazardous effects through contamination, while excluding those that do not have such impacts on the environment or human health. Moreover, we emphasize the distinction between wastes and hazardous materials in order to provide further clarity on the scope of the journal. We have a keen interest in exploring specific compounds and microbial agents that have adverse effects on the environment.
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