Understanding live oil composition effect on asphaltene precipitation as a function of temperature change during depressurization using machine learning techniques

IF 2.5 4区 化学 Q2 Engineering Chemical Papers Pub Date : 2024-11-16 DOI:10.1007/s11696-024-03784-w
Syed Imran Ali, Shaine Mohammadali Lalji, Zahoor Awan, Saud Hashmi, Nusrat Husain, Firoz Khan, Awatef Salem Balobaid, Ashraf Yahya, Muneeb Burney, Muhammad Qasim, Muhammad Asad, Muhammad Junaid
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Abstract

The study aims to determine the live crude oil compositional feature’s effect on asphaltene precipitation as a function of temperature. In this study, we have applied different modern feature engineering techniques incorporated with machine learning to understand the importance of governing composition features affecting the asphaltene precipitation as a function of temperature during depressurization. To achieve this purpose, different feature selection techniques integrated with the famous random forest (RF) algorithm were applied to the high pressure high temperature (HPTP) experimental data of ten live crude oil samples available in the published literature having outcome as asphaltene precipitation increase or decrease as a result of temperature rise. All data were visualized by using different techniques. Since the data was scarce in the literature, therefore, to avoid overfitting issues the recursive feature elimination with a fourfold cross-validation technique was applied. Random forest algorithm was trained on 60% of the dataset, while testing was done on the remaining 40% dataset. An accuracy of 100% was achieved during the training phase, while it decreased to zero when applied to the testing dataset. The results were validated using a gradient boosting machine (GBM) and found to be in excellent agreement. However, the implementation of other advanced data science techniques aided in improving the accuracy of the testing phase but to very little margin, i.e., from 0 to 25%. Generally, Heavy ends, Light ends and API were found to be the important features in deciding the trend of asphaltene precipitation with temperature changes. Crude oils with higher Heavy ends or decreased API were found to increase asphaltene precipitation when temperature rises. Since, due to the complex relationship of asphaltene precipitation concerning temperature, the study will help in the prediction of the expected trend of asphaltene precipitation for different types of crude oil under field conditions when the temperature will change during production.

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利用机器学习技术了解减压过程中温度变化对活油成分对沥青质沉淀的影响
研究目的是确定原油成分特征对沥青质析出的影响,并以此作为温度的函数。在本研究中,我们将不同的现代特征工程技术与机器学习相结合,以了解减压过程中影响沥青质沉淀的组成特征作为温度函数的重要性。为了实现这一目的,将不同的特征选择技术与著名的随机森林(RF)算法相结合,应用于已发表文献中10个活原油样品的高压高温(HPTP)实验数据,结果表明沥青质沉淀随着温度的升高而增加或减少。使用不同的技术将所有数据可视化。由于文献中数据稀缺,因此,为了避免过拟合问题,采用了四倍交叉验证技术的递归特征消除。随机森林算法在60%的数据集上进行训练,在剩余40%的数据集上进行测试。在训练阶段达到100%的准确率,而在应用于测试数据集时下降到零。用梯度增强机(GBM)对结果进行了验证,结果非常吻合。然而,其他高级数据科学技术的实现有助于提高测试阶段的准确性,但幅度很小,即从0到25%。一般来说,重端、轻端和API是决定沥青质随温度变化趋势的重要特征。当温度升高时,重质端较高或API降低的原油会增加沥青质的析出。由于沥青质析出与温度的复杂关系,本研究有助于预测生产过程中温度变化时不同类型原油在现场条件下沥青质析出的预期趋势。
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来源期刊
Chemical Papers
Chemical Papers Chemical Engineering-General Chemical Engineering
CiteScore
3.30
自引率
4.50%
发文量
590
期刊介绍: Chemical Papers is a peer-reviewed, international journal devoted to basic and applied chemical research. It has a broad scope covering the chemical sciences, but favors interdisciplinary research and studies that bring chemistry together with other disciplines.
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