Electrical Impedance Tomography Monitoring of Salt Transportation in Cellulose Hydrogel for Solar-Driven Evaporative Desalination via Laser Defined Wettability

IF 19 1区 材料科学 Q1 CHEMISTRY, MULTIDISCIPLINARY Advanced Functional Materials Pub Date : 2025-02-05 DOI:10.1002/adfm.202425052
Yang Xu, Haosong Zhong, Xupeng Lu, Miao Tang, Siyu Chen, Cuiyun Yang, Yi Chen, Minseong Kim, Yang Liu, Mitch Guijun Li
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Abstract

The scarcity of clean water has become a growing problem worldwide. Solar-driven desalination based on evaporation has become a promising green technology for obtaining drinking water from saline water for the welfare of human society. However, the accumulation of salt precipitated from the saline at the evaporator surface remains a severe problem in improving evaporation efficiency. To overcome this problem, it is crucial to investigate the transportation mechanism of salt in the saline during the evaporation process. Herein, an in situ monitoring strategy with the electrical impedance tomography (EIT) method is proposed to characterize the salt transportation and accumulation process inside the nano-crystal cellulose (NCC)-MnO2 nanoparticle solar evaporator. The coating of laser-induced graphene (LIG) with tunable water wettability shows that the hydrophobic structures can suppress salt accumulation during evaporation. The collected condensation water generated from the bacteria-polluted saline proves to be clean. It is hoped that this work can further inspire research on the salt-resistive evaporator design.

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利用激光定义润湿性对太阳能驱动蒸发脱盐的纤维素水凝胶中盐运移的电阻抗层析监测
清洁水的短缺已成为一个日益严重的世界性问题。以蒸发为基础的太阳能海水淡化已经成为一项有前途的绿色技术,可以从咸水中获得饮用水,造福人类社会。然而,蒸发器表面沉淀的盐的积累仍然是提高蒸发效率的一个严重问题。为了解决这一问题,研究盐碱蒸发过程中盐的运移机制至关重要。本文采用电阻抗层析成像(EIT)方法对纳米纤维素-二氧化锰太阳能蒸发器内部盐的运移和积累过程进行了原位监测。采用可调水润湿性的激光诱导石墨烯(LIG)涂层表明,疏水结构可以抑制蒸发过程中的盐积累。被细菌污染的盐水产生的冷凝水被证明是清洁的。希望本工作能进一步启发耐盐蒸发器设计的研究。
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来源期刊
Advanced Functional Materials
Advanced Functional Materials 工程技术-材料科学:综合
CiteScore
29.50
自引率
4.20%
发文量
2086
审稿时长
2.1 months
期刊介绍: Firmly established as a top-tier materials science journal, Advanced Functional Materials reports breakthrough research in all aspects of materials science, including nanotechnology, chemistry, physics, and biology every week. Advanced Functional Materials is known for its rapid and fair peer review, quality content, and high impact, making it the first choice of the international materials science community.
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