A bioinspired photothermal evaporator for enhanced salt separation during saline soil remediation

IF 9.8 1区 工程技术 Q1 ENGINEERING, CHEMICAL Desalination Pub Date : 2025-05-01 Epub Date: 2025-02-02 DOI:10.1016/j.desal.2025.118647
Pan Wu , Dalong Zhou , Yuejianshu Li , Xiong Yang , Yafei Shi , Xiong Shi , Gary Owens , Kewu Pi
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Abstract

Soil salinization is a major global challenge for agriculture and ecosystems, with current remediation methods limited by lengthy operation times, high costs, significant energy demands, risk of secondary pollution, and potential for increased soil degradation. Herein, a bioinspired photothermal evaporator (NW-PPy), created by polymerizing pyrrole to form a polypyrrole coating on a nonwoven fabric is introduced as a sustainable soil salinization reduction tool. This synthesis enhanced the material's photothermal efficiency, enabling rapid water evaporation and targeted salt extraction from soil. The NW-PPy evaporator facilitates salt migration from the soil matrix to the evaporator surface, where salt crystallization occurs above the soil surface, effectively isolating salts from the soil and reducing salinity. Under one-sun irradiation, the three-dimensional evaporator achieved a high evaporation rate of 2.47 kg m−2 h−1. A 10-day outdoor trial further demonstrated an 80 % reduction in overall soil salinity. Furthermore, plant cultivation tests to assess relative phytotoxicity indicated significant improvements in lettuce seed germination and stem growth in treated soil. Life cycle assessment (LCA) and techno-economic analysis (TEA) confirmed the evaporator's low environmental impact and economic viability, which underscored that this approach has significant potential as a sustainable solution for saline soil remediation.

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一种用于盐渍土壤修复过程中增强盐分离的生物光热蒸发器
土壤盐碱化是农业和生态系统面临的一个重大全球挑战,目前的修复方法受到操作时间长、成本高、能源需求大、二次污染风险和土壤退化加剧的可能性的限制。本文介绍了一种生物光热蒸发器(NW-PPy),该蒸发器是通过聚合吡咯在非织造布上形成聚吡咯涂层而制成的,是一种可持续的土壤盐渍化减少工具。这种合成提高了材料的光热效率,使水分快速蒸发和从土壤中有针对性地提取盐分成为可能。NW-PPy蒸发器有利于盐从土壤基质迁移到蒸发器表面,盐结晶发生在土壤表面以上,有效地将盐从土壤中分离出来,降低盐分。在单太阳照射下,三维蒸发器的蒸发速率高达2.47 kg m−2 h−1。一项为期10天的室外试验进一步表明,土壤总体盐度降低了80%。此外,评估相对植物毒性的植物栽培试验表明,处理过的土壤显著改善了生菜种子发芽和茎的生长。生命周期评估(LCA)和技术经济分析(TEA)证实了蒸发器的低环境影响和经济可行性,这强调了该方法作为盐碱地修复的可持续解决方案具有巨大的潜力。
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来源期刊
Desalination
Desalination 工程技术-工程:化工
CiteScore
14.60
自引率
20.20%
发文量
619
审稿时长
41 days
期刊介绍: Desalination is a scholarly journal that focuses on the field of desalination materials, processes, and associated technologies. It encompasses a wide range of disciplines and aims to publish exceptional papers in this area. The journal invites submissions that explicitly revolve around water desalting and its applications to various sources such as seawater, groundwater, and wastewater. It particularly encourages research on diverse desalination methods including thermal, membrane, sorption, and hybrid processes. By providing a platform for innovative studies, Desalination aims to advance the understanding and development of desalination technologies, promoting sustainable solutions for water scarcity challenges.
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