Observation of Out-of-Plane Antidamping Torque at the Platinum/Permalloy Interface

IF 8.2 2区 材料科学 Q1 MATERIALS SCIENCE, MULTIDISCIPLINARY ACS Applied Materials & Interfaces Pub Date : 2025-02-07 DOI:10.1021/acsami.4c18895
John Rex Mohan, Utkarsh Shashank, Angshuman Deka, Takayasu Hanashima, Rohit Medwal, Surbhi Gupta, Rajdeep Singh Rawat, Hironori Asada, Yasuhiro Fukuma
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Abstract

Achieving electrical control of ferromagnets without magnetic fields is crucial for the dense integration of nanodevices in modern memory and computing technologies. Current methods using spin orbit torques from the spin Hall effect and interfacial Rashba effect are limited to in-plane magnetized ferromagnets. Out-of-plane antidamping torque is essential for the electrical only control of ferromagnets with perpendicular magnetic anisotropy. In this work, we report the observation of out-of-plane polarized spin currents in platinum/permalloy bilayers, linked to interfacial perpendicular magnetic anisotropy at the interface between two metallic layers, as revealed by polarized neutron reflectometry. In-plane angle-resolved spin-torque ferromagnetic resonance measurements characterized the out-of-plane damping-like torque, constituting about 12% of the total torque in ultrathin Pt films, which vanishes when platinum thickness exceeds 4 nm, confirming its interfacial origin. This interfacial perpendicular magnetic anisotropy-induced torque is significant compared to the bulk spin Hall effect, which can be obtained in a typical heavy metal/ferromagnet bilayer. This advancement holds promise for enhancing the efficiency and reliability of spin orbit torque magnetic random-access memory (SOT-MRAM), spin Hall oscillators, and other spintronic devices.

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铂/坡莫合金界面面外抗阻尼力矩的观察
实现无磁场铁磁体的电气控制是现代存储和计算技术中纳米器件密集集成的关键。目前利用自旋霍尔效应和界面拉什巴效应产生的自旋轨道力矩的方法仅限于平面内磁化的铁磁体。对于具有垂直磁各向异性的铁磁体,面外抗阻尼力矩是电控制所必需的。在这项工作中,我们报告了在铂/坡莫合金双层层中观察到的面外极化自旋电流,这与两个金属层之间界面的垂直磁各向异性有关,这是由极化中子反射仪揭示的。平面内角分辨自旋转矩铁磁共振测量表征了面外类阻尼转矩,约占超薄Pt薄膜总转矩的12%,当铂厚度超过4 nm时,该转矩消失,证实了其界面起源。这种界面垂直磁各向异性诱导的转矩与典型的重金属/铁磁体双分子层中产生的体自旋霍尔效应相比是显著的。这一进展有望提高自旋轨道转矩磁随机存取存储器(SOT-MRAM)、自旋霍尔振荡器和其他自旋电子器件的效率和可靠性。
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来源期刊
ACS Applied Materials & Interfaces
ACS Applied Materials & Interfaces 工程技术-材料科学:综合
CiteScore
16.00
自引率
6.30%
发文量
4978
审稿时长
1.8 months
期刊介绍: ACS Applied Materials & Interfaces is a leading interdisciplinary journal that brings together chemists, engineers, physicists, and biologists to explore the development and utilization of newly-discovered materials and interfacial processes for specific applications. Our journal has experienced remarkable growth since its establishment in 2009, both in terms of the number of articles published and the impact of the research showcased. We are proud to foster a truly global community, with the majority of published articles originating from outside the United States, reflecting the rapid growth of applied research worldwide.
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