Innovative Catalysis Approaches for Methane Utilization

IF 6.7 Q1 ENGINEERING, ENVIRONMENTAL ACS ES&T engineering Pub Date : 2025-02-02 DOI:10.1021/acsestengg.4c00700
Jedy Prameswari,  and , Yu-Chuan Lin*, 
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Abstract

Methane, a potent greenhouse gas (GHG), has exhibited a persistent escalation in emissions from the energy sector. The imperative to mitigate these emissions has become paramount, and one promising avenue is the catalytic conversion of methane into diverse chemicals. This review focuses on the exploration of methane conversion into valuable compounds, including syngas, olefins, and methanol. As advancements in catalysis technology and studies have unfolded, numerous additional insights into the catalytic conversion of methane into novel and significant compounds have surfaced. This review provides an in-depth analysis, focusing predominantly on the latest advancements and cutting-edge innovations in catalytic methane conversion methodologies encompassing methane to acetonitrile and hydrogen cyanide conversion, selective methane conversion to formaldehyde, pyrolysis of methane into solid carbon and hydrogen, and the application of plasma-aided technology. Additionally, it endeavors to elucidate critical parameters and advantages and addresses the intricate array of limitations and future prospects such as theoretical calculations and artificial intelligence (AI)-aided catalyst design.

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甲烷利用的创新催化方法
甲烷是一种强效温室气体(GHG),能源部门的排放量持续上升。减少这些排放的必要性已经变得至关重要,其中一个有希望的途径是将甲烷催化转化为多种化学品。本文综述了甲烷转化为合成气、烯烃和甲醇等有价值化合物的研究进展。随着催化技术和研究的进步,许多关于甲烷催化转化为新型重要化合物的新见解已经浮出水面。本文对甲烷催化转化方法的最新进展和创新进行了深入分析,主要包括甲烷转化乙腈和氰化氢、甲烷选择性转化甲醛、甲烷热解成固体碳和氢以及等离子体辅助技术的应用。此外,它还努力阐明关键参数和优势,并解决了理论计算和人工智能(AI)辅助催化剂设计等一系列复杂的限制和未来前景。
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来源期刊
ACS ES&T engineering
ACS ES&T engineering ENGINEERING, ENVIRONMENTAL-
CiteScore
8.50
自引率
0.00%
发文量
0
期刊介绍: ACS ES&T Engineering publishes impactful research and review articles across all realms of environmental technology and engineering, employing a rigorous peer-review process. As a specialized journal, it aims to provide an international platform for research and innovation, inviting contributions on materials technologies, processes, data analytics, and engineering systems that can effectively manage, protect, and remediate air, water, and soil quality, as well as treat wastes and recover resources. The journal encourages research that supports informed decision-making within complex engineered systems and is grounded in mechanistic science and analytics, describing intricate environmental engineering systems. It considers papers presenting novel advancements, spanning from laboratory discovery to field-based application. However, case or demonstration studies lacking significant scientific advancements and technological innovations are not within its scope. Contributions containing experimental and/or theoretical methods, rooted in engineering principles and integrated with knowledge from other disciplines, are welcomed.
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