Synergistic effect of graphene oxide and glass fiber on mchanical and thermal properties of composites: Experimental and simulation investigations

IF 5.1 3区 工程技术 Q1 CHEMISTRY, APPLIED Reactive & Functional Polymers Pub Date : 2025-05-01 Epub Date: 2025-02-18 DOI:10.1016/j.reactfunctpolym.2025.106201
Long Chen , Jiaxin Liu , Hui Liu , Zhanqiang Liu , Qinghua Song
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Abstract

In this investigation, the effects of short glass fibers and graphene oxide on the thermal and mechanical properties on shape memory composites were investigated. The thermal conductivity results showed that the highest efficiency was achieved at 0.05 wt% graphene oxide, with the heat transfer rate increasing by 22.09 % compared to pure epoxy resin. The addition of short glass fibers improved graphene oxide dispersion, further enhancing thermal conductivity. Mechanical tests indicated that tensile strength increased by 26.8 % at a glass fiber content of 0.15 wt%, while elongation at break improved by 3.51 %, demonstrating the significant role of glass fibers in enhancing both strength and toughness. However, graphene oxide had a limited effect on mechanical properties. Shape memory tests demonstrated a shape fixation rate exceeding 99.4 % and revealed that glass fibers enhanced the shape recovery rate, while graphene oxide improved thermal conductivity, accelerating the recovery process. The short glass fibers and graphene oxide have a synergistic effect on the thermal and mechanical performance of epoxy resin-based shape memory composites, providing valuable data and guidance for optimizing high-performance structural materials.

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氧化石墨烯和玻璃纤维对复合材料力学和热性能的协同效应:实验和模拟研究
在本研究中,研究了短玻璃纤维和氧化石墨烯对形状记忆复合材料热性能和力学性能的影响。导热结果表明,氧化石墨烯在0.05% wt%时效率最高,传热率比纯环氧树脂提高22.09%。短玻璃纤维的加入改善了氧化石墨烯的分散性,进一步增强了导热性。力学试验表明,当玻璃纤维含量为0.15 wt%时,拉伸强度提高26.8%,断裂伸长率提高3.51%,表明玻璃纤维在提高强度和韧性方面都有显著作用。然而,氧化石墨烯对机械性能的影响有限。形状记忆测试表明,形状固定率超过99.4%,并表明玻璃纤维提高了形状恢复率,而氧化石墨烯提高了导热性,加速了恢复过程。短玻璃纤维和氧化石墨烯对环氧树脂基形状记忆复合材料的热性能和力学性能具有协同效应,为优化高性能结构材料提供了有价值的数据和指导。
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来源期刊
Reactive & Functional Polymers
Reactive & Functional Polymers 工程技术-高分子科学
CiteScore
8.90
自引率
5.90%
发文量
259
审稿时长
27 days
期刊介绍: Reactive & Functional Polymers provides a forum to disseminate original ideas, concepts and developments in the science and technology of polymers with functional groups, which impart specific chemical reactivity or physical, chemical, structural, biological, and pharmacological functionality. The scope covers organic polymers, acting for instance as reagents, catalysts, templates, ion-exchangers, selective sorbents, chelating or antimicrobial agents, drug carriers, sensors, membranes, and hydrogels. This also includes reactive cross-linkable prepolymers and high-performance thermosetting polymers, natural or degradable polymers, conducting polymers, and porous polymers. Original research articles must contain thorough molecular and material characterization data on synthesis of the above polymers in combination with their applications. Applications include but are not limited to catalysis, water or effluent treatment, separations and recovery, electronics and information storage, energy conversion, encapsulation, or adhesion.
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