Temperature-stable tunneling current in serial double quantum dots: insights from nonequilibrium green functions and Pauli spin blockade

IF 2.9 3区 化学 Q3 CHEMISTRY, PHYSICAL Physical Chemistry Chemical Physics Pub Date : 2025-02-21 DOI:10.1039/D4CP04224G
David M. T. Kuo
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Abstract

We theoretically investigate charge transport through serial double quantum dots (SDQDs) with strong electron correlations using nonequilibrium Green's function techniques. In the linear response regime, we compute the charge stability diagram and analyze the Coulomb oscillatory tunneling current, revealing both thermal and nonthermal broadening effects on the current spectra in relation to two gate voltages. In the nonlinear response regime, we focus on tunneling currents in SDQDs under the Pauli spin blockade (PSB) scenario. We find that current rectification with negative differential conductance is significantly degraded as temperature increases, making it challenging to distinguish between the inter-site spin triplet and singlet states. Notably, we observe a robust reversed tunneling current that remains stable against temperature variations, provided the resonant channel in the PSB scenario is coupled to the states of the right (left) electrode, which is fully occupied (unoccupied) by particles. This characteristic provides valuable insights for designing transistors capable of operating over a wide temperature range.

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连续双量子点中的温度稳定隧道电流:来自非平衡格林函数和泡利自旋封锁的见解
利用非平衡格林函数技术,从理论上研究了具有强电子相关性的串行双量子点(SDQDs)的电荷输运。在线性响应机制下,我们计算了电荷稳定性图并分析了库仑振荡隧道电流,揭示了与两个栅极电压相关的电流谱的热和非热展宽效应。在非线性响应机制下,我们重点研究了泡利自旋阻滞(PSB)情况下SDQDs中的隧穿电流。我们发现具有负差分电导的电流整流随着温度的升高而显着退化,这使得区分位间自旋三重态和单重态变得具有挑战性。值得注意的是,我们观察到一个强大的反向隧道电流,在温度变化下保持稳定,前提是PSB场景中的谐振通道耦合到右(左)电极的状态,该状态被粒子完全占据(未占据)。这一特性为设计能够在宽温度范围内工作的晶体管提供了有价值的见解。
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来源期刊
Physical Chemistry Chemical Physics
Physical Chemistry Chemical Physics 化学-物理:原子、分子和化学物理
CiteScore
5.50
自引率
9.10%
发文量
2675
审稿时长
2.0 months
期刊介绍: Physical Chemistry Chemical Physics (PCCP) is an international journal co-owned by 19 physical chemistry and physics societies from around the world. This journal publishes original, cutting-edge research in physical chemistry, chemical physics and biophysical chemistry. To be suitable for publication in PCCP, articles must include significant innovation and/or insight into physical chemistry; this is the most important criterion that reviewers and Editors will judge against when evaluating submissions. The journal has a broad scope and welcomes contributions spanning experiment, theory, computation and data science. Topical coverage includes spectroscopy, dynamics, kinetics, statistical mechanics, thermodynamics, electrochemistry, catalysis, surface science, quantum mechanics, quantum computing and machine learning. Interdisciplinary research areas such as polymers and soft matter, materials, nanoscience, energy, surfaces/interfaces, and biophysical chemistry are welcomed if they demonstrate significant innovation and/or insight into physical chemistry. Joined experimental/theoretical studies are particularly appreciated when complementary and based on up-to-date approaches.
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