{"title":"Temperature-stable tunneling current in serial double quantum dots: insights from nonequilibrium green functions and Pauli spin blockade","authors":"David M. T. Kuo","doi":"10.1039/d4cp04224g","DOIUrl":null,"url":null,"abstract":"We theoretically investigate charge transport through serial double quantum dots (SDQDs) with strong electron correlations using nonequilibrium Green's function techniques. In the linear response regime, we compute the charge stability diagram and analyze the Coulomb oscillatory tunneling current, revealing both thermal and nonthermal broadening effects on the current spectra in relation to two gate voltages. In the nonlinear response regime, we focus on tunneling currents in SDQDs under the Pauli spin blockade (PSB) scenario. We find that current rectification with negative differential conductance is significantly degraded as temperature increases, making it challenging to distinguish between the inter-site spin triplet and singlet states. Notably, we observe a robust reversed tunneling current that remains stable against temperature variations, provided the resonant channel in the PSB scenario is coupled to the states of the right (left) electrode, which is fully occupied (unoccupied) by particles. This characteristic provides valuable insights for designing transistors capable of operating over a wide temperature range.","PeriodicalId":99,"journal":{"name":"Physical Chemistry Chemical Physics","volume":"19 1","pages":""},"PeriodicalIF":2.9000,"publicationDate":"2025-02-21","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":null,"platform":"Semanticscholar","paperid":null,"PeriodicalName":"Physical Chemistry Chemical Physics","FirstCategoryId":"92","ListUrlMain":"https://doi.org/10.1039/d4cp04224g","RegionNum":3,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q3","JCRName":"CHEMISTRY, PHYSICAL","Score":null,"Total":0}
引用次数: 0
Abstract
We theoretically investigate charge transport through serial double quantum dots (SDQDs) with strong electron correlations using nonequilibrium Green's function techniques. In the linear response regime, we compute the charge stability diagram and analyze the Coulomb oscillatory tunneling current, revealing both thermal and nonthermal broadening effects on the current spectra in relation to two gate voltages. In the nonlinear response regime, we focus on tunneling currents in SDQDs under the Pauli spin blockade (PSB) scenario. We find that current rectification with negative differential conductance is significantly degraded as temperature increases, making it challenging to distinguish between the inter-site spin triplet and singlet states. Notably, we observe a robust reversed tunneling current that remains stable against temperature variations, provided the resonant channel in the PSB scenario is coupled to the states of the right (left) electrode, which is fully occupied (unoccupied) by particles. This characteristic provides valuable insights for designing transistors capable of operating over a wide temperature range.
期刊介绍:
Physical Chemistry Chemical Physics (PCCP) is an international journal co-owned by 19 physical chemistry and physics societies from around the world. This journal publishes original, cutting-edge research in physical chemistry, chemical physics and biophysical chemistry. To be suitable for publication in PCCP, articles must include significant innovation and/or insight into physical chemistry; this is the most important criterion that reviewers and Editors will judge against when evaluating submissions.
The journal has a broad scope and welcomes contributions spanning experiment, theory, computation and data science. Topical coverage includes spectroscopy, dynamics, kinetics, statistical mechanics, thermodynamics, electrochemistry, catalysis, surface science, quantum mechanics, quantum computing and machine learning. Interdisciplinary research areas such as polymers and soft matter, materials, nanoscience, energy, surfaces/interfaces, and biophysical chemistry are welcomed if they demonstrate significant innovation and/or insight into physical chemistry. Joined experimental/theoretical studies are particularly appreciated when complementary and based on up-to-date approaches.