Quad-narrowband perfect absorption in near infrared for optical switching and sensing based on quasi-bound states in the continuum

IF 2.9 3区 化学 Q3 CHEMISTRY, PHYSICAL Physical Chemistry Chemical Physics Pub Date : 2025-02-21 DOI:10.1039/D5CP00012B
Yuanwen Deng, Boxun Li, Lili Zeng, Qiang Wang, Zhengchao Ma, Yang Fan, Zhengzheng Shao and Chaosheng Deng
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Abstract

The absorption of light based on quasi-BICs is a significant factor influencing the performance of solar cells and photodetectors. Nevertheless, the development of multiple narrowband perfect absorbers remains a significant challenge. In this study, three distinct types of BIC were first discovered to coexist within a metasurface structure. This paper proposes a dual grating metasurface (DGM) structure based on three classes of BICs supported by near-infrared spectroscopy. It achieves perfect absorption in four narrow bands dominated by quasi-BICs, with each of the peaks exceeding 99.5%. The physical mechanism of each resonance has been analysed using temporal coupled mode theory, which has revealed the existence of the Symmetry-Protected BIC, Friedrich–Wintgen BIC and Fabry–Pérot BIC. Moreover, the underlying mechanisms of the distinct resonance modes are revealed through the multipolar decomposition of these resonances. The metasurface has significant potential for utilisation as an optical switch, which is capable of achieving an optimal modulation depth, switching contrast, extinction ratio, and insertion loss of 99.9%, 127 932%, −31.1 dB, and 0.0007 dB, respectively. The DGM structure offers a superior quad-frequency synchronised optical switch in comparison to conventional optical switches. And it also exhibited a maximum sensitivity of 328.6 nm RIU−1 and a maximum FOM of 93.9 RIU−1 when used as a sensor. The work presented herein will facilitate the exploration of a novel avenue for the study of ultra-high performance multifunctional devices based on a multitude of types of BICs.

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基于准束缚态的近红外四窄带完美吸收光开关和传感
基于准bic的光吸收是影响太阳能电池和光电探测器性能的重要因素。然而,多窄带完美吸收器的开发仍然是一个重大挑战。在这项研究中,首次发现三种不同类型的BIC在超表面结构中共存。本文提出了一种基于三种BICs的近红外光谱双光栅超表面结构。在以准bic为主的4个窄波段内均实现了完美的吸收,每个峰均超过99.5%。利用时间耦合模理论分析了每一种共振的物理机制,揭示了对称保护BIC、Friedrich-Wintgen BIC和fabry - prot BIC的存在。此外,通过这些共振的多极分解揭示了不同共振模式的潜在机制。该超表面具有作为光开关的巨大潜力,能够实现最佳的调制深度、开关对比度、消光比和插入损耗,分别为99.9%、127932%、-31.1 dB和0.0007 dB。与传统光开关相比,DGM结构提供了优越的四频同步光开关。当用作传感器时,其最大灵敏度为328.6 nm/RIU,最大FOM为93.9 RIU-1。本文提出的工作将有助于探索基于多种类型bic的超高性能多功能器件研究的新途径。
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来源期刊
Physical Chemistry Chemical Physics
Physical Chemistry Chemical Physics 化学-物理:原子、分子和化学物理
CiteScore
5.50
自引率
9.10%
发文量
2675
审稿时长
2.0 months
期刊介绍: Physical Chemistry Chemical Physics (PCCP) is an international journal co-owned by 19 physical chemistry and physics societies from around the world. This journal publishes original, cutting-edge research in physical chemistry, chemical physics and biophysical chemistry. To be suitable for publication in PCCP, articles must include significant innovation and/or insight into physical chemistry; this is the most important criterion that reviewers and Editors will judge against when evaluating submissions. The journal has a broad scope and welcomes contributions spanning experiment, theory, computation and data science. Topical coverage includes spectroscopy, dynamics, kinetics, statistical mechanics, thermodynamics, electrochemistry, catalysis, surface science, quantum mechanics, quantum computing and machine learning. Interdisciplinary research areas such as polymers and soft matter, materials, nanoscience, energy, surfaces/interfaces, and biophysical chemistry are welcomed if they demonstrate significant innovation and/or insight into physical chemistry. Joined experimental/theoretical studies are particularly appreciated when complementary and based on up-to-date approaches.
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