A lightweight two-stage physics-informed neural network for SOH estimation of lithium-ion batteries with different chemistries

IF 13.1 1区 化学 Q1 Energy Journal of Energy Chemistry Pub Date : 2025-02-18 DOI:10.1016/j.jechem.2025.01.057
Chunsong Lin , Longxing Wu , Xianguo Tuo , Chunhui Liu , Wei Zhang , Zebo Huang , Guiyu Zhang
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Abstract

Accurately estimating the battery state of health (SOH) is essential for ensuring the safe and reliable operation of battery systems of electric vehicles. However, due to the complex and variable operating conditions encountered in practical applications, achieving precise and physics-informed SOH estimation remains challenging. To address these problems, this paper develops a lightweight two-stage physics-informed neural network (TSPINN) method for SOH estimation of lithium-ion batteries with different chemistries. Specifically, this paper utilizes firstly relaxation voltage data obtained after a full charge to determine the aging-related parameters of physical equivalent circuit model (ECM). Additionally, incremental capacity (IC) feature is extracted by analyzing peak values of the IC curve during the charging phase, which thereby constitutes the first stage of the proposed TSPINN, termed as physics-informed data augmentation for SOH estimation. Additionally, the physical information can be further embedded by incorporating feature knowledge related to mechanisms into the loss function, and ultimately, the second stage of the proposed TSPINN is developed, which is named the physics-informed loss function. The effectiveness of the TSPINN method was confirmed through the experimental data for LiNi0.86Co0.11Al0.03O2 (NCA) and LiNi0.83Co0.11Mn0.07O2 (NCM) battery materials under different temperature conditions. The final experimental results indicate that the TSPINN method achieved SOH estimation with a mean absolute error (MAE) of 0.675%, showing improvements of approximately 29.3%, 60.3%, and 8.1% compared to methods using only ECM, IC, and integrated features, respectively. The results validate the effectiveness and adaptability of TSPINN, establishing it as a reliable solution for advanced battery management systems.

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用于估算不同化学成分锂离子电池 SOH 的轻量级两阶段物理信息神经网络
准确估计电池的健康状态(SOH)对于确保电动汽车电池系统的安全可靠运行至关重要。然而,由于在实际应用中会遇到复杂多变的运行条件,实现精确的物理信息 SOH 估算仍具有挑战性。为了解决这些问题,本文开发了一种轻量级两阶段物理信息神经网络(TSPINN)方法,用于估算不同化学成分的锂离子电池的 SOH。具体来说,本文首先利用充满电后获得的弛豫电压数据来确定物理等效电路模型(ECM)的老化相关参数。此外,还通过分析充电阶段 IC 曲线的峰值来提取增量容量 (IC) 特征,从而构成了拟议 TSPINN 的第一阶段,即用于 SOH 估算的物理信息数据增强。此外,物理信息还可以通过将与机制相关的特征知识纳入损失函数来进一步嵌入,最终形成了拟议 TSPINN 的第二阶段,并将其命名为物理信息损失函数。通过对不同温度条件下 LiNi0.86Co0.11Al0.03O2 (NCA) 和 LiNi0.83Co0.11Mn0.07O2 (NCM) 电池材料的实验数据,证实了 TSPINN 方法的有效性。最终实验结果表明,TSPINN 方法实现了 SOH 估算,平均绝对误差 (MAE) 为 0.675%,与仅使用 ECM、IC 和集成特征的方法相比,分别提高了约 29.3%、60.3% 和 8.1%。这些结果验证了 TSPINN 的有效性和适应性,使其成为先进电池管理系统的可靠解决方案。
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来源期刊
Journal of Energy Chemistry
Journal of Energy Chemistry CHEMISTRY, APPLIED-CHEMISTRY, PHYSICAL
CiteScore
19.10
自引率
8.40%
发文量
3631
审稿时长
15 days
期刊介绍: The Journal of Energy Chemistry, the official publication of Science Press and the Dalian Institute of Chemical Physics, Chinese Academy of Sciences, serves as a platform for reporting creative research and innovative applications in energy chemistry. It mainly reports on creative researches and innovative applications of chemical conversions of fossil energy, carbon dioxide, electrochemical energy and hydrogen energy, as well as the conversions of biomass and solar energy related with chemical issues to promote academic exchanges in the field of energy chemistry and to accelerate the exploration, research and development of energy science and technologies. This journal focuses on original research papers covering various topics within energy chemistry worldwide, including: Optimized utilization of fossil energy Hydrogen energy Conversion and storage of electrochemical energy Capture, storage, and chemical conversion of carbon dioxide Materials and nanotechnologies for energy conversion and storage Chemistry in biomass conversion Chemistry in the utilization of solar energy
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