Electronic stopping force of 16O, 19F, 48Ti and 63Cu ions in molybdenum over a continuous energy range of 0.08–0.6 MeV/n

IF 3.9 2区 材料科学 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY Vacuum Pub Date : 2025-03-04 DOI:10.1016/j.vacuum.2025.114210
A. Belalia , A. Guesmia , M. Masenya , Z.M. Khumalo , M. Msimanga , M. Madhuku , C.B. Mtshali , M. Nkosi
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Abstract

In this work, Time-of-Flight spectrometry was used to measure the electronic stopping force of 16O, 19F, 48Ti and 63Cu partially stripped heavy ions crossing Molybdenum over an energy range of (0.08–0.6) MeV/nucleon with errors less than 5 %. Theoretical predictions from the PASS code, SRIM-2013 simulation, Readjusted Bohr Model (RBM) that Guesmia et al. proposed, and the Convolution approximation for swift Particles (CasP) code including electrons capture, were compared with the measured values. While the RBM model, the PASS and CasP codes describe accurately the electronic stopping force in the region where the nuclear stopping force is negligible for 48Ti and 63Cu ions, it turns out to deviate from the experimental data by about 10–25 % in the region where the nuclear stopping force becomes appreciable for the same ions. For 16O and 19F where the studied energy range is near the Bragg's peak, the RBM model and the PASS code describe accurately the electronic stopping force. Even though the SRIM simulation accurately describes the ions (48Ti, 63Cu and 16O), it turns out to deviate from the experimental data by about 10–18 % for 19F.
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钼中的16O、19F、48Ti和63Cu离子在0.08-0.6 MeV/n的连续能量范围内的电子停止力
本文采用飞行时间光谱法测量了16O, 19F, 48Ti和63Cu部分剥离重离子在(0.08-0.6)MeV/核子范围内穿过钼的电子停止力,误差小于5%。将PASS代码的理论预测、SRIM-2013模拟、Guesmia等人提出的rejusted Bohr Model (RBM)以及包含电子捕获的swift Particles (CasP)代码的卷积近似与实测值进行比较。虽然RBM模型、PASS和CasP代码准确地描述了48Ti和63Cu离子在核停止力可以忽略的区域的电子停止力,但在相同离子的核停止力变得明显的区域,电子停止力与实验数据的偏差约为10 - 25%。对于所研究的能量范围接近布拉格峰的16O和19F, RBM模型和PASS代码准确地描述了电子停止力。尽管SRIM模拟准确地描述了离子(48Ti, 63Cu和16O),但结果表明,对于19F,它与实验数据偏差约为10 - 18%。
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来源期刊
Vacuum
Vacuum 工程技术-材料科学:综合
CiteScore
6.80
自引率
17.50%
发文量
0
审稿时长
34 days
期刊介绍: Vacuum is an international rapid publications journal with a focus on short communication. All papers are peer-reviewed, with the review process for short communication geared towards very fast turnaround times. The journal also published full research papers, thematic issues and selected papers from leading conferences. A report in Vacuum should represent a major advance in an area that involves a controlled environment at pressures of one atmosphere or below. The scope of the journal includes: 1. Vacuum; original developments in vacuum pumping and instrumentation, vacuum measurement, vacuum gas dynamics, gas-surface interactions, surface treatment for UHV applications and low outgassing, vacuum melting, sintering, and vacuum metrology. Technology and solutions for large-scale facilities (e.g., particle accelerators and fusion devices). New instrumentation ( e.g., detectors and electron microscopes). 2. Plasma science; advances in PVD, CVD, plasma-assisted CVD, ion sources, deposition processes and analysis. 3. Surface science; surface engineering, surface chemistry, surface analysis, crystal growth, ion-surface interactions and etching, nanometer-scale processing, surface modification. 4. Materials science; novel functional or structural materials. Metals, ceramics, and polymers. Experiments, simulations, and modelling for understanding structure-property relationships. Thin films and coatings. Nanostructures and ion implantation.
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