Engineering-Scale Demonstration of the High CO2 Capture Rate by the Water-Lean Solvent at Technology Centre Mongstad

IF 3.9 3区 工程技术 Q2 ENGINEERING, CHEMICAL Industrial & Engineering Chemistry Research Pub Date : 2025-03-06 DOI:10.1021/acs.iecr.4c04273
Jak Tanthana, Vijay Gupta, Paul Mobley, Marty Lail
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Abstract

NAS, a novel water-lean solvent, has demonstrated its technical and economic feasibility through extensive testing and demonstration projects. This study presents results from a recent campaign conducted at Technology Centre Mongstad, Norway, where NAS was evaluated under high CO2 capture rates for both coal- and natural gas-derived flue gases. With minor process modifications, the NAS operated effectively within the existing amine plant. Accurate mass and energy balances were essential for assessing performance, particularly at high capture rates. The capture rates of 97.63% and 99.72% were achieved under coal- and natural gas- derived (NGCC) flue gas conditions, respectively. The specific reboiler duty of 2.59–2.63 GJ/t-CO2 is reported for coal cases and 3.08–4.19 GJ/t-CO2 for NGCC cases. The study found that NAS consistently outperformed traditional 30 wt % MEA in terms of CO2 avoided costs, with reductions ranging from 36 to 38% across various capture rates. These findings highlight the potential of NAS as a promising solution for efficient and cost-effective CO2 capture.

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蒙斯塔德技术中心低水溶剂高CO2捕集率的工程规模示范
NAS是一种新型的水贫溶剂,通过大量的试验和示范工程证明了其技术和经济可行性。本研究介绍了最近在挪威蒙斯塔德技术中心开展的一项活动的结果,在该中心对煤和天然气衍生烟道气体的高二氧化碳捕获率进行了评价。经过轻微的工艺修改,NAS在现有的胺厂内有效地运行。准确的质量和能量平衡对于评估性能至关重要,特别是在高捕获率的情况下。在煤和天然气衍生(NGCC)烟气条件下,捕集率分别达到97.63%和99.72%。煤的再沸器负荷为2.59-2.63 GJ/t-CO2, NGCC的再沸器负荷为3.08-4.19 GJ/t-CO2。研究发现,NAS在二氧化碳减排成本方面一直优于传统的30% MEA,在不同的捕集率下,减排幅度从36%到38%不等。这些发现突出了NAS作为一种高效且具有成本效益的二氧化碳捕获解决方案的潜力。
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来源期刊
Industrial & Engineering Chemistry Research
Industrial & Engineering Chemistry Research 工程技术-工程:化工
CiteScore
7.40
自引率
7.10%
发文量
1467
审稿时长
2.8 months
期刊介绍: ndustrial & Engineering Chemistry, with variations in title and format, has been published since 1909 by the American Chemical Society. Industrial & Engineering Chemistry Research is a weekly publication that reports industrial and academic research in the broad fields of applied chemistry and chemical engineering with special focus on fundamentals, processes, and products.
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