Micromixing performance of a static mixer with an internal triply periodic minimal surface structure

IF 3.9 3区 工程技术 Q3 ENERGY & FUELS Chemical Engineering and Processing - Process Intensification Pub Date : 2025-06-01 Epub Date: 2025-03-10 DOI:10.1016/j.cep.2025.110264
Xinjun Yang , Xiaohan Lin , Dongxiang Wang , Fangyang Yuan , Wei Yu , Jiyun Du
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Abstract

This study explores TPMS-Diamond structures in static mixers to enhance mixing and reaction processes. Pressure drops were measured in the fine chemicals flow range (0.6–3 L/min), and correlations between Reynolds number, porosity, unit size, and friction factor were established. Energy dissipation rates were calculated, and micromixing performance was evaluated using the Villermaux–Dushman reaction system.The results indicated that micromixing predominantly occurred in the initial contact region, with smaller unit sizes enhancing micromixing performance. When the porosity, ε, is greater than or equal to 0.75, the local energy dissipation rate of the TPMS-Diamond structure was found to be similar to that of the Kenics mixer, yet it achieved significantly better micromixing performance. Additionally, the effects of H+ concentration, flow rate, and volume flow ratio on the micromixing performance of the TPMS-Diamond structure were analyzed. By applying experimental data and agglomeration model techniques, micromixing times for TPMS-Diamond structures with different unit sizes and porosity were determined to range from 0.15 to 1.02 ms, all shorter than those of Kenics mixers. The relationship between micromixing time and energy dissipation rate demonstrates the excellent energy efficiency of TPMS structures. These results demonstrate the substantial potential of TPMS structures in optimizing chemical reaction processes.

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内部三周期最小表面结构静态混合器的微混合性能
本研究在静态混合器中探索TPMS-Diamond结构,以增强混合和反应过程。在精细化学品流量范围(0.6 ~ 3 L/min)内测量了压降,建立了雷诺数、孔隙度、单位尺寸和摩擦系数之间的相关性。计算了能量耗散率,并用Villermaux-Dushman反应体系评价了微混合性能。结果表明,微混合主要发生在初始接触区域,较小的单元尺寸增强了微混合性能。当孔隙率ε大于或等于0.75时,TPMS-Diamond结构的局部能量耗散率与Kenics混合器相似,但微混合性能明显优于Kenics混合器。此外,还分析了H+浓度、流量和体积流比对TPMS-Diamond结构微混合性能的影响。通过实验数据和团聚模型技术,确定了不同单位尺寸和孔隙度的TPMS-Diamond结构的微混合时间在0.15 ~ 1.02 ms之间,均比Kenics混合器的微混合时间短。微混合时间与能量耗散率之间的关系表明TPMS结构具有良好的能量效率。这些结果证明了TPMS结构在优化化学反应过程中的巨大潜力。
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来源期刊
CiteScore
7.80
自引率
9.30%
发文量
408
审稿时长
49 days
期刊介绍: Chemical Engineering and Processing: Process Intensification is intended for practicing researchers in industry and academia, working in the field of Process Engineering and related to the subject of Process Intensification.Articles published in the Journal demonstrate how novel discoveries, developments and theories in the field of Process Engineering and in particular Process Intensification may be used for analysis and design of innovative equipment and processing methods with substantially improved sustainability, efficiency and environmental performance.
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