FGM-LES study of premixed H2/CH4/air flame flashback in a bluff-body swirl burner: The impact of preferential diffusion

IF 5.8 2区 工程技术 Q2 ENERGY & FUELS Combustion and Flame Pub Date : 2025-03-15 DOI:10.1016/j.combustflame.2025.114059
Hao Xia , Weijie Zhang , Wang Han , Jinhua Wang , Zuohua Huang , Jeroen van Oijen
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Abstract

One of the major difficulties to adapt H2-enriched fuels in industrial combustors is the high tendency of flashback. Given the challenge of transient flashback diagnostics in experiment, large eddy simulation (LES) becomes an effective approach to study it. In this study, the flamelet generated manifold (FGM) coupled with LES is applied to simulate the flashback of premixed CH4/air and (95% H2/5% CH4)/air flames in a bluff-body swirl burner established by University of Texas. A revised tabulation method to include the preferential diffusion of H2 was proposed, which is special to also efficiently cover the heat loss and stretch effects. Good agreement between experimental and numerical results is attained as to the flashback mode and speed. It is found that the preferential diffusion of H2 significantly promotes the flashback, which causes increased H2 concentration near the flame front, and leads to higher flame temperature and lower tip–wall distance. The flame front area is also increased with preferential diffusion thus expected to promote the flashback speed.
Novelty and Significance Statement
A revised FGM method including preferential diffusion of hydrogen in the multi-dimension tabulation is proposed and applied to improve hydrogen-enriched flashback prediction. Especially, the varied mixture fraction in the FGM table is attained by varying the inlet mixture components instead of modifying the inlet equivalence ratio as traditionally conducted, which can capture the species and element variation better and cover the heat loss and stretch effects more efficiently. For both flames with or without hydrogen enrichment, the simulated flashback mode and flashback speed correspond well to the experimental results. The flashback behaviors were examined and major reasons for the improved flashback prediction due to the inclusion of hydrogen preferential diffusion were revealed.
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在工业燃烧器中使用富含 H2 的燃料的主要困难之一是容易发生闪蒸。鉴于实验中瞬态闪蒸诊断所面临的挑战,大涡模拟(LES)成为研究闪蒸的有效方法。在本研究中,应用火焰子生成歧管(FGM)与 LES 相结合,模拟了德克萨斯大学建立的崖体漩涡燃烧器中预混合 CH4/空气和(95% H2/5% CH4)/空气火焰的闪蒸。提出了一种包含 H2 优先扩散的修订制表方法,该方法还特别有效地涵盖了热损失和拉伸效应。实验结果和数值结果在闪回模式和速度方面取得了良好的一致。研究发现,H2 的优先扩散显著促进了回火,使火焰前沿附近的 H2 浓度增加,并导致火焰温度升高和顶壁距离减小。新颖性和意义声明提出并应用了在多维表格中包括氢气优先扩散的修正烟气脱硫方法,以改进富氢闪蒸预测。特别是,FGM 表中变化的混合物组分是通过改变入口混合物组分来实现的,而不是像传统方法那样修改入口当量比,这样可以更好地捕捉物种和元素的变化,更有效地覆盖热损失和拉伸效应。对于富氢或不富氢的火焰,模拟闪回模式和闪回速度与实验结果非常吻合。对闪回行为进行了研究,并揭示了由于加入了氢优先扩散而改善闪回预测的主要原因。
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来源期刊
Combustion and Flame
Combustion and Flame 工程技术-工程:化工
CiteScore
9.50
自引率
20.50%
发文量
631
审稿时长
3.8 months
期刊介绍: The mission of the journal is to publish high quality work from experimental, theoretical, and computational investigations on the fundamentals of combustion phenomena and closely allied matters. While submissions in all pertinent areas are welcomed, past and recent focus of the journal has been on: Development and validation of reaction kinetics, reduction of reaction mechanisms and modeling of combustion systems, including: Conventional, alternative and surrogate fuels; Pollutants; Particulate and aerosol formation and abatement; Heterogeneous processes. Experimental, theoretical, and computational studies of laminar and turbulent combustion phenomena, including: Premixed and non-premixed flames; Ignition and extinction phenomena; Flame propagation; Flame structure; Instabilities and swirl; Flame spread; Multi-phase reactants. Advances in diagnostic and computational methods in combustion, including: Measurement and simulation of scalar and vector properties; Novel techniques; State-of-the art applications. Fundamental investigations of combustion technologies and systems, including: Internal combustion engines; Gas turbines; Small- and large-scale stationary combustion and power generation; Catalytic combustion; Combustion synthesis; Combustion under extreme conditions; New concepts.
期刊最新文献
Numerical simulations of direct detonation initiation and propagation in methane/air mixtures containing coal particles Chemical kinetics uncertainty quantification on the dynamic detonation parameters for hydrogen–air mixtures FGM-LES study of premixed H2/CH4/air flame flashback in a bluff-body swirl burner: The impact of preferential diffusion A comparative study of hydrogen and methane enrichment on laminar flame propagation of ammonia Laminar burning velocity and unburnt temperature: Comparative analysis across a broad temperature range of atmospheric NH3+H2 flames
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