Betül Ersöz , Ali Öter , Zeynep Berktaş , Halil İbrahim Bülbül , Antonio Di Bartolomeo , Şeref Sağıroğlu , Elif Orhan
{"title":"Artificial intelligence-driven data generation for temperature-dependent current–voltage characteristics of diodes","authors":"Betül Ersöz , Ali Öter , Zeynep Berktaş , Halil İbrahim Bülbül , Antonio Di Bartolomeo , Şeref Sağıroğlu , Elif Orhan","doi":"10.1016/j.flatc.2025.100847","DOIUrl":null,"url":null,"abstract":"<div><div>Artificial intelligence has the potential to develop models that accurately predict the behavior of electronic devices under various operating conditions. Such models allow researchers to conduct precise performance evaluations during the design phase, reducing development time and costs. For instance, by analyzing the effects of current, voltage, and temperature on diode performance, these models can shorten the diode development cycle and promote sustainable industry growth. In this study, a nanocomposite diode based on lanthanum-doped polyethyleneimine-functionalized graphene quantum dots was fabricated to investigate the impact of temperature on diode performance. The diode's current–voltage characteristics were measured experimentally over a temperature range of 77–400 K. These measurements were used to train machine learning algorithms. Specifically, K-Nearest Neighbors, Decision Trees, and Gradient Boosting were employed to predict current–voltage characteristics at temperatures lacking experimental data. The performance of these models was evaluated using metrics such as the coefficient of determination, mean squared error, and mean absolute error. Among the models, Gradient Boosting demonstrated the highest accuracy, achieving a coefficient of determination of 0.9998, a mean squared error of 0.0026, and a mean absolute error of 0.0222, though accuracy varied with temperature. To test the accuracy of the predicted values, experimental measurements were repeated for the corresponding temperatures, confirming the model's performance. The findings indicate that artificial intelligence-assisted, temperature-dependent data generation can enhance the development of a sustainable diode industry by reducing energy consumption.</div></div>","PeriodicalId":316,"journal":{"name":"FlatChem","volume":"51 ","pages":"Article 100847"},"PeriodicalIF":5.9000,"publicationDate":"2025-03-10","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":null,"platform":"Semanticscholar","paperid":null,"PeriodicalName":"FlatChem","FirstCategoryId":"88","ListUrlMain":"https://www.sciencedirect.com/science/article/pii/S2452262725000418","RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q2","JCRName":"CHEMISTRY, PHYSICAL","Score":null,"Total":0}
引用次数: 0
Abstract
Artificial intelligence has the potential to develop models that accurately predict the behavior of electronic devices under various operating conditions. Such models allow researchers to conduct precise performance evaluations during the design phase, reducing development time and costs. For instance, by analyzing the effects of current, voltage, and temperature on diode performance, these models can shorten the diode development cycle and promote sustainable industry growth. In this study, a nanocomposite diode based on lanthanum-doped polyethyleneimine-functionalized graphene quantum dots was fabricated to investigate the impact of temperature on diode performance. The diode's current–voltage characteristics were measured experimentally over a temperature range of 77–400 K. These measurements were used to train machine learning algorithms. Specifically, K-Nearest Neighbors, Decision Trees, and Gradient Boosting were employed to predict current–voltage characteristics at temperatures lacking experimental data. The performance of these models was evaluated using metrics such as the coefficient of determination, mean squared error, and mean absolute error. Among the models, Gradient Boosting demonstrated the highest accuracy, achieving a coefficient of determination of 0.9998, a mean squared error of 0.0026, and a mean absolute error of 0.0222, though accuracy varied with temperature. To test the accuracy of the predicted values, experimental measurements were repeated for the corresponding temperatures, confirming the model's performance. The findings indicate that artificial intelligence-assisted, temperature-dependent data generation can enhance the development of a sustainable diode industry by reducing energy consumption.
期刊介绍:
FlatChem - Chemistry of Flat Materials, a new voice in the community, publishes original and significant, cutting-edge research related to the chemistry of graphene and related 2D & layered materials. The overall aim of the journal is to combine the chemistry and applications of these materials, where the submission of communications, full papers, and concepts should contain chemistry in a materials context, which can be both experimental and/or theoretical. In addition to original research articles, FlatChem also offers reviews, minireviews, highlights and perspectives on the future of this research area with the scientific leaders in fields related to Flat Materials. Topics of interest include, but are not limited to, the following: -Design, synthesis, applications and investigation of graphene, graphene related materials and other 2D & layered materials (for example Silicene, Germanene, Phosphorene, MXenes, Boron nitride, Transition metal dichalcogenides) -Characterization of these materials using all forms of spectroscopy and microscopy techniques -Chemical modification or functionalization and dispersion of these materials, as well as interactions with other materials -Exploring the surface chemistry of these materials for applications in: Sensors or detectors in electrochemical/Lab on a Chip devices, Composite materials, Membranes, Environment technology, Catalysis for energy storage and conversion (for example fuel cells, supercapacitors, batteries, hydrogen storage), Biomedical technology (drug delivery, biosensing, bioimaging)