Non-metal roofing materials as potential sources of pollutants- laboratory leaching studies on various roofing materials

IF 11.3 1区 环境科学与生态学 Q1 ENGINEERING, ENVIRONMENTAL Journal of Hazardous Materials Pub Date : 2025-07-05 Epub Date: 2025-03-19 DOI:10.1016/j.jhazmat.2025.137972
Julia Udvary , Regina Schwerd , Sabine Johann , Brigitte Helmreich
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Abstract

Stormwater runoff from urban surfaces contains pollutants that harm the water quality of surface or groundwater bodies. While runoff quality from metal roofs has already been widely studied, the contribution of non-metal roofing materials to stormwater pollution is still unclear. A leaching test was conducted to determine the substance emission from non-metal roofing materials. Analyzing parameters in the leachate of eight leaching rounds at predefined time intervals allowed for determining area release rates and leaching mechanisms. The test was conducted with commonly used materials applied on inclined roofs: clay tiles, concrete tiles, fiber cement, bitumen shingles, wood shingles, and plastic roofing tiles. The scope of the analysis is based on substances repeatedly detected in stormwater: anions, cations, heavy metals, biocides, phthalates, PCBs, PFAS, PAHs, nonylphenols, and Bisphenol A. Several roofing materials released relevant amounts of hazardous substances impacting water quality. Clay tiles are a source of vanadium, manganese, and arsenic. Treated wood shingles release ammonium, boron, copper, and Bisphenol A. Fiber cement and concrete roofing tiles are a source of biocides. Bitumen shingles released Bisphenol A. Further research is recommended regarding leaching in long-term field experiments to evaluate the impact of real weather conditions and on developing treatment facilities.

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非金属屋面材料作为污染物的潜在来源-各种屋面材料的实验室浸出研究
来自城市地表的雨水径流含有污染物,会损害地表水或地下水的水质。虽然金属屋顶的径流质量已经得到了广泛的研究,但非金属屋顶材料对雨水污染的贡献仍然不清楚。进行了浸出试验,以确定非金属屋面材料的物质排放。在预先确定的时间间隔内分析8轮浸出液的参数,以确定区域释放速率和浸出机制。试验采用斜屋顶常用材料:粘土瓦、混凝土瓦、纤维水泥、沥青瓦、木瓦和塑料瓦。分析的范围是基于在雨水中反复检测到的物质:阴离子、阳离子、重金属、杀菌剂、邻苯二甲酸盐、多氯联苯、PFAS、PAHs、壬基酚和双酚a。几种屋顶材料释放出影响水质的有害物质。粘土瓦是钒、锰和砷的来源。处理过的木瓦会释放出铵、硼、铜和双酚a。纤维水泥和混凝土瓦片是杀菌剂的来源。沥青瓦释放双酚a,建议在长期现场试验中进一步研究浸出,以评估实际天气条件对发展处理设施的影响。
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来源期刊
Journal of Hazardous Materials
Journal of Hazardous Materials 工程技术-工程:环境
CiteScore
25.40
自引率
5.90%
发文量
3059
审稿时长
58 days
期刊介绍: The Journal of Hazardous Materials serves as a global platform for promoting cutting-edge research in the field of Environmental Science and Engineering. Our publication features a wide range of articles, including full-length research papers, review articles, and perspectives, with the aim of enhancing our understanding of the dangers and risks associated with various materials concerning public health and the environment. It is important to note that the term "environmental contaminants" refers specifically to substances that pose hazardous effects through contamination, while excluding those that do not have such impacts on the environment or human health. Moreover, we emphasize the distinction between wastes and hazardous materials in order to provide further clarity on the scope of the journal. We have a keen interest in exploring specific compounds and microbial agents that have adverse effects on the environment.
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