Dongsheng Ren , Languang Lu , Rui Hua , Gaolong Zhu , Xiang Liu , Yuqiong Mao , Xinyu Rui , Shan Wang , Bosheng Zhao , Hao Cui , Min Yang , Haorui Shen , Chen-Zi Zhao , Li Wang , Xiangming He , Saiyue Liu , Yukun Hou , Tiening Tan , Pengbo Wang , Yoshiaki Nitta , Minggao Ouyang
{"title":"Challenges and opportunities of practical sulfide-based all-solid-state batteries","authors":"Dongsheng Ren , Languang Lu , Rui Hua , Gaolong Zhu , Xiang Liu , Yuqiong Mao , Xinyu Rui , Shan Wang , Bosheng Zhao , Hao Cui , Min Yang , Haorui Shen , Chen-Zi Zhao , Li Wang , Xiangming He , Saiyue Liu , Yukun Hou , Tiening Tan , Pengbo Wang , Yoshiaki Nitta , Minggao Ouyang","doi":"10.1016/j.etran.2023.100272","DOIUrl":null,"url":null,"abstract":"<div><p>All-solid-state batteries (ASSBs) are regarded as the most promising next-generation batteries for electric vehicles in virtue of their potential advantages of enhanced safety, high energy density and power capability. Among the ASSBs based on various solid electrolytes (SEs), sulfide-based ASSBs have attracted increasing attention due to the high ionic conductivity of sulfide SEs which is comparable to that of liquid electrolytes. Extensive efforts from academia and industry have been made to develop sulfide-based ASSBs, and several significant progress has been achieved in recent years. However, successful fabrication of high-performance sulfide-based ASSBs has been rarely reported, and the practical application of sulfide-based ASSBs still faces a variety of challenges. Herein, following a bottom-up approach, we present a comprehensive review of the critical issues of practical sulfide-based ASSBs from the material, interface, composite electrode to cell levels. The existing challenges, recent advances, and future research directions of sulfide-based ASSBs at multiple levels are discussed. Finally, several fabrication processes for scaling up sulfide-based ASSBs and existing pilot/mass production schedules of sulfide-based ASSBs of the leading companies are also introduced. Facing the existing challenges and future opportunities, we highly encourage joint efforts and cooperation across the battery community to promote the practical application of sulfide-based ASSBs.</p></div>","PeriodicalId":36355,"journal":{"name":"Etransportation","volume":null,"pages":null},"PeriodicalIF":15.0000,"publicationDate":"2023-10-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":null,"platform":"Semanticscholar","paperid":null,"PeriodicalName":"Etransportation","FirstCategoryId":"5","ListUrlMain":"https://www.sciencedirect.com/science/article/pii/S2590116823000474","RegionNum":1,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"ENERGY & FUELS","Score":null,"Total":0}
引用次数: 0
Abstract
All-solid-state batteries (ASSBs) are regarded as the most promising next-generation batteries for electric vehicles in virtue of their potential advantages of enhanced safety, high energy density and power capability. Among the ASSBs based on various solid electrolytes (SEs), sulfide-based ASSBs have attracted increasing attention due to the high ionic conductivity of sulfide SEs which is comparable to that of liquid electrolytes. Extensive efforts from academia and industry have been made to develop sulfide-based ASSBs, and several significant progress has been achieved in recent years. However, successful fabrication of high-performance sulfide-based ASSBs has been rarely reported, and the practical application of sulfide-based ASSBs still faces a variety of challenges. Herein, following a bottom-up approach, we present a comprehensive review of the critical issues of practical sulfide-based ASSBs from the material, interface, composite electrode to cell levels. The existing challenges, recent advances, and future research directions of sulfide-based ASSBs at multiple levels are discussed. Finally, several fabrication processes for scaling up sulfide-based ASSBs and existing pilot/mass production schedules of sulfide-based ASSBs of the leading companies are also introduced. Facing the existing challenges and future opportunities, we highly encourage joint efforts and cooperation across the battery community to promote the practical application of sulfide-based ASSBs.
期刊介绍:
eTransportation is a scholarly journal that aims to advance knowledge in the field of electric transportation. It focuses on all modes of transportation that utilize electricity as their primary source of energy, including electric vehicles, trains, ships, and aircraft. The journal covers all stages of research, development, and testing of new technologies, systems, and devices related to electrical transportation.
The journal welcomes the use of simulation and analysis tools at the system, transport, or device level. Its primary emphasis is on the study of the electrical and electronic aspects of transportation systems. However, it also considers research on mechanical parts or subsystems of vehicles if there is a clear interaction with electrical or electronic equipment.
Please note that this journal excludes other aspects such as sociological, political, regulatory, or environmental factors from its scope.