Challenges and opportunities of practical sulfide-based all-solid-state batteries

IF 15 1区 工程技术 Q1 ENERGY & FUELS Etransportation Pub Date : 2023-10-01 DOI:10.1016/j.etran.2023.100272
Dongsheng Ren , Languang Lu , Rui Hua , Gaolong Zhu , Xiang Liu , Yuqiong Mao , Xinyu Rui , Shan Wang , Bosheng Zhao , Hao Cui , Min Yang , Haorui Shen , Chen-Zi Zhao , Li Wang , Xiangming He , Saiyue Liu , Yukun Hou , Tiening Tan , Pengbo Wang , Yoshiaki Nitta , Minggao Ouyang
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Abstract

All-solid-state batteries (ASSBs) are regarded as the most promising next-generation batteries for electric vehicles in virtue of their potential advantages of enhanced safety, high energy density and power capability. Among the ASSBs based on various solid electrolytes (SEs), sulfide-based ASSBs have attracted increasing attention due to the high ionic conductivity of sulfide SEs which is comparable to that of liquid electrolytes. Extensive efforts from academia and industry have been made to develop sulfide-based ASSBs, and several significant progress has been achieved in recent years. However, successful fabrication of high-performance sulfide-based ASSBs has been rarely reported, and the practical application of sulfide-based ASSBs still faces a variety of challenges. Herein, following a bottom-up approach, we present a comprehensive review of the critical issues of practical sulfide-based ASSBs from the material, interface, composite electrode to cell levels. The existing challenges, recent advances, and future research directions of sulfide-based ASSBs at multiple levels are discussed. Finally, several fabrication processes for scaling up sulfide-based ASSBs and existing pilot/mass production schedules of sulfide-based ASSBs of the leading companies are also introduced. Facing the existing challenges and future opportunities, we highly encourage joint efforts and cooperation across the battery community to promote the practical application of sulfide-based ASSBs.

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实用硫化物基全固态电池的挑战和机遇
全固态电池(assb)具有安全性强、能量密度高、动力能力强等潜在优势,被认为是最有前途的下一代电动汽车电池。在基于各种固体电解质(SEs)的assb中,硫化物基assb因其具有与液体电解质相当的高离子电导率而越来越受到人们的关注。近年来,学术界和工业界对硫化物基assb的开发进行了广泛的努力,并取得了一些重大进展。然而,成功制备高性能硫化物基assb的报道很少,硫化物基assb的实际应用仍面临各种挑战。在此,遵循自下而上的方法,我们从材料,界面,复合电极到电池水平全面回顾了实用硫化物基assb的关键问题。从多个层面讨论了硫化物基assb存在的挑战、最新进展和未来的研究方向。最后,还介绍了几种扩大硫化物基assb的制造工艺以及领先公司现有的硫化物基assb中试/量产计划。面对当前的挑战和未来的机遇,我们高度鼓励电池界共同努力与合作,推动硫化物基assb的实际应用。
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来源期刊
Etransportation
Etransportation Engineering-Automotive Engineering
CiteScore
19.80
自引率
12.60%
发文量
57
审稿时长
39 days
期刊介绍: eTransportation is a scholarly journal that aims to advance knowledge in the field of electric transportation. It focuses on all modes of transportation that utilize electricity as their primary source of energy, including electric vehicles, trains, ships, and aircraft. The journal covers all stages of research, development, and testing of new technologies, systems, and devices related to electrical transportation. The journal welcomes the use of simulation and analysis tools at the system, transport, or device level. Its primary emphasis is on the study of the electrical and electronic aspects of transportation systems. However, it also considers research on mechanical parts or subsystems of vehicles if there is a clear interaction with electrical or electronic equipment. Please note that this journal excludes other aspects such as sociological, political, regulatory, or environmental factors from its scope.
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