Confocal photoluminescence characterization of silicon-vacancy color centers in 4H-SiC fabricated by a femtosecond laser

Jiayu Liu , Zongwei Xu , Ying Song , Hong Wang , Bing Dong , Shaobei Li , Jia Ren , Qiang Li , Mathias Rommel , Xinhua Gu , Bowen Liu , Minglie Hu , Fengzhou Fang
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引用次数: 15

Abstract

Silicon-vacancy (VSi) centers in silicon carbide (SiC) are expected to serve as solid qubits, which can be used in quantum computing and sensing. As a new controllable color center fabrication method, femtosecond (fs) laser writing has been gradually applied in the preparation of VSi in SiC. In this study, 4H-SiC was directly written by an fs laser and characterized at 293 K by atomic force microscopy, confocal photoluminescence (PL), and Raman spectroscopy. PL signals of VSi were found and analyzed using 785 nm laser excitation by means of depth profiling and two-dimensional mapping. The influence of machining parameters on the VSi formation was analyzed, and the three-dimensional distribution of VSi defects in the fs laser writing of 4H-SiC was established.

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飞秒激光制备4H-SiC中硅空位色中心的共聚焦光致发光特性
碳化硅(SiC)中的硅空位(VSi)中心有望用作固体量子比特,可用于量子计算和传感。飞秒激光写入作为一种新的可控色心制备方法,已逐渐应用于碳化硅中VSi的制备。在本研究中,4H-SiC由fs激光直接写入,并通过原子力显微镜、共聚焦光致发光(PL)和拉曼光谱在293 K下进行了表征。在785 nm激光激发下,采用深度剖面和二维映射的方法对VSi的PL信号进行了分析。分析了加工参数对VSi形成的影响,建立了fs激光刻蚀4H-SiC过程中VSi缺陷的三维分布。
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