Characteristics of nutrient release from sediments under different flow conditions

Q3 Chemical Engineering Chemical Speciation and Bioavailability Pub Date : 2017-01-01 DOI:10.1080/09542299.2017.1320950
Zhongbo Yu, Xiaoyang Zhong, Cong-rong Yu, Chuanhai Wang, Peiyi Duan, Lei Wen, Yang You
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引用次数: 4

Abstract

Abstract Contaminated sediments, as a secondary pollution source in rivers and lakes, are of critical importance to water quality. More and more attention thus has been paid to understand the release mechanisms of nutrients from river sediments, especially in estuary and water transfer areas. In this work, flume experiments were conducted to measure the release characteristics of total dissolved phosphorus (TDP) and nitrogen (TDN) from sediments collected from a river bed near Lake Tai under various flow conditions. The release of TDP and TDN was the most dramatic in the initial 30 min, then slowed down from 30 to 60 min, and finally achieved equilibria. Total amount of TDP and TDN released and their equilibrium concentrations were all significantly increased with the increase of flow rate, but slow down after a critical velocity was reached, which could be described as a Logarithmic relationship. A process-based mathematical model was established to describe the distribution of nutrients in the water columns and model simulations matched experimental data well. The re-suspension of sediments induced by flow rate higher than the threshold, is the dominant process affecting nutrient release from sediments.
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不同流动条件下沉积物养分释放特征
污染沉积物作为河流和湖泊的二次污染源,对水质有着至关重要的影响。因此,河流沉积物中营养物质的释放机制越来越受到人们的关注,特别是在河口和调水区。通过水槽实验,研究了太湖附近河床沉积物在不同流量条件下的总溶解磷(TDP)和总溶解氮(TDN)的释放特征。TDP和TDN的释放在前30min最为剧烈,在30 ~ 60min逐渐减缓,最终达到平衡。TDP和TDN释放总量及其平衡浓度均随流量的增加而显著增加,但在达到临界流速后下降,呈对数关系。建立了一个基于过程的数学模型来描述水体中营养物的分布,模型模拟结果与实验数据吻合较好。流速大于阈值引起的沉积物再悬浮是影响沉积物养分释放的主要过程。
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来源期刊
CiteScore
1.62
自引率
0.00%
发文量
0
审稿时长
1 months
期刊介绍: Chemical Speciation & Bioavailability ( CS&B) is a scholarly, peer-reviewed forum for insights on the chemical aspects of occurrence, distribution, transport, transformation, transfer, fate, and effects of substances in the environment and biota, and their impacts on the uptake of the substances by living organisms. Substances of interests include both beneficial and toxic ones, especially nutrients, heavy metals, persistent organic pollutants, and emerging contaminants, such as engineered nanomaterials, as well as pharmaceuticals and personal-care products as pollutants. It is the aim of this Journal to develop an international community of experienced colleagues to promote the research, discussion, review, and spread of information on chemical speciation and bioavailability, which is a topic of interest to researchers in many disciplines, including environmental, chemical, biological, food, medical, toxicology, and health sciences. Key themes in the scope of the Journal include, but are not limited to, the following “6Ms”: Methods for speciation analysis and the evaluation of bioavailability, especially the development, validation, and application of novel methods and techniques. Media that sustain the processes of release, distribution, transformation, and transfer of chemical speciation; of particular interest are emerging contaminants, such as engineered nanomaterials, pharmaceuticals, and personal-care products. Mobility of substance species in environment and biota, either spatially or temporally. Matters that influence the chemical speciation and bioavailability, mainly environmentally relevant conditions. Mechanisms that govern the transport, transformation, transfer, and fate of chemical speciation in the environment, and the biouptake of substances. Models for the simulation of chemical speciation and bioavailability, and for the prediction of toxicity. Chemical Speciation & Bioavailability is a fully open access journal. This means all submitted articles will, if accepted, be available for anyone to read, anywhere, at any time. immediately on publication. There are no charges for submission to this journal.
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